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arXiv:2505.16669

An open harmonic chain: Exact vs global and local reduced dynamics

Melika Babakan, Fabio Benatti, Laleh Memarzadeh

Published May 22, 2025• 0 citations
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Abstract

In the following, we study the dissipative time-evolution of a quantum chain consisting of three coupled harmonic oscillators, the first and third of which weakly interact quadratically with two independent thermal baths in equilibrium at different temperatures. Due to the quadratic form of the total Hamiltonian, the unitary dynamics of the compound system is formally analytically solvable and defines a one-parameter group of Gaussian maps which enables us to solve the exact dynamics of the chain numerically. Following the Gorini-Kossakowski-Sudarshan-Lindblad (GKSL) approach to open quantum systems, one can perform the rotating wave approximation with respect to the interacting, or non-interacting chain Hamiltonian and respectively derive the so-called global and local master equations. The solutions of the ensuing different master equations can then be compared with the exact one, possibly sorting out the two approaches in correspondence to different time-scales of the system. We derive the steady states of the open chain quantum dynamics in the two approaches and show that the behaviour of fidelity between them versus inter-oscillator coupling depends on the two bath temperatures, revealing the existence of a temperature-dependent critical inter-oscillator coupling strength that determines the domain of validity of each approach. When the newly found coupling is less than this critical value, the local approach outperforms the global approach, whereas for larger inter-oscillator coupling, the global approach is a better approximation of the exact evolution. This critical value of inter-oscillator coupling depends on the two bath temperatures, which then play a crucial role in deciding the best possible approximating open dynamics.

