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arXiv:2507.13658 · Physical Review A

Splitting of the three-body Förster resonance in Rb Rydberg atoms as a measure of the dipole-dipole interaction strength

I. I. Ryabtsev, I. N. Ashkarin, Ilya I. Beterov, Denis B. Tretyakov, Elena A. Yakshina, Vasily M. Entin, Patrick Cheinet

Published Nov 15, 2025• 3 citations
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Abstract

Three-body F\"orster resonances controlled by a dc electric field are of interest for the implementation of three-qubit quantum gates with single atoms in optical traps using their laser excitation into strongly interacting Rydberg states. In our recent theoretical paper [Zh. Eksp. Teor. Fiz. 168, 14 (2025)], it was found that the proposed earlier three-body F\"orster resonance $3\ifmmode\times\else\texttimes\fi{}n{P}_{3/2}\ensuremath{\rightarrow}n{S}_{1/2}+(n+1){S}_{1/2}+n{P}_{1/2}$ in Rb Rydberg atoms presents a splitting, with one of the split components having weaker dependence of the resonant electric field (and the corresponding dynamic shift) on the distance $R$ between the atoms. Here we study this effect in more detail, since this resonance appears as the most suitable for performing experiments on observing coherent oscillations of populations of collective three-body states and implementing three-qubit quantum gates based on them. For a linear spatial configuration of three interacting Rydberg atoms, the physical mechanism of this phenomenon is revealed and analytical formulas are obtained that describe the behavior of split structure of the F\"orster resonance depending on $R$. It is found that the splitting is a measure of the energy of the resonant dipole-dipole exchange interaction with an excitation hopping between neighboring Rydberg states $S$ and $P$.

