Electromagnetic radiation by accelerated charges is a fundamental process in physics. Here, we introduce a quantum-optical framework for controlling the emission of radiation of an electron in an intense laser field via squeezed vacuum states. By engineering the quantum fluctuations of the emission modes, we demonstrate that the probability of nonlinear Compton scattering can be significantly enhanced or suppressed through tunable squeezing amplitude and angle. We show numerically that our predictions are experimentally accessible with current squeezing technologies, establishing a new paradigm for quantum control in high-intensity light-matter interactions.
Electromagnetic radiation by accelerated charges is a fundamental process in physics. Here, we introduce a quantum-optical framework for controlling the emission of radiation of an electron in an intense laser field via squeezed vacuum states. By engineering the quantum fluctuations of the emission modes, we demonstrate that the probability of nonlinear Compton scattering can be significantly enhanced or suppressed through tunable squeezing amplitude and angle. We show numerically that our predictions are experimentally accessible with current squeezing technologies, establishing a new paradigm for quantum control in high-intensity light-matter interactions.
When an electron is accelerated, it emits radiation. In the relativistic quantum realm the elementary radiation process is the emission of a single photon, a process known as nonlinear Compton scattering in the case of an electron moving in the presence of a strong electromagnetic wave. This process is typically described within the Furry picture, where the electromagnetic wave is described as a classical background field and the electron-positron field is quantized in the presence of that background field. Equivalently one can quantize the electron-positron field in the vacuum but then the photon emission process is described as a transition from an initial state to a final state both featuring, apart from the electron (the initial state) and the electron and the photon (the final state), the same coherent state of photons appropriately related to the electromagnetic wave. Here, we consider a more general situation where the initial and the final state feature the same squeezed coherent state. Then, we specialize to the case where the coherent state corresponds to a plane-wave field and the mostly populated modes of the coherent state are also squeezed. We show that, when quantum fluctuations induced by the squeezing in the coherent field are negligible, a condition well satisfied at available squeezing levels, the squeezing effects effectively reduce to a frequency modulation of the plane-wave field corresponding to the coherent state. By means of numerical examples we show that at already available squeezing levels the emission spectrum of nonlinear Compton scattering and the total photon yield can be altered significantly. Analytical explanations of the main numerical results are also provided.
We develop a fully quantized theory of nonlinear Compton scattering driven by a single-mode quantum field. Exact quantum-Volkov states retain pump depletion, back-action, and final-state correlations through displaced or squeezed-displaced Fock-state ladders. A finite Fock-state pump produces discrete photon-transfer edges and a terminal spectral cutoff. In the bright, weakly depleted regime, the exact theory reduces to a Wigner-function weighted-average of scattering probabilities evaluated at fixed complex field amplitudes, with ordinary and generalized Bessel functions describing the harmonic structure for circular and linear polarization, respectively. For squeezed coherent light, the squeezing angle controls the high-energy emission through photon-number fluctuations.
Nonlinear optical processes, mediated by multiphoton interactions rather than single-photon response, are routinely exploited to enable a range of light-based functionalities in devices and applications. Nonlinear effects are enhanced through higher intensity fields, which is a limiting strategy owing to potential radiation damage. An alternative strategy relies on the fluctuation redistribution typical of quantum light, but experimental demonstrations at the most fundamental level have been limited. Here we report experimental nonlinear tunnelling ionization of isolated atoms, a pivotal nonlinear process that drives high-harmonic generation and forms the basis of attosecond science, boosted by quantum light -- bright squeezed vacuum (BSV). A BSV light with an average pulse energy of 300 nJ achieves an effective intensity equivalent to that of a coherent light with 7.1 {\textmu}J, demonstrating a more than 20-fold quantum boost in nonlinear effect from BSV light. This boost is revealed by matching the peaks of the photoelectron momentum spectra produced by the BSV and coherent light using angular streaking. Furthermore, we demonstrate control of the effective intensity of the BSV by tuning the correlation function at fixed average pulse energy, establishing a robust method to tailor nonlinear processes via quantum statistics rather than classical intensity scaling. These findings may facilitate the development of quantum-controlled strong-field dynamics using tailored quantum light sources.
The extreme light-matter interaction has brought unique tools for the subfemtosecond control of electron dynamics [1] and ultra-fast spectroscopy [2]. Until recently, the strong-field regime was accessible only with coherent states of light, which can be well described by classical electric fields when many photons are present (Fig. 1a). With the use of intense states of non-classical light, this situation has changed. New opportunities emerge with bright squeezed vacuum (BSV), which can be generated from optical parametric amplification of quantum vacuum fluctuations. Unlike classical light, BSV is a quantum superposition of coherent states with an amplitudes spanning a range from zero to very high values, up to ~1 TW/cm2[3]. BSV has a zero mean electric field and the variance of the electric field oscillates at the double carrier frequency (Fig. 1a). How such a non-classical electric field can affect the dynamics of photoemitted electrons was theoretically demonstrated recently [4]. Furthermore, the photon-number distribution of BSV has a very long tail in contrast to coherent light. These photon-number distributions can be imprinted onto the photon statistics of optical harmonics [3] and the statistics of electrons [5].
Squeezed coherent quantum light is described by the complex squeeze parameter ζ = s e i ϑ and the coherent-state displacement parameter β = | β | e i ϕ β . Our study of strong-field ionization [D. Habibović and D. B. Milošević, ], which focused on bright squeezed vacuum quantum light with β = 0 and s ≫ 1 , is extended to ionization by squeezed coherent light. It is shown that the amplitudes s and | β | strongly influence the ionization process, whereas phases ϑ and ϕ β play a less significant role. The present work provides a unified treatment of coherent, squeezed vacuum, and squeezed coherent light within a single theoretical framework. The quantum nature of the driving field is incorporated by averaging the strong-field ionization probability over the Husimi-Kano phase-space distribution. Using neon as a representative target, we analyze how the parameters characterizing squeezed coherent light modify photoelectron spectra and intensity-dependent enhancements. We show that nonclassical photon statistics can lead to a pronounced steepening of the rescattering plateau and, at low mean intensities, to an effective suppression of the nominal high-energy cutoff. These effects originate from the reduced weight of high-intensity field components inherent to squeezed states and have no analog in strong-field ionization driven by a coherent light. Our results highlight the potential for quantum-statistical control of strong-field ionization and provide a foundation for exploring laser-matter interactions driven by quantum light.
Squeezed optical fields are a powerful resource for a variety of investigations in basic research and technology. However, the generation of intense squeezed light is challenging. Here, we show that intense squeezed light can be produced using strongly laser driven atoms and the so far unrelated process of high harmonic generation. We demonstrate that when the intensity of the driving field significantly depletes the ground state of the atoms, leading to dipole moment correlations, the quantum state of the driving field and the generated high harmonics are entangled and squeezed. Furthermore, we analyze how the resulting quadrature squeezing of the fundamental laser mode after the interaction can be controlled. The findings open the way for the generation of high intensity squeezed light states for a wide range of applications.