DOI
10.48550/arxiv.2505.16669

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In the following, we study the dissipative time-evolution of a quantum chain consisting of three coupled harmonic oscillators, the first and third of which weakly interact quadratically with two independent thermal baths in equilibrium at different temperatures. Due to the quadratic form of the total Hamiltonian, the unitary dynamics of the compound system is formally analytically solvable and defines a one-parameter group of Gaussian maps which enables us to solve the exact dynamics of the chain numerically. Following the Gorini-Kossakowski-Sudarshan-Lindblad (GKSL) approach to open quantum systems, one can perform the rotating wave approximation with respect to the interacting, or non-interacting chain Hamiltonian and respectively derive the so-called global and local master equations. The solutions of the ensuing different master equations can then be compared with the exact one, possibly sorting out the two approaches in correspondence to different time-scales of the system. We derive the steady states of the open chain quantum dynamics in the two approaches and show that the behaviour of fidelity between them versus inter-oscillator coupling depends on the two bath temperatures, revealing the existence of a temperature-dependent critical inter-oscillator coupling strength that determines the domain of validity of each approach. When the newly found coupling is less than this critical value, the local approach outperforms the global approach, whereas for larger inter-oscillator coupling, the global approach is a better approximation of the exact evolution. This critical value of inter-oscillator coupling depends on the two bath temperatures, which then play a crucial role in deciding the best possible approximating open dynamics.
In the following, we study the dissipative time evolution of a quantum chain consisting of three coupled harmonic oscillators, the first and third of which weakly interact quadratically with two independent thermal baths in equilibrium at different temperatures. Due to the quadratic form of the total Hamiltonian, the uni- tary dynamics of the compound system is formally analytically solvable and defines a one-parameter group of Gaussian maps which enables us to solve the exact dynamics of the chain numerically. Following the Gorini-Kossakowski-Sudarshan-Lindblad approach to open quantum systems, one can perform the rotating-wave approximation with respect to the interacting or noninteracting chain Hamiltonian and respectively derive the so-called global and local master equations. The solutions of the ensuing different master equations can then be compared with the exact one, possibly sorting out the two approaches in correspondence to different timescales of the system. We derive the steady states of the open chain quantum dynamics in the two approaches and show that the behavior of fidelity between them versus interoscillator coupling depends on the two bath temperatures, revealing the existence of a temperature-dependent critical interoscillator coupling strength that determines the domain of validity of each approach. When the newly found coupling is less than this critical value, the local approach outperforms the global approach, whereas for larger interoscillator coupling, the global approach is a better approximation of the exact evolution. This critical value of interoscillator coupling depends on the two bath temperatures, which then play a crucial role in deciding the best possible approximating open dynamics.
This dataset contains: 1-Fidelity between the local and global steady state versus inter-oscillator coupling, 2- The evolution of fidelity between the local staedy state and evolved local steady state under the evolution of exact approach as well as the evolution of fidelity between the global staedy state and evolved global steady state under the evolution of exact approach, 3- Critical inter-oscillator coupling versus the temperature of the right bath, for the paper: "An open harmonic chain: Exact vs global and local reduced dynamics" submitted to Physical Review A.
The Lindblad theory of open quantum systems has been successfully applied in various fields ranging from quantum optics, condensed matter physics, and quantum thermodynamics to quantum chemistry. Nevertheless, there are situations where we can compare its predictions to those of exact methods or numerically exact results and find discrepancies between them. One example is the case where a single harmonic oscillator is coupled to a thermal bath of independent harmonic oscillators. In this case, for certain parameters, the exact master equation describes equilibration of the system to a thermal state with a temperature different from the one predicted by the Lindblad master equation. The Lindblad theory, based on a weak coupling between the system and environment as well as the Born-Markov approximation, predicts that the system will evolve to a thermal state whose temperature is equal to the initial temperature of the bath. This result is a consequence of the Born approximation, which supposes that throughout the evolution, the bath only fluctuates around its initial equilibrium state. In this master thesis we study the validity of the Born approximation as well as its consistency with other approximations. By starting from a Hamiltonian for the total system we show that, if the the Born approximation is not invoked, the dynamics of the system is determined by a hierarchy of equations for matrices which can be used to reconstruct the reduced density matrix of the system. This hierarchy approach is fundamentally different from the standard approach, which describes the system dynamics with a weak-coupling master equation, because the hierarchy does not restrict the amount of entanglement possible between the system and the environment. Furthermore, we show how invoking the Born approximation reduces to the usual result and how a generalised ansatz, which we refer to as a generalised Born approximation, reduces the hierarchy to a master equation where the bath temperature is an additional degree of freedom. Finally, we analyse the conservation of the energy of the total system and its relationship to the Markov and secular approximations, and discuss whether imposing it as a condition can fix the time-dependent temperature.
Identifying which master equation is preferable for the description of a multipartite open quantum system is not trivial and has led in recent years to the local vs global debate in the context of Markovian dissipation. We treat here a paradigmatic scenario in which the system is composed of two interacting harmonic oscillators A and B, with only A interacting with a thermal bath---collection of other harmonic oscillators---and we study the equilibration process of the system initially in the ground state with the bath finite temperature. We show that the completely positive version of the Redfield equation obtained using coarse-grain and an appropriate time-dependent convex mixture of the local and global solutions give rise to the most accurate approximations of the whole exact system dynamics, i.e., both at short and at long timescales, outperforming the local and global approaches.
A finite-dimensional quantum system is coupled to a bath of oscillators in thermal equilibrium at temperature T>0 . We show that for fixed, small values of the coupling constant λ , the true reduced dynamics of the system is approximated by the completely positive, trace preserving Markovian semigroup generated by the Davies-Lindblad generator. The difference between the true and the Markovian dynamics is O(|λ|1/4) for all times, meaning that the solution of the Gorini-Kossakowski-Sudarshan-Lindblad master equation is approximating the true dynamics to accuracy O(|λ|1/4) for all times. Our method is based on a recently obtained expansion of the full system-bath propagator. It applies to reservoirs with correlation functions decaying in time as 1/t4 or faster, which is a significant improvement relative to the previously required exponential decay.
In various fields from quantum physics to biology, the open quantum dynamics of a system consisting of interacting subsystems emphasizes its fundamental functionality. The local approach, deriving a dissipator in a master equation by ignoring the inter-subsystem interaction, has been widely used to describe the reduced dynamics due to its robustness to keep the positivity of a density operator. However, one critique is that a stationary state obtained by the approach in the limit of weak system-environment coupling is written in the form of the Gibbs state for the partial Hamiltonian by excluding the inter-subsystem interaction from the total one of the relevant system. As an alternative, the global approach, deriving a dissipator with including the inter-subsystem interaction, under the Born--Markov and secular approximations has attracted much attention, and there is debate concerning its violation of positivity in the short-term region and/or limited parameter region for the Bohr frequencies of the subsystems. In this study, we present a formalism that leads to the time-convolutionless (time-local) master equation obtained by extending the global approach beyond the Born-Markov and secular approximations. We apply it to the excitation energy transfer between interacting sites in which only the terminal site weakly interacts with a bosonic environment of finite temperature in a manner beyond the rotating-wave approximation. We find that the formulation (1) gives the short-time behavior while preserving positivity, (2) shows the oscillatory features that the secular approximation would obscure, and (3) leads to a stationary state very near to the Gibbs state for the total Hamiltonian of the relevant system.