Neutral Rydberg atoms trapped in optical tweezer arrays provide a platform for quantum simulation and computation. In this work, we investigate the Lamb-Dicke dynamics of coupled Rydberg atoms for different trapping frequencies. We model the atomic motion by both internal and motional degrees of freedom, in which the motional states arise due to the oscillation of each atom in optical tweezer traps due to the light-atom interaction. In this setup, the internal states are coupled to a laser light with a Rabi frequency, while each internal state of each atom is also harmonically trapped with a trap frequency that depends on the internal state. The impact of the coherent motion of the optical tweezers on the collective dynamics of the many-body Rydberg atoms is explored for varying Lamb-Dicke parameters and with different trap frequencies. We see the occurrence of dynamical phases e.g., Rabi oscillations in the decoupled limit, the limit torus phase for magic trapping, and the limit cycle phase as the trap frequency is further increased.
Neutral Rydberg atoms trapped in optical tweezer arrays provide a platform for quantum simulation and computation. In this work, we investigate the Lamb-Dicke dynamics of coupled Rydberg atoms for different trapping frequencies. We model the atomic motion by both internal and motional degrees of freedom, in which the motional states arise due to the oscillation of each atom in optical tweezer traps due to the light-atom interaction. In this setup, the internal states are coupled to a laser light with a Rabi frequency, while each internal state of each atom is also harmonically trapped with a trap frequency that depends on the internal state. The impact of the coherent motion of the optical tweezers on the collective dynamics of the many-body Rydberg atoms is explored for varying Lamb-Dicke parameters and with different trap frequencies. We see the occurrence of dynamical phases e.g., Rabi oscillations in the decoupled limit, the limit torus phase for magic trapping, and the limit cycle phase as the trap frequency is further increased.
Neutral atoms trapped and manipulated by laser light provide experimentally well accessible quantum systems allowing for a high degree of control over external and internal degrees of freedom. Arrays of dipole traps in which the atoms are confined individually in a configurable geometry constitute a versatile platform for quantum simulation and information applications. By exciting these atoms into Rydberg states, interactions of variable strength and range can be introduced into the system, allowing for the implementation of entangling gate operations or spin Hamiltonians. A crucial requirement for these schemes to function in a reliable way is the ability to create defect-free arrays of single atoms. This is generally a challenge in these types of systems, as common atom loading schemes are limited to roughly 50% probability of filling each site. In this work, a technique for the rearrangement of atoms within a scalable architecture based on micro-optical lens arrays was developed and implemented, resulting in the creation of uniformly filled regions containing more than 100 atoms, which represent the largest defect-free structures realized so far in systems of this kind. This was accomplished by filling the empty traps in a pre-defined pattern with an atom one by one using an optical tweezer. Thus, structures with up to 5 x 5 atoms could be rendered defect-free in more than 99% of attempts. Although the success rate drops below unity for larger clusters, a value of 3.1% for a 100-atom structure is still viable for experiments working with post-selection methods. The filling fraction of even the largest examined structures was observed to be higher than 88%, surpassing common loading schemes by a significant margin. The measurements presented in this thesis build on a region of the array containing 361 sites, being limited by available laser power. In contrast, the addressable range of the optical tweezer includes more than 1500 sites and microlens arrays with up to a million lenses are commercially available. By implementing coherent Rydberg excitation of this assembled atom array, significant progress toward a universal quantum computer or flexible quantum simulator has been made. Using a two-photon excitation scheme, coherent dynamics between the ground and Rydberg state could be observed simultaneously in a 5 x 5 region of the array, with two-photon Rabi frequencies on the order of Omega = 2Pi x 500kHz measured for a Rydberg laser beam waist of w_0,B = 18.7(10) µm. The choice of an appropriate Rydberg state and interatomic spacing led to the presence of strong nearest-neighbor interactions and allowed for the demonstration of the Rydberg blockade effect by observing a collective enhancement of the Rabi frequency consistent with the expected scaling ~ sqrt(N) as well as the suppression of multiple excitations. This mechanism represents the fundamental constituent of a two-qubit gate operation. The architecture introduced in this work offers a scalability unique among quantum simulation platforms and the presented results underpin its potential to propel the atom-optical approach for quantum information processing beyond the threshold of quantum supremacy. Different approaches for scaling up the system have been explored, indicating that defect-free structures of more than 1000 atoms are within range with feasible experimental improvements. Through a detailed analysis of the factors limiting the coherence of the observed dynamics, strategies for future experimental improvements have been developed. Among these, increasing the coupling strength to the Rydberg state into the megahertz regime by increasing laser power and implementing single-site addressing represents the most straight-forward and promising approach.
Coupling electronic and vibrational degrees of freedom of Rydberg atoms held in optical tweezer arrays offers a flexible mechanism for creating and controlling atom-atom interactions. We find that the state-dependent coupling between Rydberg atoms and local oscillator modes gives rise to two- and three-body interactions which are controllable through the strength of the local confinement. This approach even permits the cancellation of two-body terms such that three-body interactions become dominant. We analyze the structure of these interactions on two-dimensional bipartite lattice geometries and explore the impact of three-body interactions on system ground state on a square lattice. Focusing specifically on a system of ^{87}Rb atoms, we show that the effects of the multibody interactions can be maximized via a tailored dressed potential within a trapping frequency range of the order of a few hundred kilohertz and for temperatures corresponding to a >90% occupation of the atomic vibrational ground state. These parameters, as well as the multibody induced timescales, are compatible with state-of-the-art arrays of optical tweezers. Our work shows a highly versatile handle for engineering multibody interactions of quantum many-body systems in most recent manifestations on Rydberg lattice quantum simulators.
