We introduce the , a nonperiodic analog of the discrete time crystal that arises in periodically driven dissipative quantum many-body systems. This phase is defined by two key features: (1) spatial long-range order arising from the spontaneous breaking of an internal symmetry and (2) temporally chaotic oscillations of the order parameter, whose lifetime diverges with system size. In other words, a time glass is a state of matter in which all components evolve in a synchronized yet chaotic manner. To characterize the time glass phase, we focus on the spectral gap of the one-cycle (Floquet) Liouvillian, which determines the decay rate of the slowest relaxation mode. Theoretical arguments and numerical studies of periodically driven dissipative Ising models show that, in the time glass phase, the Liouvillian gap remains finite in the thermodynamic limit, in contrast to time crystals where the gap closes exponentially with system size. We further demonstrate that the Liouvillian gap converges to the decay rate of the order-parameter autocorrelation derived from the classical (mean-field) dynamics in the thermodynamic limit. This result establishes a direct correspondence between microscopic spectral features and emergent macroscopic dynamics in driven dissipative quantum systems. At first glance, the existence of a nonzero Liouvillian gap appears incompatible with the presence of indefinitely persistent chaotic oscillations. We resolve this apparent paradox by showing that the quantum Rényi divergence between a localized coherent initial state and the highly delocalized steady state grows unboundedly with system size. This divergence allows long-lived transients to persist even in the presence of a finite Liouvillian gap.
We introduce the , a nonperiodic analog of the discrete time crystal that arises in periodically driven dissipative quantum many-body systems. This phase is defined by two key features: (1) spatial long-range order arising from the spontaneous breaking of an internal symmetry and (2) temporally chaotic oscillations of the order parameter, whose lifetime diverges with system size. In other words, a time glass is a state of matter in which all components evolve in a synchronized yet chaotic manner. To characterize the time glass phase, we focus on the spectral gap of the one-cycle (Floquet) Liouvillian, which determines the decay rate of the slowest relaxation mode. Theoretical arguments and numerical studies of periodically driven dissipative Ising models show that, in the time glass phase, the Liouvillian gap remains finite in the thermodynamic limit, in contrast to time crystals where the gap closes exponentially with system size. We further demonstrate that the Liouvillian gap converges to the decay rate of the order-parameter autocorrelation derived from the classical (mean-field) dynamics in the thermodynamic limit. This result establishes a direct correspondence between microscopic spectral features and emergent macroscopic dynamics in driven dissipative quantum systems. At first glance, the existence of a nonzero Liouvillian gap appears incompatible with the presence of indefinitely persistent chaotic oscillations. We resolve this apparent paradox by showing that the quantum Rényi divergence between a localized coherent initial state and the highly delocalized steady state grows unboundedly with system size. This divergence allows long-lived transients to persist even in the presence of a finite Liouvillian gap.
Boundary Time Crystals (BTCs) represent a distinctive form of nonequilibrium temporal order in which persistent oscillations emerge in open dissipative quantum systems without external periodic driving. Although their dynamical characterization is well established through the spectral properties of the Liouvillian, the thermodynamic meaning of persistent temporal order remains less systematically articulated. This work develops a nonequilibrium-thermodynamic framework for interpreting BTCs as emergent dissipative structures sustained by irreversible energy and entropy exchange. The framework connects Liouvillian temporal dynamics with thermodynamic forces and fluxes, entropy production, dissipative organization, and self-organization, thereby providing a common language for describing temporal persistence and irreversible activity within open quantum systems. In addition, phenomenological measures are introduced to characterize the balance between coherent temporal dynamics and dissipative relaxation, together with a normalized entropy-production measure for comparing dynamical regimes. A concrete numerical demonstration based on the established collective-spin BTC model illustrates the framework by contrasting non-BTC and BTC regimes, finite-size temporal decay, and the associated dissipative activity. The results support a thermodynamic interpretation in which persistent temporal order is maintained as a nonequilibrium organized state rather than as a consequence of equilibrium thermodynamics. The proposed framework is complementary to microscopic quantum-thermodynamic treatments of BTCs and does not replace the established Liouvillian criterion for identifying temporal-crystalline order. Instead, it provides a broader conceptual bridge between temporal symmetry breaking, irreversible thermodynamics, and dissipative self-organization, offering a basis for future quantitative studies of the thermodynamic structure and stability of time-crystalline phases.
