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arXiv:2508.20520 · Physical Review A

Superradiant interactions for relic detection with entangled nuclear spins

M.D. Galanis, Onur Hosten, Asimina Arvanitaki, Savas Dimopoulos

Published Apr 27, 2026• 0 citations
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Abstract

We recently showed that macroscopic nuclear spin ensembles prepared in coherent spin states can dramatically enhance the interaction rates of weakly interacting cosmic relics-such as dark matter and the cosmic neutrino background-through collective quantum effects analogous to Dicke superradiance, where the de-excitation and excitation rates scale as the square of the number of spins, $N^2$. We thus coined these processes superradiant interactions. In this paper, we propose a protocol to realize this enhancement and boost the discovery potential for such relics. We show how concepts from quantum optics can be adapted to nuclear spins coupled to superconducting circuits, enabling high-sensitivity systems. The spins are first initialized into a coherent spin state via a $π/2$ Rabi pulse from the ground state. When the circuit is sufficiently detuned from resonance, the spin-circuit interaction implements a squeezing Hamiltonian. Because squeezing must outpace spin relaxation and dephasing, the protocol favors macroscopic ensembles and high-quality superconducting circuits. During this squeezing phase, the standard quantum variance is reduced by up to 4.8 orders of magnitude-equivalent to 48 dB of squeezing-for circuits with quality factors $Q \sim 10^8$-$10^9$. The signal imprinted on the spins during the squeezing protocol can be magnified by further utilizing the squeezing interactions, easing the requirement for shot-noise-limited readout. This protocol has the potential to significantly accelerate axion and dark photon dark matter searches and extend the reach of existing axion experiments to probe QCD axion-nuclear spin couplings. More broadly, it paves the way for detecting coherent inelastic interactions from other cosmic relics-most notably the cosmic neutrino background-and establishes nuclear-spin-based systems as a new class of quantum, ultra-low-threshold detectors.

DOI
10.1103/z2d9-4gv6

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We recently showed that macroscopic nuclear spin ensembles prepared in coherent spin states can dramatically enhance the interaction rates of weakly interacting cosmic relics-such as dark matter and the cosmic neutrino background-through collective quantum effects analogous to Dicke superradiance, where the de-excitation and excitation rates scale as the square of the number of spins, N2N^2N2. We thus coined these processes superradiant interactions. In this paper, we propose a protocol to realize this enhancement and boost the discovery potential for such relics. We show how concepts from quantum optics can be adapted to nuclear spins coupled to superconducting circuits, enabling high-sensitivity systems. The spins are first initialized into a coherent spin state via a π/2π/2π/2 Rabi pulse from the ground state. When the circuit is sufficiently detuned from resonance, the spin-circuit interaction implements a squeezing Hamiltonian. Because squeezing must outpace spin relaxation and dephasing, the protocol favors macroscopic ensembles and high-quality superconducting circuits. During this squeezing phase, the standard quantum variance is reduced by up to 4.8 orders of magnitude-equivalent to 48 dB of squeezing-for circuits with quality factors Q∼108Q \sim 10^8Q∼108-10910^9109. The signal imprinted on the spins during the squeezing protocol can be magnified by further utilizing the squeezing interactions, easing the requirement for shot-noise-limited readout. This protocol has the potential to significantly accelerate axion and dark photon dark matter searches and extend the reach of existing axion experiments to probe QCD axion-nuclear spin couplings. More broadly, it paves the way for detecting coherent inelastic interactions from other cosmic relics-most notably the cosmic neutrino background-and establishes nuclear-spin-based systems as a new class of quantum, ultra-low-threshold detectors.
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Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter.
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Abstract Nuclear magnetic resonance is a promising experimental approach to search for ultra-light axion-like dark matter. Searches such as the cosmic axion spin-precession experiments (CASPEr) are ultimately limited by quantum-mechanical noise sources, in particular, spin-projection noise. We discuss how such fundamental limits can potentially be reached. We consider a circuit model of a magnetic resonance experiment and quantify three noise sources: spin-projection noise, thermal noise, and amplifier noise. Calculation of the total noise spectrum takes into account the modification of the circuit impedance by the presence of nuclear spins, as well as the circuit back-action on the spin ensemble. Suppression of the circuit back-action is especially important in order for the spin-projection noise limits of searches for axion-like dark matter to reach the quantum chromodynamic axion sensitivity.
Quantum amplification is recognized as a key resource for precision measurements. However, most conventional paradigms employ an ensemble of independent particles that usually limit the performance of quantum amplification in gain, spectral linewidth, etc. Here we demonstrate a new signal amplification using cooperative 129Xe nuclear spins embedded within a feedback circuit, where the noble-gas spin coherence time is enhanced by at least one order of magnitude. Using such a technique, magnetic field can be substantially pre-enhanced by more than three orders and is in situ readout with an embedded 87Rb magnetometer. We realize an ultrahigh magnetic sensitivity of 4.0 fT/Hz1/2^{1/2}1/2 that surpasses the photon-shot noise and even below the spin-projection noise of the embedded atomic magnetometer, allowing for exciting applications including searches for dark matter with sensitivity well beyond supernova constraints. Our findings extend the physics of quantum amplification to cooperative spin systems and can be generalized to a wide variety of existing sensors, enabling a new class of cooperative quantum sensors.
Conventional nuclear magnetic resonance searches for the galactic axion wind lose sensitivity at low frequencies due to the unfavourable scaling of inductive readout. Here, we propose a hybrid architecture where the hyperfine interaction transduces axion-driven nuclear precession into a high-bandwidth electron-spin readout channel. We demonstrate analytically that this dispersive upconversion preserves the specific sidereal and annual modulation signatures required to distinguish dark matter signals from instrumental backgrounds. When instantiated in a silicon 209Bi{ }^{209} \text{Bi}209Bi donor platform, the hybrid sensor is projected to outperform direct nuclear detection by more than an order of magnitude over the 10−16−10−10eV10^{-16}-10^{-10} \text{eV}10−16−10−10eV wide mass range. With collective enhancement, the design reaches a 5σ5 σ5σ sensitivity to DFSZ axion-nucleon couplings within one year, establishing hyperfine-mediated sensing as a competitive path for compact, solid-state dark matter searches.