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arXiv:2506.00248 · Physical review. B./Physical review. B

Higher-dimensional generalization of the Kitaev spin liquid

Po-Jui Chen, Piers Coleman

Published Mar 19, 2026• 0 citations
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Abstract

We construct an exactly solvable model of a four-dimensional Kitaev spin liquid. The lattice structure is orthorhombic and each unit cell contains six sublattice degrees of freedom. We demonstrate that the Fermi surface of the model is made up of two-dimensional surfaces. Additionally, we evaluate the energy cost of creating visons using scattering theory. The positive bond-flip energy suggests that the flux-free state is locally stable. Our model sheds light on the realization of high-dimensional fractionalization.

DOI
10.1103/fvjg-pb5k

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We construct an exactly solvable model of a four-dimensional Kitaev spin liquid. The lattice structure is orthorhombic and each unit cell contains six sublattice degrees of freedom. We demonstrate that the Fermi surface of the model is made up of two-dimensional surfaces. Additionally, we evaluate the energy cost of creating visons using scattering theory. The positive bond-flip energy suggests that the flux-free state is locally stable. Our model sheds light on the realization of high-dimensional fractionalization.
We study an exactly solvable quantum spin model of Kitaev type on the kagome lattice. We find a rich phase diagram which includes a topological (gapped) chiral spin liquid with gapless chiral edge states, and a gapless chiral spin liquid phase with a spin Fermi surface. The ground state of the current model contains an odd number of electrons per unit cell, which qualitatively distinguishes it from previously studied exactly solvable models with a spin Fermi surface. Moreover, we show that the spin Fermi surface is stable against weak perturbations.
We develop an exactly solvable model with Kitaev-type interactions and study its phase diagram on the dual lattice of the quasicrystalline Ammann-Beenker lattice. Our construction is based on the $\mathrm{\ensuremath{\Gamma}}$-matrix generalization of the Kitaev model and utilizes the cut-and-project correspondence between the four-dimensional simple cubic lattice and the Ammann-Beenker lattice to designate four types of bonds. We obtain a rich phase diagram with gapped (chiral and abelian) and gapless spin liquid phases via Monte Carlo simulations and variational analysis. We show that the ground state can be further tuned by the inclusion of an onsite term that selects 21 different vison configurations while maintaining the integrability of the model. Our results highlight the rich physics at the intersection of quasicrystals and quantum magnetism.
We introduce an extension of the Kitaev honeycomb model by including four-spin interactions that preserve the local gauge structure and, hence, the integrability of the original model. The extended model has a rich phase diagram containing five distinct vison crystals, as well as a symmetric π-flux spin liquid with a Fermi surface of Majorana fermions and a sequence of Lifshitz transitions. We discuss possible experimental signatures and, in particular, present finite-temperature Monte Carlo calculations of the specific heat and the static vison structure factor. We argue that our extended model emerges naturally from generic perturbations to the Kitaev honeycomb model.
The excitation spectrum of Kitaev quantum spin liquids consists of itinerant Majorana fermions, which can be gapless or gapped, and vortices of a Z2\mathbb{Z}_2Z2​ gauge field, known as visons, which are \new{gapped within a stable Z2\mathbb Z_2Z2​ spin liquid phase}. In this work, we investigate visons in Kitaev-type models where the Majorana fermions form a Fermi surface. In this case, the creation of a vison pair is analogous to introducing a local impurity potential in a metal. Since the gapless modes lead to strong finite-size effects, we compare the numerical calculation of the \new{two-vison gap} on finite lattices with the result from an analytical approach based on Green's function techniques. We find that the \new{two-vison gap} decreases as the size of the Fermi surface increases, signalling an instability of the quantum spin liquid ground state. We also show that larger Fermi surfaces tend to suppress the change in local spin correlations due to the Majorana-vison scattering potential.
The exactly solvable Kitaev honeycomb lattice model is realized as the low-energy effect Hamiltonian of a spin-1/2 model with spin rotation and time-reversal symmetry. The mapping to low-energy effective Hamiltonian is exact without truncation errors in traditional perturbation series expansions. This model consists of a honeycomb lattice of clusters of four spin-1/2 moments and contains short-range interactions up to six-spin (or eight-spin) terms. The spin in the Kitaev model is represented not as these spin-1/2 moments but as pseudospin of the two-dimensional spin-singlet sector of the four antiferromagnetically coupled spin-1/2 moments within each cluster. Spin correlations in the Kitaev model are mapped to dimer correlations or spin-chirality correlations in this model. This exact construction is quite general and can be used to make other interesting spin-1/2 models from spin-rotation invariant Hamiltonians. We discuss two possible routes to generate the high-order spin interactions from more natural couplings, which involves perturbative expansions thus breaks the exact mapping, although in a controlled manner.
Three-dimensional Kitaev models -- generalizations of the well known exactly solvable Kitaev honeycomb model -- exhibit a rich variety of quantum spin liquid phases. Their fractionalized excitations are Majorana fermions that may form topological band structures. These can be enriched by lattice symmetries, as shown in the present work. In particular, the authors propose two new instances of Kitaev spin liquids that exhibit nodal chains and 3D Dirac nodes in the bulk. Such crystalline Kitaev spin liquids are direct generalizations of crystalline topological insulators, albeit in an interacting spin system. A potential material realization in metal-organic frameworks is also discussed.