Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2507.17823

Two-dimensional nonlinear dynamical response of the magnetoelectrically driven dimerized spin-$1{/}2$ chain

Wolfram Brenig

Published Jul 23, 2025• 0 citations
arXivHTMLPDF

Abstract

A study of the dynamical two-dimensional (2D) nonlinear response of the dimerized spin-$1{/}2$ chain to external electric fields is presented. The coupling of the spin system to those fields is set to arise from the inverse Dzyaloshinskii-Moriya interaction. In the XY-limit, we provide analytical expressions for the second-order nonlinear dynamical response function. Apart from multi spinon continua, this response displays a strong antidiagonal, i.e. galvanoelectric, feature in the 2D frequency plane. This allows to read off scattering rates of the fractional spinon excitations. For the XXZ-case, we focus on the interaction-driven renormalization of the light-matter coupling by considering vertex corrections which are induced by the zz-exchange. We show this renormalization to modify the spinon joint density of states significantly, potentially allowing for the formation of in-gap bound states. As a result, the vertex corrected light-matter coupling can induce a dramatic spectral weight transfer to lower energies for the dynamical response function within the 2D frequency plane.

DOI
10.48550/arxiv.2507.17823

Related papers

2DNL dynamical response of the magnetoelectrically driven dimerized XXZ-chain

Wolfram Brenig

A study of the dynamical two-dimensional (2D) nonlinear response of the dimerized spin-1/2 chain to external electric fields is presented. The coupling of the spin system to light is set to arise from the inverse Dzyaloshinskii-Moriya interaction. In the XY-limit, we provide analytical expressions for the second-order nonlinear dynamical response function. Apart from multi spinon continua, this response displays a strong antidiagonal, i.e. galvanoelectric, feature in the 2D frequency plane. This allows to read off scattering rates of the fractional spinon excitations. For the XXZ-case, we focus on the interaction-driven renormalization of the light-matter coupling by considering vertex corrections which are induced by the zz-exchange. We show this renormalization to modify the spinon joint density of states significantly, potentially allowing for the formation of in-gap bound states. As a result, the vertex corrected light-matter coupling can induce a dramatic spectral weight transfer to lower energies for the dynamical response function within the 2D frequency plane.

Journal of Physics Condensed Matter•Oct 20, 2026•0 citations

Response functions for electric field induced two-dimensional nonlinear spectroscopy in a Kitaev magnet

Wolfram Brenig, Olesia Krupnitska

We study the dynamical response functions relevant for electric field induced two-dimensional (2D) coherent nonlinear optical spectroscopy in a Kitaev magnet at finite temperature. We show that these response functions are susceptible to both types of fractional quasiparticles of this quantum spin-liquid, i.e. fermions and flux visons. Focusing on the second order response, we find a strong antidiagonal feature in the 2D frequency plane, related to the galvanoelectric effect of the fractional fermions. Perpendicular to the antidiagonal, the width of this feature is set by quasiparticle relaxation rates beyond the bare Kitaev magnet, thereby providing access to single-particle characteristics within a multi-particle continuum. While the 2D spectrum of the response is set by the fermionic quasiparticles and displays Fermi blocking versus temperature, the emergent bond randomness which arises due to thermally populated visons strongly modifies the fermionic spectrum. Therefore also the presence of gauge excitations is manifest in the 2D nonlinear response as the temperature is increased beyond the flux proliferation crossover.

Journal of Physics Condensed Matter•Sep 13, 2024•6 citations

Finite temperature electric field induced two-dimensional coherent nonlinear spectroscopy in a Kitaev magnet

Wolfram Brenig, Olesia Krupnitska

We study electric field induced two-dimensional coherent nonlinear optical spectroscopy (2DCS) in a Kitaev magnet at finite temperature. We show that 2DCS is susceptible to both types of fractional quasiparticles of this quantum spin-liquid, i.e., fermions and flux visons. Focusing on the second order response, we find a strong antidiagonal feature in the two-dimensional frequency plane, related to the galvanoelectric effect of the fractional fermions. Perpendicular to the antidiagonal, the width of this feature is set by quasiparticle relaxation rates beyond the bare Kitaev magnet, thereby providing access to single-particle characteristics within the multi-particle 2DCS continuum. While the structure of the 2DCS susceptibility stems from the fermionic quasiparticles and displays Fermi blocking versus temperature, the emergent bond randomness which arises due to thermally populated visons strongly modifies the fermionic spectrum. Therefore also the presence of gauge excitations is manifest in the 2DCS susceptibility as the temperature is increased beyond the flux proliferation crossover. Our results are consistent with and extend previous findings on second harmonic generation in Kitaev magnets.

