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arXiv:2506.16134 · Physical Review Research

Optical centrifuge for nanoparticles

Peiyao Xiong, Ka Kit Kelvin Ho, Jonathan M. H. Gosling, Markus Rademacher, P. F. Barker

Published Nov 21, 2025• 1 citation
arXivHTMLPDF

Abstract

We study theoretically the creation of an optical centrifuge for the controlled rotation of levitated nanorotors within an optical tweezer. The optical centrifuge's motion is simulated by rapidly rotating the linear polarization of the tightly focused optical field used to form an optical trap. We show that nanorotors, formed by anisotropic nanoparticles levitated within a trap, can be accelerated to well-defined rotational rates in excess of 100 MHz over durations of hundreds of microseconds. The initial conditions required for stable acceleration, based on optical trap properties and the anisotropic susceptibility of the nanorotor are established and confirmed by numerical simulations. We also present initial experiments that have developed tools for the rapid angular acceleration of the polarization vector of the linearly polarized beam that is required to create the centrifuge. We show that over acceleration durations in the 100 μ s range, high rotational speeds could be achieved in modest vacuum.

DOI
10.1103/ylw9-22jj

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We study theoretically the creation of an optical centrifuge for the controlled rotation of levitated nanorotors within an optical tweezer. The optical centrifuge's motion is simulated by rapidly rotating the linear polarization of the tightly focused optical field used to form an optical trap. We show that nanorotors, formed by anisotropic nanoparticles levitated within a trap, can be accelerated to well-defined rotational rates in excess of 100 MHz over durations of hundreds of microseconds. The initial conditions required for stable acceleration, based on optical trap properties and the anisotropic susceptibility of the nanorotor are established and confirmed by numerical simulations. We also present initial experiments that have developed tools for the rapid angular acceleration of the polarization vector of the linearly polarized beam that is required to create the centrifuge. We show that over acceleration durations in the 100 μ s range, high rotational speeds could be achieved in modest vacuum.
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We perform free-fall experiments with a charge-neutral, optically levitated nanoparticle. This is achieved using an optical tweezer that can be rapidly toggled on and off and vertically displaced, enabling the particle to be released and recaptured after each free fall. The particle is insensitive to electric fields due to its charge neutrality and, during free evolution, is not subject to photon recoil heating. We achieve free-fall durations of up to 0.25 ms and observe a nearly two hundred-fold increase in the particle's position uncertainty at recapture. The current limit on the free-fall time arises from the performance of the initial cooling step. By implementing linear feedback techniques and reducing the background pressure, we expect to perform millisecond-scale free-fall experiments in ultra-high vacuum, opening new opportunities for generating large delocalizations of levitated objects.
We perform free-fall experiments with a charge-neutral, optically levitated nanoparticle. This is achieved using an optical tweezer that can be rapidly toggled on and off and vertically displaced, enabling the particle to be released and recaptured after each free fall. The particle is insensitive to electric fields due to its charge neutrality, and during free evolution, is not subject to photon recoil heating. We achieve free-fall durations of up to 0.25ms and observe a nearly 200-fold increase in the particle's position uncertainty at recapture. The current limit on the free-fall time arises from the performance of the initial cooling step. By implementing linear feedback techniques and reducing the background pressure, we expect to perform millisecond-scale free-fall experiments in an ultrahigh vacuum, opening new opportunities for generating large delocalizations of levitated objects.
Control of the potential energy and free evolution lie at the heart of levitodynamics as key requirements for sensing, wave function expansion, and mechanical squeezing protocols. Here, we experimentally demonstrate full control over the optical potential governing the librational degrees of freedom of a levitated anisotropic nanoparticle. This control is achieved by introducing the degree of polarization as a new tool for rotational levitodynamics. We demonstrate the free rotation of a levitated anisotropic scatterer around its short axis and and we use the rotational degrees of freedom to probe the local spin of a strongly focused laser beam.
We demonstrate optical levitation and feedback cooling of a silica nanoparticle (radius = 78~nm) trapped within a radial vector beam (RVB) in high vacuum. Radial vector beams, when focused by a high-NA lens, produce a smaller focal spot than conventional Gaussian beams, yielding tighter optical potentials and potentially reduced photon-recoil heating rates. A vortex wave plate was used to generate the RVB using an aspheric lens (NA = 0.77) to form the trap. Cold-damping feedback was used to cool the center of mass motion in the radial and axial trap directions to temperatures in the mK range. At higher temperatures and pressures, additional trap frequencies arising from the nonlinear RVB optical potential are observed. This demonstration is a step toward exploiting structured light for levitated quantum optomechanics where these traps can be used to suppress bulk and motional heating.