Individually trapped neutral atoms are a promising candidate for use in quantum computing and simulation applications. They are highly scalable, have long coherence times and can be entangled via strong dipole-dipole interactions by driving to highly excited Rydberg states. However, the fidelity of single atom operations as well as two-atom entangling operations is limited by intrinsic sources of decoherence such as atomic motion, as well as technical sources of noise such as laser intensity fluctuations and phase/frequency fluctuations. We study the effect of these factors on single atom Rabi oscillations and two-atom Rydberg blockaded Rabi oscillations, using perturbation theory and numerical simulation. We develop a window function approach which helps us qualitatively understand the significance of the different spectral components of the noise as well as quantitatively understand the dependence of the Rabi oscillation fidelity on Rabi frequency. This allows us to predict the maximum experimentally achievable fidelities using independent measurements of experimental parameters such as noise spectra and atomic temperature. Turning to the question of near-term scalability of the experimental system, we prototype and test a method of generating a ’ladder’ configuration of optical tweezers utilizing two independent lasers. Our setup allows us to fully tune the geometry of the ladder, namely the separation between the two rows, the angle between them, and their relative position along the axis of the ladder. This pseudo-2D configuration enables us to reach larger system sizes in the near future and allows us to access beyond 1D physics.
Quantum simulation offers the possibility to study quantum mechanical problems which are untraceable on classical computers. This thesis introduces a novel platform for quantum simulation and presents the first experimental realisation of single potassium atoms trapped in optical tweezers. Interactions between individual atoms are induced by strong energy shifts of atoms excited to states with large principal quantum number, so-called Rydberg states. Either direct excitation to Rydberg states or off-resonant dressing can be used to induce these interactions. We argue that potassium is well-suited for the implementation of Rydberg dressing, enabling simultaneous dressing of both ground states to engineer complex interactions. Using techniques to cool and trap cold atoms, single potassium atoms are prepared in arrays of optical tweezers. Raman sideband cooling reduces vibrational excitations and prepares the atoms close to the motional ground state. This cooling technique mitigates severe limitations for Rydberg dressing, arising from thermal broadening and inhomogeneous light shifts in the array of atoms. To directly excite atoms to Rydberg states, a high power laser setup with two cavity-enhanced frequency doubling stages is constructed, generating up to one Watt of ulta-violet light at 286 nm. By exciting atoms to Rydberg states we observe Rabi oscillations with Rabi frequencies of up to 1 MHz, demonstrating coherent control of Rydberg atoms. Finally, we combine these techniques to observe interactions in two ways: First, we create a so-called superatom of up to four individual atoms using direct excitation and Rydberg-blockade and observe coherent oscillations to this collective state. We measure the expected square root scaling of the effective Rabi frequency with the number of individual atoms, confirming the creation of a many-body entangled state. Secondly, we off-resonantly dress the atoms prepared in a one-dimensional chain and measure correlated interaction shifts over multiple sites. In summary, we have developed a platform for quantum simulation with single atoms in optical tweezers. The presented results show coherent control of single atoms and interactions induced by Rydberg states. We have thus demonstrated that the system is well-suited for quantum simulation of many-body systems.
Rydberg atoms in optical lattices and tweezers is now a well-established platform for simulating quantum spin systems. However, the role of the atoms' spatial wave function has not been examined in detail experimentally. Here, we show a strong spin-motion coupling emerging from the large variation of the interaction potential over the wave function spread. We observe its clear signature on the ultrafast many-body nanosecond-dynamics of atoms excited to a Rydberg S state, using picosecond pulses, from an unity-filling atomic Mott-insulator. We also propose an approach to tune arbitrarily the strength of the spin-motion coupling relative to the motional energy scale set by trapping potentials. Our work provides a new direction for exploring the dynamics of strongly correlated quantum systems by adding the motional degree of freedom to the Rydberg simulation toolbox.
The rapid advancement of quantum science and technology has established Rydberg-atom arrays as a premier platform for exploring quantum many-body physics with exceptional precision and controllability. Traditionally, each atom is modeled as a spin degree of freedom with its spatial motion effectively frozen. This simplification has facilitated the discovery of a rich variety of novel equilibrium and nonequilibrium phases, including ZN symmetry-breaking orders and quantum scars. In this work, we investigate the consequences of incorporating atomic vibrations in optical tweezers, which give rise to spin-phonon coupling. For systems in thermal equilibrium, we find that this coupling leads to a new symmetry-breaking phase in the weak driving limit, as a result of induced three-spin interactions. Furthermore, we show that the violation of quantum thermalization in Z2-ordered states is suppressed when spin-phonon coupling is introduced. Our results are readily testable in state-of-the-art Rydberg-atom array experiments.