We study the collective decay of an initially inverted ensemble of two-level emitters in two distinct scenarios: when coupled to a squeezed photonic reservoir and when interacting with a one-dimensional waveguide. Using a quantum-state diffusion approach to unravel the emission process, we investigate entanglement and classical correlations along individual quantum trajectories over time. This numerical analysis shows that despite an initial buildup of entanglement and a significant amount of entanglement due to either spin squeezing or dark states at late times, the essential features of the superradiant burst are well described by averages over fully factorizable states. We explain this observation in terms of an almost complete factorization of all 2-local observables, which we identify as a generic property of superradiant decay. Based on this insight, we provide a purely classical theory for the burst in squeezed superradiance, which is both intuitive and exact for a large number of emitters. Moreover, we find that our numerical approach also performs well in the presence of subradiant states, which dominate the slow residual decay of nonuniform ensembles at late times.
We study the collective decay of an initially inverted ensemble of two-level emitters in two distinct scenarios: when coupled to a squeezed photonic reservoir and when interacting with a one-dimensional waveguide. Using a quantum-state diffusion approach to unravel the emission process, we investigate entanglement and classical correlations along individual quantum trajectories over time. This numerical analysis shows that despite an initial buildup of entanglement and a significant amount of entanglement due to either spin squeezing or dark states at late times, the essential features of the superradiant burst are well described by averages over fully factorizable states. We explain this observation in terms of an almost complete factorization of all 2-local observables, which we identify as a generic property of superradiant decay. Based on this insight, we provide a purely classical theory for the burst in squeezed superradiance, which is both intuitive and exact for a large number of emitters. Moreover, we find that our numerical approach also performs well in the presence of subradiant states, which dominate the slow residual decay of nonuniform ensembles at late times.
We study the collective emission of a disordered array of N excited two-level atoms into a one-dimensional photonic waveguide. In the perfectly ordered case, where atoms are spaced by exact integer multiples of the wavelength, the system exhibits the characteristic superradiant burst with a peak emission rate scaling as N 2 . Using large-scale semiclassical simulations, we find that this key signature of superradiance remains asymptotically robust under strong spatial and spectral disorder, but also exhibits subtle finite-size scaling toward this limit. To explain our observations, we provide an analytical variational estimate for the maximal decay rate, which tightly bounds the numerical results and reveals how disorder shapes the collective decay. Specifically, we find that even in the presence of strong disorder, the spins tend to self-organize spontaneously according to their locations, which overall optimizes constructive interference effects and explains the emergence of mirror-asymmetric correlations in superradiant decay. These findings resolve important open questions regarding the existence and nature of superradiance in strongly disordered arrays and offer valuable insights for understanding collective quantum optical phenomena in realistic systems.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
An array of initially excited emitters coupled to a one-dimensional waveguide exhibits superradiant decay under the Born-Markov approximation, manifested as a coherent burst of photons in the output field. In this work, we employ tensor-network methods to investigate its non-Markovian dynamics induced by finite time delays in photon exchange among the emitters. We find that the superradiant burst breaks into a structured train of correlated photons, each intensity peak corresponding to a specific photon number. We quantify the emitter-photon and emitter-emitter entanglement generated during this process and show that the latter emerges in the long-time limit, as part of the excitation becomes trapped within the emitters' singlet subspace. We finally consider the decay of the system's most radiant state, the symmetric Dicke state, and show that time delay can lead to decay rates exceeding those predicted by the Markovian approximation.
We experimentally investigate the collective radiative decay of a fully inverted ensemble of two-level atoms for a chiral, i.e., propagation direction-dependent light-matter coupling. Despite a fundamentally different interaction Hamiltonian which has a reduced symmetry compared to the standard Dicke case of superradiance, we do observe a superradiant burst of light. The burst occurs above a threshold number of atoms, and its peak power scales faster with the number of atoms than in the case of free-space Dicke superradiance. We measure the first-order coherence of the burst and experimentally distinguish two regimes, one dominated by the coherence induced during the excitation process and the other governed by vacuum fluctuations. Our results shed light on the collective radiative dynamics of cascaded quantum many-body systems, i.e., systems in which each quantum emitter is only driven by light radiated by emitters that are upstream in the cascade. Our findings may turn out useful for generating multiphoton Fock states as a resource for quantum technologies. Published by the American Physical Society 2024
We show that idealized Dicke superradiant decay from a fully inverted state can at all times be described by a positive statistical mixture of coherent spin states (CSS). Since CSS are separable, this implies that no entanglement is involved in Dicke decay. Based on this result, we introduce a new numerical quantum trajectory approach leading to low-entanglement unravelings. This opens up new possibilities for employing matrix product state (MPS) techniques for large-scale numerical simulations with collective decay processes.
Dicke superradiance by an ensemble of quantum emitters produces a collective burst of radiation, but no entanglement in the mixed state of the emitters. We show that adding a local kinetic constraint between the emitters generates extensive mixed-state entanglement, while otherwise preserving all key features of Dicke superradiance. Specifically, for any local Boolean constraint, we analytically derive a lower bound for the emission rate which implies a peak intensity ∝N2 and a peak time ∝(logN)/N with number of spins N. This effect enables the superradiantly accelerated preparation of entangled dark states. Hereby, Hilbert-space fragmentation of the Dicke ladder leads to an exponentially branching decay tree that generates a hierarchy of dark states. Importantly, these disconnected manifolds include exponentially many long-range entangled singlet dark states. The explored kinetic constraints and superradiant dynamics can be realized in neutral-atom arrays coupled to an optical cavity, and we suggest a simple and accessible witness to detect the predicted mixed-state entanglement in such experiments. Moreover, we show that entanglement generation is robust against atomic decay and collective dephasing, and should be observable under recently reported experimental conditions. Our results, thereby, offer a general framework and experimentally viable approach for the dissipative engineering of entangled dark states enhanced by superradiance.