Ultrabright, two-color photon pair source based on thin-film lithium niobate for bridging visible and telecom wavelengths
Silia Babel, Laura Bollmers, Franz Roeder, Werner Ridder, Christian Golla, Ronja Köthemann, Bernhard Reineke, Harald Herrmann, Benjamin Brecht, Christof Eigner, Laura Padberg, Christine Silberhorn
We present the design and characterization of a guided-wave, bright, and highly frequency non-degenerate parametric down-conversion (PDC) source in thin-film lithium niobate. The source generates photon pairs with wavelengths of 815 nm and 1550 nm, linking the visible wavelength regime with telecommunication wavelengths. We confirm the high quality of the generated single photons by determining a value for the heralded second-order correlation function as low as g h (2) (0)=(6.7±1.1)⋅10 −3 . Furthermore, we achieve a high spectral brightness of 0.44·10 7 pairss⋅mW⋅GHz which is two orders of magnitude higher than sources based on weakly guiding waveguides. The shape of the PDC spectrum and the strong agreement between the effective and nominal bandwidth highlight our high fabrication quality of periodically poled waveguides. The good agreement between the measured and simulated spectral characteristics of our source demonstrates our excellent understanding of the PDC process. Our result is a valuable step towards practical and scalable quantum communication networks as well as photonic quantum computing.
We present the design and characterization of a guided-wave, bright, and highly frequency non-degenerate parametric down-conversion (PDC) source in thin-film lithium niobate. The source generates photon pairs with wavelengths of 815 nm and 1550 nm, linking the visible wavelength regime with telecommunication wavelengths. We confirm the high quality of the generated single photons by determining a value for the heralded second-order correlation function as low as g h (2) (0)=(6.7±1.1)⋅10 −3 . Furthermore, we achieve a high spectral brightness of 0.44·10 7 pairss⋅mW⋅GHz which is two orders of magnitude higher than sources based on weakly guiding waveguides. The shape of the PDC spectrum and the strong agreement between the effective and nominal bandwidth highlight our high fabrication quality of periodically poled waveguides. The good agreement between the measured and simulated spectral characteristics of our source demonstrates our excellent understanding of the PDC process. Our result is a valuable step towards practical and scalable quantum communication networks as well as photonic quantum computing.
Efficient on-chip entangled photon pair generation at telecom wavelengths is an integral aspect of emerging quantum optical technologies, particularly for quantum communication and computing. However, moving to shorter wavelengths enables the use of more accessible silicon detector technology, and opens up applications in imaging and spectroscopy. Here, we present high brightness ((1.6 ± 0.3) × 10 9 pairs/s/mW/nm) visible–near-IR photon pair generation in a periodically poled lithium niobate nanophotonic waveguide. The degenerate spectrum of the photon pairs is centered at 811 nm with a bandwidth of 117 nm when pumped with a spectrally multimode laser diode. The measured on-chip source efficiency of (2.3 ± 0.5) × 10 11 pairs/s/mW is on par with source efficiencies at telecom wavelengths and is also orders of magnitude higher than the efficiencies of other visible sources implemented in bulk crystal or diffused waveguide-based technologies. Further improvements in the brightness and efficiencies are possible by pumping the device with a single-frequency laser, which would also shrink the pair bandwidth. These results represent the shortest wavelength of photon pairs generated in a nanophotonic waveguide reported to date by nearly an octave.
Chip-integrated photon-pair sources based on spontaneous parametric down-conversion (SPDC) have emerged as a promising solution for scalable quantum light generation. Thin-film lithium tantalate (TFLT) is a compelling χ(2) platform, combining strong nonlinearity with a high optical-damage threshold, weak photorefractive response, and ferroelectricity that enables quasi-phase matching. However, SPDC-based photon-pair generation on TFLT has not yet been demonstrated. Here, we combine high-quality periodic poling with low-loss nanophotonic waveguides to realize photon-pair sources on TFLT in both traveling-wave and resonant configurations. In periodically poled straight waveguides, we achieve broadband photon-pair generation with high efficiency (2.1GHzmW−1) and coincidence-to-accidental ratio (up to 3.8×105). We further confirm high-purity single-photon operation via heralded second-order correlation (gH(2)(0)=0.0018±0.0002) and high-fidelity time-energy entanglement through Franson interference (visibility of 98.9±0.5%). In periodically poled racetrack resonators, we map out a broad quantum frequency comb spanning the telecom C- and L-bands. By isolating individual frequency-correlated pairs, we measure a high spectral brightness of 11GHzmW−1GHz−1. These results are competitive with the state of the art across χ(2) integrated platforms, positioning TFLT as a strong contender for integrated quantum light sources, with applications in wavelength-multiplexed quantum communications and photonic quantum information processing.
