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arXiv:2506.00575

Quantum computation with longlived Rydberg-Landau atoms featuring suppressed ionization by the Magnetic Cage

Amir Momtaheni, Mohammadsadegh Khazali

Published May 31, 2025• 0 citations
arXivHTMLPDF

Abstract

Atomic processing units require robust entanglement between individual qubits, typically achieved via excitation to highly interacting Rydberg states. However, short Rydberg lifetimes and ionization risks limit the quantum volume score of the atomic processing units. Inspired by Landau resonances in alkaline atoms, we introduce Rydberg-Landau (rLandau) states created under a strong magnetic field (2.5 Tesla). These states exhibit significantly extended lifetimes and a magnetic confinement mechanism that prevents ionization, even under intense laser fields. We analyze their wavefunctions, excitation dynamics, dipole transition rules, lifetimes, and interactions, identifying states optimal for high-fidelity quantum operations. This approach simplifies the coherent excitation of long-lived, strongly interacting rLandau circular states akin to Coulombic counterparts, enabling deeper and more complex quantum algorithms.

DOI
10.48550/arxiv.2506.00575

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Atomic processing units require robust entanglement between individual qubits, typically achieved via excitation to highly interacting Rydberg states. However, short Rydberg lifetimes and ionization risks limit the quantum volume score of the atomic processing units. Inspired by Landau resonances in alkaline atoms, we introduce Rydberg-Landau (rLandau) states created under a strong magnetic field (2.5 Tesla). These states exhibit significantly extended lifetimes and a magnetic confinement mechanism that prevents ionization, even under intense laser fields. We analyze their wavefunctions, excitation dynamics, dipole transition rules, lifetimes, and interactions, identifying states optimal for high-fidelity quantum operations. This approach simplifies the coherent excitation of long-lived, strongly interacting rLandau circular states akin to Coulombic counterparts, enabling deeper and more complex quantum algorithms.
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Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from decay due to selection rules. This manifests spectacularly in highly excited Rydberg states. Low angular momentum Rydberg states are at the heart of recent breakthroughs in quantum computing, simulation and sensing with neutral atoms. For these applications the lifetime of the Rydberg levels sets fundamental limits for gate fidelities, coherence times, or spectroscopic precision. The quest for longer Rydberg state lifetimes has motivated the generation, coherent control and trapping of circular Rydberg atoms, which are characterized by the maximally allowed electron orbital momentum and were key to seminal experiments with single atoms and photons. Here, we report the observation of individually trapped circular Rydberg atoms with lifetimes of more than 10 milliseconds, two orders of magnitude longer-lived than the established low angular momentum orbitals. This is achieved via Purcell suppression of blackbody modes at room temperature. We coherently control individual circular Rydberg levels at so far elusive principal quantum numbers of up to n = 103, and observe tweezer trapping of the Rydberg atoms on the hundred millisecond scale. Our results pave the way for quantum information processing and sensing utilizing the combination of extreme lifetimes and giant Rydberg blockade.
The short Doppler-limited coherence time of the laser-excited Rydberg state, usually orders of magnitude shorter than the lifetime of the Rydberg state, hinders the Rydberg-mediated quantum technologies. Here, we show that a 649~nm~−-−~658~nm two-photon excitation of the 6sng 1G46sng~^1G_46sng 1G4​ Rydberg state from a long-lived d-orbital clock state of barium can be achieved with a two-photon wavevector that is tiny, which effectively removes the Doppler-limited decoherence. Moreover, the 6sng 1G46sng~^1G_46sng 1G4​ Rydberg state has strong dipole-dipole interaction due to small Förster defect with nearby Rydberg states and possesses long radiative lifetime. These can benefit quantum computing based on individually trapped neutral atoms, and can enable long-lived Rydberg polaritons in atomic media, which brings fresh opportunities in all-optical quantum information.
We study a hitherto unexplored regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole interaction strength while their ionization rate can be changed over 2 orders of magnitude by small variations of the electric field. We demonstrate laser excitation of the interacting Rydberg states followed by their detection using controlled ionization and magnified imaging with high spatial and temporal resolution. Our work reveals new possibilities to engineer the interaction strength and dynamically control the ionization and detection of Rydberg atoms, which can be useful for realizing and assessing quantum simulators that vary in space and time.
Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of magnitude, as they can be effectively protected from decay due to their maximum angular momentum. We report the first realization of alkaline-earth circular Rydberg atoms trapped in optical tweezers, which provide unique and novel control possibilities due to the optically active ionic core. Specifically, we demonstrate creation of very high- n ( n = 79 ) circular states of Sr 88 . We measure lifetimes as long as 2.55 ms at room temperature, which are achieved via cavity-assisted suppression of black-body radiation. We show coherent control of a microwave qubit encoded in circular states of nearby manifolds, and characterize the qubit coherence time via Ramsey and spin-echo spectroscopy. Finally, circular-state tweezer trapping exploiting the Sr + core polarizability is quantified via measurements of the trap-induced light shift on the qubit. Our work opens routes for quantum simulations with circular Rydberg states of divalent atoms, exploiting the emergent toolbox associated with the optically active core ion. Published by the American Physical Society 2024
Individual neutral atoms excited to Rydberg states are a promising platform for quantum simulation and quantum information processing. However, experimental progress to date has been limited by short coherence times and relatively low gate fidelities associated with such Rydberg excitations. We report progress towards high-fidelity quantum control of Rydberg-atom qubits. Enabled by a reduction in laser phase noise, our approach yields a significant improvement in coherence properties of individual qubits. We further show that this high-fidelity control extends to the multi-particle case by preparing a two-atom entangled state with a fidelity exceeding 0.97(3), and extending its lifetime with a two-atom dynamical decoupling protocol. These advances open up new prospects for scalable quantum simulation and quantum computation with neutral atoms.