Boundary time crystals are a class of exotic dissipative quantum phases that spontaneously break continuous time-translation symmetry in the thermodynamic limit of open quantum systems. In finite-size systems, the long-time evolution of boundary time crystals exhibits decaying oscillations that cannot be captured by widely used mean-field theory. To address this issue, we develop an effective approach called the stroboscopic rotating wave approximation, which provides a well-approximated state for the long-time evolution of boundary time crystals in the strongly driven regime. In this approach, the order parameter exhibits both a long-time decaying envelope governed by an effective Lindblad superoperator and short-time oscillations dominated by a reduced quantum dynamical semigroup. Our results reveal that the competition among dephasing processes along three directions induces persistent oscillations, marking the emergence of the boundary-time-crystal phase. We obtain the analytical expressions for the steady-state density operator, the oscillation period, and the decay rate of the order parameter when the coherent energy splitting exceeds the dissipation rate. Our work provides a beyond-mean-field tool for studying the dynamics of periodically driven open quantum systems and understanding the formation of time crystals.
Continuous time crystals (CTCs) represent a nonequilibrium quantum phase that spontaneously breaks time-translation symmetry without periodic external driving, manifesting as persistent, long-lived oscillations under steady pumping. The lifetime is constrained by the instability of the limit cycle phase, balanced between nonlinear feedback and energy dissipation, which have rarely been studied in experiments before. Here, we report an observation of an ultralong-lived Rydberg-atom CTC in a driven-dissipative many-body atomic system. By harnessing long-range interactions and engineering a dissipative environment that stabilizes the limit-cycle dynamics, we suppress heating and decay effects that typically destroy time-crystalline order. The key factor underlying the ultralong-lived CTC is the closing of the Liouvillian gap and the near-zero real part of the system's Liouvillian eigenspectrum. Through systematic optimization, we achieve an oscillatory lifetime exceeding 16.95 hours-orders of magnitude longer than previous CTC realizations. Our work establishes a robust platform for exploring long-lived autonomous nonequilibrium phases and paves the way for applications in quantum sensing and continuous-time quantum information processing.
It presents a significant challenge to elucidate the relationship between the phases of open quantum many-body systems and the spectral structure of their governing Liouvillian, which determines how the density matrix evolves. Previous studies have focused on the Liouvillian gap, defined as the decay rate of the most slowly decaying mode, as a key indicator of dissipative phase transition, noting its closure in symmetry-broken phases and opening in disordered phases. In this work, we propose an additional spectral gap, termed the oscillating-mode gap, defined as the decay rate of the most slowly decaying oscillating mode. Through the analysis of a prototype dissipative boson system, we demonstrate the necessity of both the Liouvillian gap and the oscillating-mode gap for the comprehensive characterization of the system's phases and the transitions between them.
While a generic open quantum system decays to its steady state, continuous time crystals (CTCs) develop spontaneous oscillation and never converge to a stationary state. Just as crystals develop correlations in space, CTCs do so in time. Here, we introduce a continuous quasi time crystals (CQTC). Despite being characterized by the presence of nondecaying oscillations, this phase does not retain its long-range order, making it time analogous to quasicrystal structures. We investigate the emergence of this phase in a minimal model, made of two coupled collective spin subsystems, each developing a CTC phase upon the action of a strong enough drive. The addition of a coupling enables the emergence of different synchronized phases, where both subsystems oscillate at the same frequency. In the transition between different CTC orders, the system develops chaotic dynamics with aperiodic oscillations. These chaotic features differ from those of closed quantum systems, as the dynamics is not characterized by a unitary evolution. We investigate the connection between chaos and this quasicrystalline phase using mean-field techniques, and we confirm these results by including quantum fluctuations at the lowest order.
Abstract We study an emergent semiclassical time crystal composed of two interacting driven-dissipative bosonic modes. The system has a discrete Z 2 spatial symmetry which, depending on the strength of the drive, can be broken in the time-crystalline phase or it cannot. An exact semiclassical mean-field analysis, numerical simulations in the quantum regime, and the spectral analysis of the Liouvillian are combined to show the emergence of the time crystal and to prove the robustness of the oscillation period against quantum fluctuations.