arXiv:2403.08867•Mar 13, 2024•0 citations

Spin-1/2 XY chain magnetoelectric: Effect of zigzag geometry

O. R. Baran, Vadim Ohanyan, Taras Verkholyak

A spin-1/2 $XY$ chain model of magnetoelectrics on a zigzag chain is considered rigorously. The magnetoelectric coupling is described within the Katsura-Nagaosa-Balatsky mechanism. In the zigzag geometry it leads to the staggered Dzyaloshinskii-Moriya interaction. Using nonuniform spin rotations, the model is reduced to a dimerized $XY$ chain and solved exactly using the Jordan-Wigner transformation. We analyze the ground-state phase diagram of the model and the zero- and finite-temperature magnetoelectric effects and obtain the magnetization and polarization curves versus magnetic and electric fields, as well as the parameters of anisotropic dielectric and magnetoelectric response. It is also shown that the electric field may enhance the magnetocaloric effect in the model.

arXiv:1805.08442•Physical review. B./Physical review. B•Aug 20, 2018•13 citations

Exact description of magnetoelectric effect in the spin- 12 XXZ chain with Dzyaloshinskii-Moriya interaction

Michael Brockmann, Andreas Klümper, Vadim Ohanyan

We consider a simple integrable model of a spin chain exhibiting the magnetoelectric effect (MEE). Starting from the periodic $S=1/2$ XXZ chain with Dzyaloshinskii-Moriya terms, which we consider as a local electric polarization in the spirit of the Katsura-Nagaosa-Baladsky (KNB) mechanism, we perform the mapping onto the conventional XXZ chain with twisted boundary conditions. Using the techniques of quantum transfer matrix and nonlinear integral equations we obtain the magnetization, electric polarization, and magnetoelectric tensor as functions of magnetic and electric field for arbitrary temperatures. We investigate these dependencies as well as the thermal behavior of the above-mentioned physical quantities, especially in the low-temperature regime. We found several regimes of polarization. Adjusting the magnetic field one can switch the system from one regime to another. The features of the critical properties connected with the MEE are also illustrated.

arXiv:1210.7693•Physical Review B•Feb 8, 2013•42 citations

Heisenberg spin- 12 XXZ chain in the presence of electric and magnetic fields

Pradeep K. Thakur, P. Durganandini

We study the interplay of electric and magnetic order in the one-dimensional Heisenberg spin-$\frac{1}{2}$ XXZ chain with large Ising anisotropy in the presence of the Dzyaloshinskii-Moriya (DM) interaction and with longitudinal and transverse magnetic fields, interpreting the DM interaction as a coupling between the local electric polarization and an external electric field. We obtain the ground state phase diagram using the density matrix renormalization group method and compute various ground state quantities like the magnetization, staggered magnetization, electric polarization and spin correlation functions, etc. In the presence of both longitudinal and transverse magnetic fields, there are three different phases corresponding to a gapped N\'eel phase with antiferromagnetic (AF) order, gapped saturated phase, and a critical incommensurate gapless phase. The external electric field modifies the phase boundaries but does not lead to any new phases. Both external magnetic fields and electric fields can be used to tune between the phases. We also show that the transverse magnetic field induces a vector chiral order in the N\'eel phase (even in the absence of an electric field) which can be interpreted as an electric polarization in a direction parallel to the AF order.