DOI
10.1103/ws7n-926f

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Three-body F"orster resonances controlled by a dc electric field are of interest for the implementation of three-qubit quantum gates with single atoms in optical traps using their laser excitation into strongly interacting Rydberg states. In our recent theoretical paper [Zh. Eksp. Teor. Fiz. 168, 14 (2025)], it was found that the proposed earlier three-body F"orster resonance 3\ifmmode×\else\texttimes\finP3/2\ensuremath→nS1/2+(n+1)S1/2+nP1/23\ifmmode\times\else\texttimes\fi{}n{P}_{3/2}\ensuremath{\rightarrow}n{S}_{1/2}+(n+1){S}_{1/2}+n{P}_{1/2}3\ifmmode×\else\texttimes\finP3/2​\ensuremath→nS1/2​+(n+1)S1/2​+nP1/2​ in Rb Rydberg atoms presents a splitting, with one of the split components having weaker dependence of the resonant electric field (and the corresponding dynamic shift) on the distance RRR between the atoms. Here we study this effect in more detail, since this resonance appears as the most suitable for performing experiments on observing coherent oscillations of populations of collective three-body states and implementing three-qubit quantum gates based on them. For a linear spatial configuration of three interacting Rydberg atoms, the physical mechanism of this phenomenon is revealed and analytical formulas are obtained that describe the behavior of split structure of the F"orster resonance depending on RRR. It is found that the splitting is a measure of the energy of the resonant dipole-dipole exchange interaction with an excitation hopping between neighboring Rydberg states SSS and PPP.
Three-body Förster resonances controlled by a dc electric field are of interest for the implementation of three-qubit quantum gates with single atoms captured in optical traps and laser-excited into strongly interacting Rydberg states. In Ref. [P. Cheinet et al., Quantum Electronics 50(3), 213 (2020)], we proposed and analyzed a new type of three-body Förster resonance 3×nP3/2→nS1/2+(n+1)S1/2+nP1/2{\rm 3}\times nP_{3/2} \to nS_{1/2} +(n+1)S_{1/2} +nP_{1/2}3×nP3/2​→nS1/2​+(n+1)S1/2​+nP1/2​ that can be realized with Rb Rydberg atoms for an arbitrary principal quantum number nnn. Its peculiarity is that the third atom goes into a state with a total angular moment J=1/2J=1/2J=1/2, which has no Stark structure, so two-body Förster resonances are completely absent. In the present work, an extended theoretical study of this three-body Förster resonance is performed for various spatial configurations of three interacting Rb Rydberg atoms and conditions for their experimental implementation are determined. It was found that one of the resonances has a weak dependence of the resonant electric field on the distance between atoms and is therefore most suitable for performing experiments to observe coherent oscillations of populations of collective three-body states and implement three-qubit quantum gates based on them.
We have observed recently the Stark-tuned three-body F\"orster resonances $3\ifmmode\times\else\texttimes\fi{}n{P}_{3/2}(|M|)\ensuremath{\rightarrow}n{S}_{1/2}+(n+1){S}_{1/2}+n{P}_{3/2}(|{M}^{*}|)$ at long-range interactions of a few cold Rb Rydberg atoms [D. B. Tretyakov et al., Phys. Rev. Lett. 119, 173402 (2017)]. The three-body resonance appears at a different dc electric field with respect to the ordinary two-body resonance $2\ifmmode\times\else\texttimes\fi{}n{P}_{3/2}(|M|)\ensuremath{\rightarrow}n{S}_{1/2}+(n+1){S}_{1/2}$ and corresponds to a transition when the three interacting atoms change their states simultaneously (two atoms go to the SSS states, and the third atom remains in the PPP state but changes its moment projection), with the negligible contribution of the two-body resonance to the population transfer. It thus has a Borromean character and represents an effective three-body operator, which can be used to directly control the three-body interactions in quantum simulations and quantum gates implemented with Rydberg atoms. In this paper we theoretically investigate the coherence of such three-body resonances and we show that high-contrast Rabi-like population oscillations are possible for the localized Rydberg atoms in a certain spatial configuration. This paves the way to implementing three-qubit quantum gates and quantum simulations based on three-body Rydberg interactions.
Abstract The three-body Förster resonances 3 × nP3/2(|M|) →nS1/2 + (n + 1)S1/2 + nP3/2(|M*|), controlled by a constant electric field, were realised earlier by the authors in an ensemble of several cold Rydberg Rb atoms. One of the drawbacks of such resonances for potential application in three-qubit quantum gates is the proximity of the two-body Förster resonance 2 × nP3/2 → nS1/2 + (n + 1)S1/2, as well as the possibility of their implementation only for states with values of the principal quantum numbers n ⩽38. A three-body resonance of a new type, 3 × nP3/2 → nS1/2 + (n + 1)S1/2 + nP1/2, which can be realised for arbitrary n, is proposed and analysed. Its specific feature is also that the third atom transits into a state with a different total angular momentum J = 1/2, which has no Stark structure, so that the two-body resonance is completely absent. Numerical calculations showed that for not too strong interaction, it is possible to observe coherent three-body oscillations of the populations of collective states, which is of interest for developing new schemes of three-qubit quantum gates controlled by an electric field.
We propose a scheme of fast three-qubit Toffoli quantum gate for ultracold neutral-atom qubits. The scheme is based on Stark-tuned three-body F\"orster resonances, which we have observed in our recent experiment [D. B. Tretyakov et al., Phys. Rev. Lett. 119, 173402 (2017)]. The three-body resonance corresponds to a transition when the three interacting atoms change their states simultaneously, and it occurs at a different dc electric field with respect to the two-body F\"orster resonance. A combined effect of three-body and two-body F\"orster interactions in external electric and magnetic fields near the three-body resonance results in complex coherent behavior of the populations and phases of collective states of a three-atom system. We have found that it is possible to obtain experimental conditions suitable to implement three-qubit Toffoli gate with 98.3% fidelity and less than 3 $\ensuremath{\mu}\mathrm{s}$ duration.
Long-range interactions between cold Rydberg atoms, which are used in many important applications, can be enhanced using F\"orster resonances between collective many-body states controlled by an external electric field. Here we report on the first experimental observation of highly resolved radio-frequency-assisted F\"orster resonances in a few cold Rb Rydberg atoms. We also observed radio-frequency-induced F\"orster resonances which cannot be tuned by a dc electric field. They imply an efficient transition from van der Waals to resonant dipole-dipole interaction due to Floquet sidebands of Rydberg levels appearing in the rf field. This method can be applied to enhance the interactions of almost arbitrary Rydberg atoms with large principal quantum numbers.
We have developed an improved scheme of a three-qubit Toffoli gate based on a fine-structure-state-changing three-body Stark-tuned Rydberg interaction. This scheme is a substantial improvement of our previous proposal [I. I. Beterov et al., Phys. Rev. A 98, 042704 (2018)]. Due to the use of a different type of three-body F\"orster resonance we substantially simplified the scheme of laser excitation and phase dynamics of collective three-body states. This type of F\"orster resonance exists only in systems with more than two atoms, while the two-body resonance is absent. We reduced the sensitivity of the gate fidelity to fluctuations of external electric field and eliminated the necessity to use external magnetic field for fine-tuning of the resonant electric-field value, compared to the previous scheme of Toffoli gate based on Rydberg atoms. A gate fidelity of >99% was demonstrated in the calculations.