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arXiv:2506.13707 · Physical Review Letters

Dimer-Projection Contact and the Clock Shift of a Unitary Fermi Gas

Kevin G. S. Xie, Colin J. Dale, Kiera Pond Grehan, M. Wang, Tilman Enss, Paul S. Julienne, Zhenhua Yu, Joseph H. Thywissen

Published Jan 28, 2026• 2 citations
arXivHTMLPDF

Abstract

Understanding the dynamics of short-range correlations is a central challenge in strongly interacting Fermi gases. In ultracold gases, these correlations are quantified by the contact parameter, yet measurements to date have been limited to equilibrium systems or relatively slow, global dynamics. Here, we introduce a rapid spectroscopic technique based on projection of the interacting state onto an alternate scattering channel with a low-lying dimer state. We demonstrate contact measurements on the microsecond timescale-faster than the inverse Fermi energy. Using ^{40}K near a broad s-wave Feshbach resonance, we show that the strength of the dimer-projection feature scales proportionally with the contact parameter extracted from the high-frequency tail of radio-frequency spectroscopy, in agreement with coupled-channels calculations. Analysis of the spectra further reveals that the dimer feature provides the dominant contribution to the clock shift of the unitary Fermi gas, allowing the first experimental bound on this quantity. The observed deviations from universal predictions highlight the importance of multichannel effects. Our results open new avenues for studying contact correlators, hydrodynamic attractors, and quantum critical behavior.