arXiv:1801.10509•Physical review. B./Physical review. B•Feb 20, 2018•14 citations
Two-dimensional nonlinear dynamical response of the magnetoelectrically driven dimerized spin-1/21{/}21/2 chain
A study of the dynamical two-dimensional (2D) nonlinear response of the dimerized spin-1/21{/}21/2 chain to external electric fields is presented. The coupling of the spin system to those fields is set to arise from the inverse Dzyaloshinskii-Moriya interaction. In the XY-limit, we provide analytical expressions for the second-order nonlinear dynamical response function. Apart from multi spinon continua, this response displays a strong antidiagonal, i.e. galvanoelectric, feature in the 2D frequency plane. This allows to read off scattering rates of the fractional spinon excitations. For the XXZ-case, we focus on the interaction-driven renormalization of the light-matter coupling by considering vertex corrections which are induced by the zz-exchange. We show this renormalization to modify the spinon joint density of states significantly, potentially allowing for the formation of in-gap bound states. As a result, the vertex corrected light-matter coupling can induce a dramatic spectral weight transfer to lower energies for the dynamical response function within the 2D frequency plane.
A study of the dynamical two-dimensional (2D) nonlinear response of the dimerized spin-1/2 chain to external electric fields is presented. The coupling of the spin system to light is set to arise from the inverse Dzyaloshinskii-Moriya interaction. In the XY-limit, we provide analytical expressions for the second-order nonlinear dynamical response function. Apart from multi spinon continua, this response displays a strong antidiagonal, i.e. galvanoelectric, feature in the 2D frequency plane. This allows to read off scattering rates of the fractional spinon excitations. For the XXZ-case, we focus on the interaction-driven renormalization of the light-matter coupling by considering vertex corrections which are induced by the zz-exchange. We show this renormalization to modify the spinon joint density of states significantly, potentially allowing for the formation of in-gap bound states. As a result, the vertex corrected light-matter coupling can induce a dramatic spectral weight transfer to lower energies for the dynamical response function within the 2D frequency plane.
We study the dynamical response functions relevant for electric field induced two-dimensional (2D) coherent nonlinear optical spectroscopy in a Kitaev magnet at finite temperature. We show that these response functions are susceptible to both types of fractional quasiparticles of this quantum spin-liquid, i.e. fermions and flux visons. Focusing on the second order response, we find a strong antidiagonal feature in the 2D frequency plane, related to the galvanoelectric effect of the fractional fermions. Perpendicular to the antidiagonal, the width of this feature is set by quasiparticle relaxation rates beyond the bare Kitaev magnet, thereby providing access to single-particle characteristics within a multi-particle continuum. While the 2D spectrum of the response is set by the fermionic quasiparticles and displays Fermi blocking versus temperature, the emergent bond randomness which arises due to thermally populated visons strongly modifies the fermionic spectrum. Therefore also the presence of gauge excitations is manifest in the 2D nonlinear response as the temperature is increased beyond the flux proliferation crossover.
We study electric field induced two-dimensional coherent nonlinear optical spectroscopy (2DCS) in a Kitaev magnet at finite temperature. We show that 2DCS is susceptible to both types of fractional quasiparticles of this quantum spin-liquid, i.e., fermions and flux visons. Focusing on the second order response, we find a strong antidiagonal feature in the two-dimensional frequency plane, related to the galvanoelectric effect of the fractional fermions. Perpendicular to the antidiagonal, the width of this feature is set by quasiparticle relaxation rates beyond the bare Kitaev magnet, thereby providing access to single-particle characteristics within the multi-particle 2DCS continuum. While the structure of the 2DCS susceptibility stems from the fermionic quasiparticles and displays Fermi blocking versus temperature, the emergent bond randomness which arises due to thermally populated visons strongly modifies the fermionic spectrum. Therefore also the presence of gauge excitations is manifest in the 2DCS susceptibility as the temperature is increased beyond the flux proliferation crossover. Our results are consistent with and extend previous findings on second harmonic generation in Kitaev magnets.
A spin-1/2 XYXYXY chain model of magnetoelectrics on a zigzag chain is considered rigorously. The magnetoelectric coupling is described within the Katsura-Nagaosa-Balatsky mechanism. In the zigzag geometry it leads to the staggered Dzyaloshinskii-Moriya interaction. Using nonuniform spin rotations, the model is reduced to a dimerized XYXYXY chain and solved exactly using the Jordan-Wigner transformation. We analyze the ground-state phase diagram of the model and the zero- and finite-temperature magnetoelectric effects and obtain the magnetization and polarization curves versus magnetic and electric fields, as well as the parameters of anisotropic dielectric and magnetoelectric response. It is also shown that the electric field may enhance the magnetocaloric effect in the model.
We consider a simple integrable model of a spin chain exhibiting the magnetoelectric effect (MEE). Starting from the periodic S=1/2S=1/2S=1/2 XXZ chain with Dzyaloshinskii-Moriya terms, which we consider as a local electric polarization in the spirit of the Katsura-Nagaosa-Baladsky (KNB) mechanism, we perform the mapping onto the conventional XXZ chain with twisted boundary conditions. Using the techniques of quantum transfer matrix and nonlinear integral equations we obtain the magnetization, electric polarization, and magnetoelectric tensor as functions of magnetic and electric field for arbitrary temperatures. We investigate these dependencies as well as the thermal behavior of the above-mentioned physical quantities, especially in the low-temperature regime. We found several regimes of polarization. Adjusting the magnetic field one can switch the system from one regime to another. The features of the critical properties connected with the MEE are also illustrated.
We study the interplay of electric and magnetic order in the one-dimensional Heisenberg spin-12\frac{1}{2}21​ XXZ chain with large Ising anisotropy in the presence of the Dzyaloshinskii-Moriya (DM) interaction and with longitudinal and transverse magnetic fields, interpreting the DM interaction as a coupling between the local electric polarization and an external electric field. We obtain the ground state phase diagram using the density matrix renormalization group method and compute various ground state quantities like the magnetization, staggered magnetization, electric polarization and spin correlation functions, etc. In the presence of both longitudinal and transverse magnetic fields, there are three different phases corresponding to a gapped N\'eel phase with antiferromagnetic (AF) order, gapped saturated phase, and a critical incommensurate gapless phase. The external electric field modifies the phase boundaries but does not lead to any new phases. Both external magnetic fields and electric fields can be used to tune between the phases. We also show that the transverse magnetic field induces a vector chiral order in the N\'eel phase (even in the absence of an electric field) which can be interpreted as an electric polarization in a direction parallel to the AF order.