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arXiv:2507.16549

Probing subradiant dynamics in cold atomic ensembles via population and emitted light measurements

Antoine Glicenstein, Daniel Benedicto Orenes, Apoorva Apoorva, R. Saint-Jalm, Robin Kaiser

Published Jul 22, 2025• 0 citations
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Abstract

In this letter, we report on the time- and space-resolved measurement of subradiant excited state population in an ultra-cold atomic cloud of 174Yb atoms. We use a depletion imaging technique that exploits the V-type internal energy structure of alkaline-earth-like atoms to directly observe the time-resolved spatial distribution of excited state population. We characterize the decay dynamics of the subradiant modes using both the excited state population and scattered light intensity, finding good quantitative agreement with numerical predictions from simulations of two-level atomic ensembles.

DOI
10.48550/arxiv.2507.16549

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This study introduces a novel method to investigate in situ light transport within optically thick ensembles of cold atoms, exploiting the internal structure of alkaline-earth metals. A method for creating an optical excitation at the center of a large atomic cloud is demonstrated, and we observe its propagation through multiple scattering events. In conditions where the cloud size is significantly larger than the transport mean free path, a diffusive regime is identified. We measure key parameters, including the diffusion coefficient, transport velocity, and transport time, finding a good agreement with diffusion models. We also demonstrate that the frequency of the photons launched inside the system can be controlled. This approach enables direct time- and space-resolved observation of light diffusion in atomic ensembles, offering a promising avenue for exploring new diffusion regimes.
In this work we present a numerical and experimental investigation of the collective early-time decay rates of a strongly driven and optically dense cold atomic cloud. We prepare the atomic ensemble by driving the system to its steady state with varying Rabi frequencies ΩΩΩ that go from the weak Ω≪ΓΩ\ll ΓΩ≪Γ to the strong driving regime Ω≫ΓΩ\gg ΓΩ≫Γ, where ΓΓΓ is the single-atom decay rate. We investigate the early-time dynamics in the transition between the strong and weak driving regimes using: i) angular-dependent observables such as the light emitted by the cloud, and ii) global observables, i.e., the excited state population. When driving the cloud on-resonance, we find that as a function of the driving frequency, the behavior of the collected light at certain angles transitions from the single-photon subradiant regime to a superradiant regime while the behavior of the excited state population does not show superradiance. The experiment shows good agreement with numerical predictions in the regime of parameters under study.
This study introduces a novel method to investigate in-situ light transport within optically thick ensembles of cold atoms, exploiting the internal structure of alkaline-earth metals. A method for creating an optical excitation at the center of a large atomic cloud is demonstrated, and we observe its propagation through multiple scattering events. In conditions where the cloud size is significantly larger than the transport mean free path, a diffusive regime is identified. We measure key parameters including the diffusion coefficient, transport velocity, and transport time, finding a good agreement with diffusion models. We also demonstrate that the frequency of the photons launched inside the system can be controlled. This approach enables direct time- and space-resolved observation of light diffusion in atomic ensembles, offering a promising avenue for exploring new diffusion regimes.
Abstract We present a depletion imaging technique to map out the spatial and temporal dependency of the density distribution of an ultracold gas of Rydberg atoms. Locally resolved absorption depletion, observed through differential ground state absorption imaging of a 87 Rb cloud in presence and absence of pre-excited Rydberg atoms, reveals their projected two-dimensional distribution. By employing a closed two-level optical transition uncoupled from the Rydberg state, the highly excited atoms are preserved during imaging. We measure the excitation dynamics of the ∣ 48 S 〉 state of 87 Rb, observing a saturation of the two-dimensional Rydberg density. Such outcome can be explained by the Rydberg blockade effect which prevents resonant excitation of close-by Rydberg atoms due to strong dipolar interactions. By combining the superatom description, where atoms within a blockade radius are represented as collective excitations, with a Monte Carlo sampling, we can quantitatively model the observed excitation dynamics and infer the full three-dimensional distribution of Rydberg atoms, that can serve as a starting point for quantum simulation of many-body dynamics involving Rydberg spin systems.
We measure the spatial pattern associated with the superradiant emission from a cloud of cold 87Rb atoms using Fourier imaging. We observe a highly directional, ring-shaped emission structure, which corresponds to a single collective jump operator associated to the most superradiant mode of the ensemble. Using spatial filtering, we isolate this channel and find the typical superradiant burst with superlinear scaling of the intensity with atom number. We compare our results to two models that describe the competition between the various decay channels, finding good agreement. Our work shows that the collective jump operators introduced by Carmichael et al. [Optics Communications 179, 417 (2000)] can be measured and manipulated.