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arXiv:2507.08971 · Optics Letters

Temperature-tunable photon-pair source for multiplexed time-resolved fluorescence on a nanophotonic platform

Ayantika Sengupta, Nathan Harper, Emily Hwang, Scott K. Cushing

Published Jul 21, 2025• 2 citations
arXivHTMLPDF

Abstract

Compact, scalable, and multiplexed fluorescence lifetime sensors are of great interest for point-of-care diagnostics. However, current solutions either lack broad-range wavelength-tuning capabilities or involve complex optical setups that hinder miniaturization. On-chip entangled photon sources offer a promising alternative for time-resolved spectroscopy with their strong temporal correlations, tunable spectral characteristics, and small footprints. Here, we develop a temperature-tunable, visible quantum light source on thin-film lithium niobate (TFLN) with a continuous tuning range greater than one octave, spanning 564.5 nm to 1.494 $\mu$m using only one waveguide. The tunability is enabled by utilizing type-I phase matching. We measured an on-chip efficiency of $(3.88\pm 0.20)\times 10^{9}$ pairs/s/mW, comparable to the most efficient type-0 bulk lithium niobate sources. These results show that the TFLN platform is ideal for on-chip integrated photonic and multiplexed lifetime imaging and sensing.

DOI
10.1364/ol.568600

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Compact, scalable, and multiplexed fluorescence lifetime sensors are of great interest for point-of-care diagnostics. However, current solutions either lack broad-range wavelength-tuning capabilities or involve complex optical setups that hinder miniaturization. On-chip entangled photon sources offer a promising alternative for time-resolved spectroscopy with their strong temporal correlations, tunable spectral characteristics, and small footprints. Here, we develop a temperature-tunable, visible quantum light source on thin-film lithium niobate (TFLN) with a continuous tuning range greater than one octave, spanning 564.5 nm to 1.494 μ\muμm using only one waveguide. The tunability is enabled by utilizing type-I phase matching. We measured an on-chip efficiency of (3.88±0.20)×109(3.88\pm 0.20)\times 10^{9}(3.88±0.20)×109 pairs/s/mW, comparable to the most efficient type-0 bulk lithium niobate sources. These results show that the TFLN platform is ideal for on-chip integrated photonic and multiplexed lifetime imaging and sensing.
Efficient on-chip entangled photon pair generation at telecom wavelengths is an integral aspect of emerging quantum optical technologies, particularly for quantum communication and computing. However, moving to shorter wavelengths enables the use of more accessible silicon detector technology, and opens up applications in imaging and spectroscopy. Here, we present high brightness ((1.6 ± 0.3) × 10 9 pairs/s/mW/nm) visible–near-IR photon pair generation in a periodically poled lithium niobate nanophotonic waveguide. The degenerate spectrum of the photon pairs is centered at 811 nm with a bandwidth of 117 nm when pumped with a spectrally multimode laser diode. The measured on-chip source efficiency of (2.3 ± 0.5) × 10 11 pairs/s/mW is on par with source efficiencies at telecom wavelengths and is also orders of magnitude higher than the efficiencies of other visible sources implemented in bulk crystal or diffused waveguide-based technologies. Further improvements in the brightness and efficiencies are possible by pumping the device with a single-frequency laser, which would also shrink the pair bandwidth. These results represent the shortest wavelength of photon pairs generated in a nanophotonic waveguide reported to date by nearly an octave.
Quantum photonics has rapidly advanced as a key area for developing quantum technologies by harnessing photons’ inherent quantum characteristics, particularly entanglement. Generation of entangled photon pairs, known as Bell states, is crucial for quantum communications, precision sensing, and quantum computing. While bulk quantum optical setups have provided foundational progress, integrated quantum photonic platforms now offer superior scalability, efficiency, and integrative potential. In this study, we demonstrate a compact and bright source of polarization-entangled Bell state utilizing continuous-wave pumping on thin film lithium niobate (TFLN) integrated photonics. Our periodically poled lithium niobate device achieves on-chip brightness of photon pair generation rate of 518.2 MHz/mW, comparable to representative integrated photon-pair sources reported across various integrated photonic platforms. This demonstration marks the first realization, to our knowledge, of polarization entanglement on TFLN platforms. Experimentally measured metrics confirm high-quality entangled photon pairs with a purity of 0.901, a concurrence of 0.9, and a fidelity of 0.941. We expect our compact quantum devices to have great potential for advancing quantum communication systems and photonic quantum technologies.
