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arXiv:2506.19915 · Physical Review Letters

Error-Resilient Reversal of Quantum Chaotic Dynamics Enabled by Scramblons

Yu-Chen Li, Tian-Gang Zhou, Shengyu Zhang, Ze Wu, Liqiang Zhao, Haochuan Yin, Xiaoxue An, Hui Zhai, Pengfei Zhang, Xinhua Peng, Jiangfeng Du

Published Nov 20, 2025• 7 citations
arXivHTMLPDF

Abstract

The emergence of the arrow of time in quantum many-body systems stems from the inherent tendency of Hamiltonian evolution to scramble quantum information and increase entanglement. While, in principle, one might counteract this temporal directionality by engineering a perfectly inverted Hamiltonian to reverse entanglement growth, such a scenario is fundamentally unstable because even minor imperfections in the backward evolution can be exponentially amplified, a hallmark of quantum many-body chaos. Therefore, successfully reversing quantum many-body dynamics demands a deep understanding of the underlying structure of quantum information scrambling and chaotic dynamics. In this Letter, by using solid-state nuclear magnetic resonance on a macroscopic ensemble of randomly interacting spins, we measure the out-of-time-ordered correlator and validate key predictions of scramblon theory, a universal theoretical framework for information scrambling. Crucially, this theory enables us to isolate and mitigate errors in the out-of-time-ordered correlator caused by imperfections in the backward evolution. As a result, this protocol uncovers the anticipated exponential behavior of quantum many-body chaos and extracts the quantum Lyapunov exponent in a many-body experimental system for the first time. Our results push the fundamental limits of dynamical reversibility of complex quantum systems, with implications for quantum simulation and metrology.