DOI
10.1103/44rc-34n1

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Understanding the dynamics of short-range correlations is a central challenge in strongly interacting Fermi gases. In ultracold gases, these correlations are quantified by the contact parameter, yet measurements to date have been limited to equilibrium systems or relatively slow, global dynamics. Here, we introduce a rapid spectroscopic technique based on projection of the interacting state onto an alternate scattering channel with a low-lying dimer state. We demonstrate contact measurements on the microsecond timescale-faster than the inverse Fermi energy. Using ^{40}K near a broad s-wave Feshbach resonance, we show that the strength of the dimer-projection feature scales proportionally with the contact parameter extracted from the high-frequency tail of radio-frequency spectroscopy, in agreement with coupled-channels calculations. Analysis of the spectra further reveals that the dimer feature provides the dominant contribution to the clock shift of the unitary Fermi gas, allowing the first experimental bound on this quantity. The observed deviations from universal predictions highlight the importance of multichannel effects. Our results open new avenues for studying contact correlators, hydrodynamic attractors, and quantum critical behavior.
We measure radio frequency (rf) spectra of the homogeneous unitary Fermi gas at temperatures ranging from the Boltzmann regime through quantum degeneracy and across the superfluid transition. For all temperatures, a single spectral peak is observed. Its position smoothly evolves from the bare atomic resonance in the Boltzmann regime to a frequency corresponding to nearly one Fermi energy at the lowest temperatures. At high temperatures, the peak width reflects the scattering rate of the atoms, while at low temperatures, the width is set by the size of fermion pairs. Above the superfluid transition, and approaching the quantum critical regime, the width increases linearly with temperature, indicating non-Fermi-liquid behavior. From the wings of the rf spectra, we obtain the contact, quantifying the strength of short-range pair correlations. We find that the contact rapidly increases as the gas is cooled below the superfluid transition.
The contact I, introduced by Tan, has emerged as a key parameter characterizing universal properties of strongly interacting Fermi gases. For ultracold Fermi gases near a Feshbach resonance, the contact depends upon two quantities: the interaction parameter 1/(k(F)a), where k(F) is the Fermi wave vector and a is the s-wave scattering length, and the temperature T/T(F), where T(F) is the Fermi temperature. We present the first measurements of the temperature dependence of the contact in a unitary Fermi gas using Bragg spectroscopy. The contact is seen to follow the predicted decay with temperature and shows how pair-correlations at high momentum persist well above the superfluid transition temperature.
We derive universal relations for the rf spectroscopy of a two-dimensional Fermi gas consisting of two spin states interacting through an SSS-wave scattering length. The rf transition rate has a high-frequency tail that is proportional to the contact and displays logarithmic scaling violations, decreasing asymptotically like $1/({\ensuremath{\omega}}^{2}{ln}^{2}\ensuremath{\omega})$. Its coefficient is proportional to ${ln}^{2}({a}_{2\mathrm{D}}^{\ensuremath{'}}/{a}_{2\mathrm{D}})$, where a2D{a}_{2\mathrm{D}}a2D​ and ${a}_{2\mathrm{D}}^{\ensuremath{'}}$ are the two-dimensional scattering lengths associated with initial-state and final-state interactions. The clock shift is proportional to the contact and to $\mathrm{ln}({a}_{2\mathrm{D}}^{\ensuremath{'}}/{a}_{2\mathrm{D}})$. If $|\mathrm{ln}({a}_{2\mathrm{D}}^{\ensuremath{'}}/{a}_{2\mathrm{D}})|\ensuremath{\gg}1$, the clock shift arises as a cancellation between much larger contributions proportional to ${ln}^{2}({a}_{2\mathrm{D}}^{\ensuremath{'}}/{a}_{2\mathrm{D}})$ from bound-bound and bound-free rf transitions.
The Unitary Fermi Gas (UFG) is one of the most strongly interacting systems known to date, as it saturates the unitarity bound on the quantum mechanical scattering cross section. The UFG corresponds to a two-component Fermi gas in the limit of short interaction range and large scattering length, and is currently realized in ultracold-atom experiments via Feshbach resonances. While easy to define, the UFG poses a challenging quantum many-body problem, as it lacks any characteristic scale other than the density. As a consequence, accurate quantitative predictions of the thermodynamic properties of the UFG require Monte Carlo calculations. However, significant progress has also been made with purely analytical methods. Notably, in 2005 Tan derived a set of exact thermodynamic relations in which a universal quantity known as the "contact" C plays a crucial role. Recently, C has also been found to determine the prefactor of the high- frequency power-law decay of correlators as well as the right-hand-sides of shear- and bulk viscosity sum rules. The contact is therefore a central piece of information on the UFG in equilibrium as well as away from equilibrium. In this talk we describe some of the known aspects of Fermi gases at and around unitarity, show our latest Monte Carlo results for the contact at finite temperature, and summarize the open questions in the field, some of which we are starting to answer using large-scale Monte Carlo calculations by adapting methods from Lattice QCD.
The Unitary Fermi Gas (UFG) is one of the most strongly interacting systems known to date, as it saturates the unitarity bound on the quantum mechanical scattering cross section.The UFG corresponds to a two-component Fermi gas in the limit of short interaction range and large scattering length, and is currently realized in ultracold-atom experiments via Feshbach resonances.While easy to define, the UFG poses a challenging quantum many-body problem, as it lacks any characteristic scale other than the density.As a consequence, accurate quantitative predictions of the thermodynamic properties of the UFG require Monte Carlo calculations.However, significant progress has also been made with purely analytical methods.Notably, in 2005 Tan derived a set of exact thermodynamic relations in which a universal quantity known as the "contact" C plays a crucial role.Recently, C has also been found to determine the prefactor of the high-frequency power-law decay of correlators as well as the right-hand-sides of shear-and bulk viscosity sum rules.The contact is therefore a central piece of information on the UFG in equilibrium as well as away from equilibrium.In this talk we describe some of the known aspects of Fermi gases at and around unitarity, show our latest Monte Carlo results for the contact at finite temperature, and summarize the open questions in the field, some of which we are starting to answer using large-scale Monte Carlo calculations by adapting methods from Lattice QCD.
The Unitary Fermi Gas (UFG) is one of the most strongly interacting systems known to date, as it saturates the unitarity bound on the quantum mechanical scattering cross section. The UFG corresponds to a two-component Fermi gas in the limit of short interaction range and large scattering length, and is currently realized in ultracold-atom experiments via Feshbach resonances. While easy to define, the UFG poses a challenging quantum many-body problem, as it lacks any characteristic scale other than the density. As a consequence, accurate quantitative predictions of the thermodynamic properties of the UFG require Monte Carlo calculations. However, significant progress has also been made with purely analytical methods. Notably, in 2005 Tan derived a set of exact thermodynamic relations in which a universal quantity known as the "contact" C plays a crucial role. Recently, C has also been found to determine the prefactor of the high- frequency power-law decay of correlators as well as the right-hand-sides of shear- and bulk viscosity sum rules. The contact is therefore a central piece of information on the UFG in equilibrium as well as away from equilibrium. In this talk we describe some of the known aspects of Fermi gases at and around unitarity, show our latest Monte Carlo results for the contact at finite temperature, and summarize the open questions in the field, some of which we are starting to answer using large-scale Monte Carlo calculations by adapting methods from Lattice QCD.