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arXiv:2507.14371 · Photonics

Quasi-Degenerate Resonant Eigenstate Doublets of Two Quantum Emitters in a Closed Waveguide

Ammara Ammara, Paolo Facchi A, Saverio Pascazio, Francesco Vincenzo Pepe, Debmalya Das

Published Aug 27, 2025• 0 citations

Abstract

The physics of systems of quantum emitters in waveguide quantum electrodynamics is significantly influenced by the relation between their spatial separation and the wavelength of the emitted photons. If the distance that separates a pair of emitters meets specific resonance conditions, the photon amplitudes produced from decay may destructively interfere. In an infinite-waveguide setting, this effect gives rise to bound states in the continuum, where a photon remains confined between the emitters. In the case of a finite-length waveguide with periodic boundary conditions, there exist two such relevant distances for a given arrangement of the quantum emitters, leading to states in which a photon is confined to either the shorter or the longer path that connects the emitters. If the ratio of the shorter and the longer path is a rational number, these two kinds of resonant eigenstates are allowed to co-exist for the same Hamiltonian. In this paper, we investigate the existence of quasi-degenerate resonant doublets of a pair of identical emitters coupled to a linear waveguide mode. The states that form the doublet are searched among the ones in which a single excitation tends to remain bound to the emitters. We investigate the spectrum in a finite range around degeneracy points to check whether the doublet remains well separated from the closest eigenvalues in the spectrum. The identification of quasi-degenerate doublets opens the possibility to manipulate the emitters-waveguide system as an effectively two-level system in specific energy ranges, providing an innovative tool for quantum technology tasks.

DOI: 10.3390/photonics12090862

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The physics of systems of quantum emitters in waveguide quantum electrodynamics is significantly influenced by the relation between their spatial separation and the wavelength of the emitted photons. If the distance that separates a pair of emitters meets specific resonance conditions, the photon amplitudes produced from decay may destructively interfere. In an infinite-waveguide setting, this effect gives rise to bound states in the continuum, where a photon remains confined between the emitters. In the case of a finite-length waveguide with periodic boundary conditions, there exist two such relevant distances for a given arrangement of the quantum emitters, leading to states in which a photon is confined to either the shorter or the longer path that connects the emitters. If the ratio of the shorter and the longer path is a rational number, these two kinds of resonant eigenstates are allowed to co-exist for the same Hamiltonian. In this paper, we investigate the existence of quasi-degenerate resonant doublets of a pair of identical emitters coupled to a linear waveguide mode. The states that form the doublet are searched among the ones in which a single excitation tends to remain bound to the emitters. We investigate the spectrum in a finite range around degeneracy points to check whether the doublet remains well separated from the closest eigenvalues in the spectrum. The identification of quasi-degenerate doublets opens the possibility to manipulate the emitters-waveguide system as an effectively two-level system in specific energy ranges, providing an innovative tool for quantum technology tasks.

We investigate the behavior of two quantum emitters (two-level atoms) embedded in a linear waveguide, in a quasi-one-dimensional configuration. Since the atoms can emit, absorb, and reflect radiation, the pair can spontaneously relax towards an entangled bound state, under conditions in which a single atom would instead decay. Exploiting the resolvent formalism, we analyze the properties of these bound states, which occur for resonant values of the interatomic distance, and discuss their relevance with respect to entanglement generation. The stability of such states close to the resonance is studied, as well as the properties of nonresonant bound states, whose energy is below the threshold for photon propagation.

We study the bound states in the continuum for a system of

n

two-level quantum emitters, coupled with a one-dimensional photon field, when a single excitation is shared among the different components of the system. The emitters are equally spaced at fixed positions. We first consider the approximation of distant emitters and exhibit degenerate eigenspaces of bound states corresponding to resonant discrete values of the energy. We then consider the full form of the eigenvalue equation, in which the effects of the finite spacing and the field dispersion relation become relevant, yielding significant nonperturbative effects that can lift some degeneracies. We explicitly solve the cases

n=3

and

n=4

emitters.

We study a system made up of one or two two-level quantum emitters, coupled to a single transverse mode of a closed waveguide, in which photon wavenumbers and frequencies are discretized, and characterize the states in which one excitation is steadily shared between the field and the emitters. We unearth finite-size effects in the field-emitter interactions and identify a family of dressed bound states that represent the forerunners of bound states in the continuum in the limit of an infinite waveguide. We finally consider the potential interest of such states for applications in the field of quantum information.

Waveguide quantum electrodynamics (QED) has opened a new frontier in quantum optics, which enables the radiative coupling of distantly located emitters via the spatially extended waveguide mode. This coupling leads to modified emission dynamics and previous work has reported the observation of increased intensity correlations (an antidip) when probing the resonance response of multiple emitters. However, the interference between independent emitters has been shown to lead to a similar response. Here, we directly observe resonant energy transfer between two distant quantum emitters by recording an antidip in the intensity correlations, g ( 2 ) ( τ ) , while driving only one of the emitters. Under the condition that only a single emitter is driven, the antidip in photon coincidences is a distinctive signature of emitter-emitter coupling, which enables the transfer of energy from the driven to the undriven emitter. Interestingly, the observed mechanism is a long-range and waveguide-engineered version of resonant Förster transfer, which is responsible for the transport of energy between chlorophylls in the photosynthesis. Building on the established coupling, we demonstrate collective driving of the coupled emitter pair. Specifically, we control the relative driving phase and amplitude of the emitters and apply this collective excitation scheme to selectively populate the long-lived subradiant state. This results in suppressed emission, i.e., the peculiar situation where driving two emitters as opposed to one effectively reduces the probability of photon emission. Our work presents novel emission regimes and excitation schemes for a multiemitter waveguide QED system. These can be exploited to deterministically generate emitter-emitter entanglement and advanced photonic states providing robustness against losses for photonic quantum computation and quantum communication.

Two-photon bound states in the continuum provide a stringent setting in which quantum interference must suppress radiative decay despite photon--photon interactions. Here, we prove a no-go theorem showing that a single nonlinear mode linearly coupled to a noninteracting bosonic continuum cannot support an interaction-active two-photon bound state in the continuum, provided the local spectral density vanishes only at isolated energies. Apart from this regularity condition, the result is independent of the continuum dispersion and the frequency-dependent coupling. Although such an exact bound state is forbidden, long-lived two-photon quasi-bound states remain possible. For a giant Kerr cavity nonlocally coupled to a waveguide, we derive the asymptotic scaling of the two-photon decay rate with the coupling-point separation from weak nonlinearity to the hard-core limit. We further identify a regime in which the two-photon resonance is substantially longer lived than the single-photon excitation. Our work establishes the limits of exact multiphoton confinement while opening a route to engineering long-lived interacting few-photon states.

We study the emergence of two types of two-photon bounds states in waveguides of any chirality. Specifically, we present a systematic way of analytically determining the eigenstates of a system consisting of a waveguide coupled to a partially chiral, infinite array of equidistant two-level emitters. Using an effective Hamiltonian approach, we determine the properties of the two-photon bound states by determining their dispersion relation and internal structure. The bound states come in two varieties, depending on the two-photon momentum and emitter spacing. One of these states is a long-lived true bound state, whereas the other, a scattering resonance, decays in time via coupling to free two-photon states, leading to resonances and corresponding phase shifts in the photon-photon scattering.