DOI
10.1103/cg3f-rggs

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The emergence of the arrow of time in quantum many-body systems stems from the inherent tendency of Hamiltonian evolution to scramble quantum information and increase entanglement. While, in principle, one might counteract this temporal directionality by engineering a perfectly inverted Hamiltonian to reverse entanglement growth, such a scenario is fundamentally unstable because even minor imperfections in the backward evolution can be exponentially amplified, a hallmark of quantum many-body chaos. Therefore, successfully reversing quantum many-body dynamics demands a deep understanding of the underlying structure of quantum information scrambling and chaotic dynamics. In this Letter, by using solid-state nuclear magnetic resonance on a macroscopic ensemble of randomly interacting spins, we measure the out-of-time-ordered correlator and validate key predictions of scramblon theory, a universal theoretical framework for information scrambling. Crucially, this theory enables us to isolate and mitigate errors in the out-of-time-ordered correlator caused by imperfections in the backward evolution. As a result, this protocol uncovers the anticipated exponential behavior of quantum many-body chaos and extracts the quantum Lyapunov exponent in a many-body experimental system for the first time. Our results push the fundamental limits of dynamical reversibility of complex quantum systems, with implications for quantum simulation and metrology.
Quantum information scrambling, the dispersal of local information into many-body degrees of freedom, provides a powerful mechanism for generating large-scale correlations and entanglement essential for quantum-enhanced metrology. However, experimentally verifying such quantum-enhanced metrology remains a demanding task. Here, we correlate thousands of spins by engineering chaotic scrambling dynamics in a solid-state nuclear spin system. By leveraging the newly developed scramblon theory, we reveal exponential scaling in both the quantum Fisher information and the signal response to a phase shift. The signal response achieves a correlation-enabled enhancement of 33(2)33(2)33(2) dB over uncorrelated spins. After accounting for signal loss due to imperfect time reversal in the readout stage, we obtain a total metrological gain of 18(1) dB with a phase sensitivity of 40(3) μrad{\mathrm{μrad}}μrad. Our results bridge quantum chaos with practical quantum metrology, establishing reversible scrambling dynamics as a powerful resource for precision measurements.
Despite the rapid development of quantum science and technology, errors are inevitable and play a crucial role in quantum simulation and quantum computation. In quantum chaotic systems, coherent errors arising from imperfect Hamiltonian control and incoherent errors induced by coupling to the environment are both exponentially amplified during time evolution due to information scrambling. A fundamental question is how these two classes of errors imprint distinct signatures on the emergent irreversibility of many-body dynamics. In this Letter, we address this question by investigating multi-round time-reversed dynamics in the presence of both coherent and incoherent errors. By applying scramblon theory, we obtain closed-form expressions for the Loschmidt echo over different rounds of time-reversed evolution. For incoherent errors, the error accumulates linearly with the number of rounds, whereas coherent errors exhibit a crossover from quadratic to linear accumulation. These predictions are explicitly verified using the solvable Sachdev-Ye-Kitaev model. Our results provide a theoretical foundation for characterizing and calibrating coherent and incoherent errors in reversed dynamics, with particular relevance to nuclear magnetic resonance systems.
Most experimental protocols for measuring scrambling require time evolution with a Hamiltonian and with the Hamiltonian's negative counterpart (backward time evolution). Engineering controllable quantum many-body systems for which such forward and backward evolution is possible is a significant experimental challenge. Furthermore, if the system of interest is quantum chaotic, one might worry that any small errors in the time reversal will be rapidly amplified, obscuring the physics of scrambling. This paper undermines this expectation: We exhibit a renormalization protocol that extracts nearly ideal out-of-time-ordered-correlator measurements from imperfect experimental measurements. We analytically and numerically demonstrate the protocol's effectiveness, up to the scrambling time, in a variety of models and for sizable imperfections. The scheme extends to errors from decoherence by an environment.
The idea of the out-of-time-order correlator (OTOC) has recently emerged in the study of both condensed matter systems and gravitational systems.It not only plays a key role in investigating the holographic duality between a strongly interacting quantum system and a gravitational system, it also diagnoses the chaotic behavior of many-body quantum systems and characterizes information scrambling.Based on OTOCs, three different concepts-quantum chaos, holographic duality, and information scrambling-are found to be intimately related to each other.Despite its theoretical importance, the experimental measurement of the OTOC is quite challenging, and thus far there is no experimental measurement of the OTOC for local operators.Here, we report the measurement of OTOCs of local operators for an Ising spin chain on a nuclear magnetic resonance quantum simulator.We observe that the OTOC behaves differently in the integrable and nonintegrable cases.Based on the recent discovered relationship between OTOCs and the growth of entanglement entropy in the many-body system, we extract the entanglement entropy from the measured OTOCs, which clearly shows that the information entropy oscillates in time for integrable models and scrambles for nonintgrable models.With the measured OTOCs, we also obtain the experimental result of the butterfly velocity, which measures the speed of correlation propagation.Our experiment paves a way for experimentally studying quantum chaos, holographic duality, and information scrambling in many-body quantum systems with quantum simulators.
Out-of-time-order correlator (OTOC), been suggested as a measure of quantum information scrambling in quantum many-body systems, has received enormous attention recently. The experimental measurement of OTOC is quite challenging. The existing theoretical protocols consist in implementing time-reversal operations or using ancillary quantum systems, therefore only a few experiments have been reported. Recently, a new protocol to detect OTOC using statistical correlations between randomized measurements was put forward. In this work, we detect the OTOCs of a kicked-Ising model using this new measurement method on a 4-qubit nuclear magnetic resonance quantum simulator. In experiment, we use random Hamiltonian evolutions to generate the random operations that are required by the randomized OTOC detection protocol. Our experimental results are in good agreement with the theoretical predictions, thus confirming the feasibility of the protocols. Therefore, our work represents a step in exploring realistic quantum chaotic dynamics in complicated quantum systems.
The idea of the out-of-time-order correlator (OTOC) has recently emerged in the study of both condensed matter systems and gravitational systems.It not only plays a key role in investigating the holographic duality between a strongly interacting quantum system and a gravitational system, it also diagnoses the chaotic behavior of many-body quantum systems and characterizes information scrambling.Based on OTOCs, three different concepts-quantum chaos, holographic duality, and information scrambling-are found to be intimately related to each other.Despite its theoretical importance, the experimental measurement of the OTOC is quite challenging, and thus far there is no experimental measurement of the OTOC for local operators.Here, we report the measurement of OTOCs of local operators for an Ising spin chain on a nuclear magnetic resonance quantum simulator.We observe that the OTOC behaves differently in the integrable and nonintegrable cases.Based on the recent discovered relationship between OTOCs and the growth of entanglement entropy in the many-body system, we extract the entanglement entropy from the measured OTOCs, which clearly shows that the information entropy oscillates in time for integrable models and scrambles for nonintgrable models.With the measured OTOCs, we also obtain the experimental result of the butterfly velocity, which measures the speed of correlation propagation.Our experiment paves a way for experimentally studying quantum chaos, holographic duality, and information scrambling in many-body quantum systems with quantum simulators.