We demonstrate that an effective near-zero refractive index can emerge from collective light scattering in a discrete atomic lattice, using essentially exact microscopic simulations. In a 25-layer array, cooperative response leads to over a thirtyfold increase in the effective optical wavelength within the medium, almost eliminating optical phase accumulation, with potential applications in spectroscopy and optical manipulation of quantum emitters. Crucially, the near-zero refractive index arises from first-principles microscopic theory, rather than being imposed through continuous phenomenological effective-medium models-providing conceptually important insight into the emergence of macroscopic electromagnetism from atomic-scale interactions.
We demonstrate that an effective near-zero refractive index can emerge from collective light scattering in a discrete atomic lattice, using essentially exact microscopic simulations. In a 25-layer array, cooperative response leads to over a thirtyfold increase in the effective optical wavelength within the medium, almost eliminating optical phase accumulation, with potential applications in spectroscopy and optical manipulation of quantum emitters. Crucially, the near-zero refractive index arises from first-principles microscopic theory, rather than being imposed through continuous phenomenological effective-medium models-providing conceptually important insight into the emergence of macroscopic electromagnetism from atomic-scale interactions.
It is interesting to observe that all optical materials with a positive refractive index have a value of index that is of order unity.Surprisingly, though, a deep understanding of the mechanisms that lead to this universal behavior seems to be lacking.Moreover, this observation is difficult to reconcile with the fact that a single isolated atom is known to have a giant optical response, as characterized by a resonant scattering cross section that far exceeds its physical size.Here, we theoretically and numerically investigate the evolution of the optical properties of an ensemble of ideal atoms as a function of density, starting from the dilute gas limit, including the effects of multiple scattering and near-field interactions.Interestingly, despite the giant response of an isolated atom, we find that the maximum index does not indefinitely grow with increasing density but rather reaches a limiting value of n ≈ 1.7.This limit arises purely from electrodynamics, as it occurs at densities far below those where chemical processes become important.We propose an explanation based upon strong-disorder renormalization group theory, in which the nearfield interaction combined with random atomic positions results in an inhomogeneous broadening of atomic resonance frequencies.This mechanism ensures that, regardless of the physical atomic density, light at any given frequency only interacts with at most a few near-resonant atoms per cubic wavelength, thus limiting the maximum index attainable.Our work is a promising first step to understand the limits of the refractive index from a bottom-up, atomic physics perspective, and it also introduces the renormalization group as a powerful tool to understand the generally complex problem of multiple scattering of light overall.
It is interesting to observe that all optical materials with a positive refractive index have a value of index that is of order unity. Surprisingly, though, a deep understanding of the mechanisms that lead to this universal behavior seems to be lacking. Moreover, this observation is difficult to reconcile with the fact that a single isolated atom is known to have a giant optical response, as characterized by a resonant scattering cross section that far exceeds its physical size. Here, we theoretically and numerically investigate the evolution of the optical properties of an ensemble of ideal atoms as a function of density, starting from the dilute gas limit, including the effects of multiple scattering and near-field interactions. Interestingly, despite the giant response of an isolated atom, we find that the maximum index does not indefinitely grow with increasing density but rather reaches a limiting value of n ≈ 1.7. This limit arises purely from electrodynamics, as it occurs at densities far below those where chemical processes become important. We propose an explanation based upon strong-disorder renormalization group theory, in which the near-field interaction combined with random atomic positions results in an inhomogeneous broadening of atomic resonance frequencies. This mechanism ensures that, regardless of the physical atomic density, light at any given frequency only interacts with at most a few near-resonant atoms per cubic wavelength, thus limiting the maximum index attainable. Our work is a promising first step to understand the limits of the refractive index from a bottom-up, atomic physics perspective, and it also introduces the renormalization group as a powerful tool to understand the generally complex problem of multiple scattering of light overall.
We present a model describing the transmission of light through atomic media with a vanishing index of refraction. Zero-index materials are of particular interest as the infinite phase velocity of light within the material offers the potential to manipulate electromagnetic waves to mediate dipole-dipole interactions over extended distances. We focus on the preparation of near-zero-index (NZI) conditions based on atomic coherence using two distinct atomic media as exemplary of generic NZI materials. We establish a model based on the Maxwell-Bloch equations to describe the propagation of a light pulse through these media. To investigate the sustainability of NZI under minimal light conditions, we assume single-photon intensity of the propagating pulse. Specifically, we examine whether the spatial phase change of the photon remains near zero as it traverses the medium. We employ a finite-element numerical approach to solve the coupled Maxwell-Bloch equations describing the photon propagation. Our results indicate that the presence of a photon within the medium will disrupt the NZI state, thus disallowing the establishment of enhanced dipole-dipole interactions over large distances.
We present a model describing the transmission of light through atomic media with a vanishing index of refraction. Zero index materials are of particular interest as the infinite phase velocity of light within the material offers the potential to manipulate electromagnetic waves to mediate dipole-dipole interactions over extended distances. We focus on the preparation of zero-index conditions based on atomic coherence using two distinct atomic media as exemplary of generic zero-index materials. We establish a model based on the Maxwell-Bloch equations to describe the propagation of a light pulse through these media. To investigate the sustainability of the zero index under minimal light conditions, we assume single-photon intensity of the propagating pulse. Specifically, we examine whether the spatial phase change of the photon remains zero as it traverses the medium. We employ a finite-element numerical approach to solve the coupled Maxwell-Bloch equations describing the photon propagation. Our results indicate that the presence of a photon within the medium will disrupt the zero-index state, thus disallowing the establishment of enhanced dipole-dipole interactions over large distances.
The quest to manipulate light propagation in ways not possible with natural media has driven the development of artificially structured metamaterials. One of the most striking effects is negative refraction, where the light beam deflects away from the boundary normal. However, due to material characteristics, the applications of this phenomenon, such as lensing that surpasses the diffraction limit, have been constrained. Here, we demonstrate negative refraction of light in an atomic medium without the use of artificial metamaterials, employing essentially exact simulations of light propagation. High transmission negative refraction is achieved in atomic arrays for different level structures and lattice constants, within the scope of currently realised experimental systems. We introduce an intuitive description of negative refraction based on collective excitation bands, whose transverse group velocities are antiparallel to the excitation quasi-momenta. We also illustrate how this phenomenon is robust to lattice imperfections and can be significantly enhanced through subradiance.
Collective coupling between dipoles can dramatically modify the optical response of a medium. Such effects depend strongly on the geometry of the medium and the polarization of the light. Using a classical coupled dipole model, here we investigate the simplest case of one-dimensional arrays of interacting atomic dipoles driven by a weak laser field. Changing the polarization and direction of the driving field allows us to separately address superradiant, subradiant, redshifted, and blueshifted eigenmodes, as well as observe strong Fano-like interferences between different modes. The cooperative eigenvectors can be characterized by the phase difference between nearest-neighbor dipoles, ranging from all oscillating in phase to all oscillating out of phase with their nearest neighbors. Investigating the eigenvalue behavior as a function of atom number and lattice spacing, we find that certain eigenmodes of an infinite atomic chain have the same decay rate as a single atom between two mirrors. The effects we observe provide a framework for collective control of the optical response of a medium, giving insight into the behavior of more complicated geometries, as well as providing further evidence for the dipolar analog of cavity QED.