Abstract Chip-integrated photon-pair sources based on spontaneous parametric down-conversion (SPDC) have emerged as a promising solution for scalable quantum light generation. Thin-film lithium tantalate (TFLT) is a compelling χ(2) platform, combining strong nonlinearity with a high optical-damage threshold, weak photorefractive response, and ferroelectricity that enables quasi-phase matching. However, SPDC-based photon-pair generation on TFLT has not yet been demonstrated. Here, we combine high-quality periodic poling with low-loss nanophotonic waveguides to realize photon-pair sources on TFLT in both traveling-wave and resonant configurations. In periodically poled straight waveguides, we achieve broadband photon-pair generation with high efficiency (2.1~GHz~mW−1) and coincidence-to-accidental ratio (up to 3.8×105). We further confirm high-purity single-photon operation via heralded second-order correlation (gH(2)(0)=0.0018±0.0002) and high-fidelity time-energy entanglement through Franson interference (visibility of 98.9±0.5%). In periodically poled racetrack resonators, we map out a broad quantum frequency comb spanning the telecom C- and L-bands. By isolating individual frequency-correlated pairs, we measure a high spectral brightness of 11~GHz~mW−1~GHz−1. These results are competitive with the state of the art across χ(2) integrated platforms, positioning TFLT as a strong contender for integrated quantum light sources, with applications in wavelength-multiplexed quantum communications and photonic quantum information processing.
The practical prospect of quantum communication and information processing relies on sophisticated single-photon pairs, which feature a controllable waveform, narrow spectrum, excellent purity, fiber compatibility, and miniaturized design. For practical realizations, stable, miniaturized, low-cost devices are required. Sources with one or some of the above characteristics have already been demonstrated, but it is quite challenging to obtain a source with all of the described characteristics simultaneously. Here we report on an integrated single-longitudinal-mode, non-degenerate, narrowband photon pair source that exhibits all the requirements needed for quantum applications. The device is composed of a periodically poled, Ti-indiffused, lithium niobate waveguide with high reflective dielectric mirror coatings deposited on the waveguide end-faces. Photon pairs with wavelengths around 890 and 1320 nm are generated via type II phase-matched parametric down-conversion (PDC). Clustering in this dispersive cavity restricts the whole conversion spectrum to one single-longitudinal mode in a single cluster, yielding a narrow bandwidth of only 60 MHz. The high conversion efficiency in the waveguide, together with the spectral clustering in the doubly resonant waveguide, leads to a high brightness of pairs/(s mW MHz). This source exhibits prominent single-longitudinal-mode purity and remarkable temporal shaping capability. In particular, due to temporal broadening, we can observe that the coherence time of the two-photon component of the PDC state is actually longer than that of the single-photon states. The miniaturized monolithic design enables this source to have various fiber communication applications.
Abstract Spontaneous parametric down-conversion (SPDC), especially in non-linear waveguides, serves as an important process to generate quantum states of light with desired properties. In this work, we report on a design of a strongly dispersive, singly poled thin film lithium niobate (TFLN) waveguide geometry which acts as a convertible source of photon pairs across telecom band with tunable spectral properties. Through our simulations, we demonstrate that by using this optimized waveguide geometry, two completely different yet desirable type II phase-matched SPDC processes are enabled using a single poling period. One process generates spectrally correlated non-degenerate photon pairs with one photon at 1310nm (telecom O band) and the other at 1550nm (telecom C band). The second SPDC process results in spectrally uncorrelated photon pairs in telecom C band at 1533nm and 1567nm respectively.We attribute this versatility of TFLN waveguide to its strong dispersion properties and make a comparative study with the existing weakly dispersive waveguide platforms.We believe that such a versatile source of photon pairs will serve as an important ingredient in various quantum optical tasks which require photons at different telecom bands and desired spectral properties.
A thin-film periodically poled lithium niobate waveguide was designed and fabricated which generates entangled photon pairs at telecommunications wavelengths with high coincidences-to-accidentals counts ratio CAR>67000, two-photon interference visibility V>99%, and heralded single-photon autocorrelation g_{H}^{(2)}(0)<0.025. Nondestructive in situ diagnostics were used to determine the poling quality in 3D. Megahertz rates of photon pairs were generated by less than a milliwatt of pump power, simplifying the pump requirements and dissipation compared to traditional spontaneous parametric down-conversion lithium niobate devices.