Entangled photons are fundamental resources for quantum communication, computing, and networking. Among them, polarization-entangled photon pairs play an important role due to their straightforward state manipulation and direct use in quantum key distribution, teleportation, and network protocols. However, realizing compact, efficient, and scalable polarization-entangled sources that meet the requirements of practical deployment remains a major challenge. Here, we present a simple yet high-performance on-chip polarization-entangled photon-pair source on thin-film lithium niobate (TFLN). Our device employs dual quasi-phase matching (D-QPM) that sequentially supports type-0 and type-I spontaneous parametric down-conversion in a single nanophotonic waveguide, eliminating the need for interferometers, polarization rotators, or other complex circuits. The source directly produces high-fidelity Bell states with broad bandwidth, high brightness, and low noise. Using this integrated platform, we realize wavelength-multiplexed entanglement distribution in a four-user quantum network deployed over metropolitan fiber links up to 50 km. These results establish a robust and scalable pathway toward practical quantum communication systems and multi-user quantum mesh networks based on integrated photonics.
Entangled photon pairs generated by a low-power continuous-wave laser could replicate pulsed laser-based tabletop spectroscopy by taking advantage of the inherent quantum correlations between the photons. Much of the current work in the thin-film lithium niobate platform has focused on infrared wavelengths, leaving shorter wavelengths still a largely unexplored space, particularly for spectroscopy. In this work, we have fabricated periodically poled lithium niobate nanophotonic waveguides for entangled photon generation through spontaneous parametric downconversion with a visible pump (406 nm). Characterization of the waveguided pair source confirms the spectral and temporal correlations of energy-time entangled photons with an on-chip pair generation efficiency of (2.3 ± 0.5) × 1011 pairs/s/mW, brightness of (1.6 ± 0.3) × 109 pairs/s/mW/nm, and two-photon interference visibility greater than 99%. With the same material platform, we have also demonstrated second harmonic generation with on-chip powers up to 30 μW and wavelengths as low as 355 nm, demonstrating lithium niobate's potential for ultraviolet nonlinear photonics and frequency doubling in the UV-A spectral region. Through design of larger cross-section waveguides, we have also explored how variations in the lithium niobate thin film thickness can affect quasi-phase matching. To date, this is the first reported demonstration of periodically poled lithium niobate nanophotonic waveguides for spontaneous parametric downconversion at a fully visible pump wavelength (406 nm) as well as second harmonic generation in the UV (355 nm). Future work towards fully on-chip spectroscopy will explore integrating an on-chip Mach-Zehnder interferometer with the entangled photon source.
Quantum networks based on wavelength-multiplexed entanglement enable parallel distribution of quantum correlations, increasing channel capacity for secure communication and distributed quantum information processing. However, broadband integrated sources capable of generating multipartite entanglement beyond photon pairs remain scarce. Here we report on-chip generation of telecom-band four-photon entanglement in a periodically poled thin-film lithium niobate on insulator (LNOI) waveguide. Type-0 spontaneous parametric down-conversion provides a phase-matching bandwidth exceeding 200 nm, enabling spectrally separable generation of multi-photon entanglement across the telecom band. The generated photons are encoded in time bins for robust fiber compatibility, and a coherent interface enabling reversible conversion between time-bin and polarization degrees of freedom allows complete quantum state tomography. We measure two-photon entanglement with a brightness of 6.7 MHz/mW/nm and a fidelity of 0.874±0.0020.874 \pm 0.0020.874±0.002. At a pump power of 0.08 mW, the four-photon state exhibits a fourfold coincidence rate of 1 Hz and a fidelity of 0.74±0.010.74 \pm 0.010.74±0.01, representing a threefold improvement over previous integrated platforms. Our results establish LNOI as a scalable platform for broadband multi-photon entanglement and provide a practical route toward dense wavelength-multiplexed quantum networks.
Quantum photonics has rapidly advanced as a key area for developing quantum technologies by harnessing photons' inherent quantum characteristics, particularly entanglement. Generation of entangled photon pairs, known as Bell states, is crucial for quantum communications, precision sensing, and quantum computing. While bulk quantum optical setups have provided foundational progress, integrated quantum photonic platforms now offer superior scalability, efficiency, and integrative potential. In this study, we demonstrate a compact and bright source of polarization-entangled Bell state utilizing continuous-wave pumping on thin film lithium niobate (TFLN) integrated photonics. Our periodically poled lithium niobate device achieves on-chip brightness of photon pair generation rate of 508.5 MHz/mW, surpassing other integrated platforms including silicon photonics. This demonstration marks the first realization of polarization entanglement on TFLN platforms. Experimentally measured metrics confirm high-quality entangled photon pairs with a purity of 0.901, a concurrence of 0.9, and a fidelity of 0.944. We expect our compact quantum devices to have great potential for advancing quantum communication systems and photonic quantum technologies.