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arXiv:2505.10035 · Nature Communications

Observation of Genuine High-dimensional Multi-partite Non-locality in Entangled Photon States

Xiao‐Min Hu, Cen-Xiao Huang, Nicola d'Alessandro, Gabriele Cobucci, Chao Zhang, Yu Guo, Yun‐Feng Huang, Chuan‐Feng Li, Guang‐Can Guo, Xiaoqin Gao, Marcus Huber, Armin Tavakoli, Bi‐Heng Liu

Published May 30, 2025• 12 citations

Abstract

Quantum information science has leaped forward with the exploration of high-dimensional quantum systems, offering greater potential than traditional qubits in quantum communication and quantum computing. To advance the field of high-dimensional quantum technology, a significant effort is underway to progressively enhance the entanglement dimension between two particles. An alternative effective strategy involves not only increasing the dimensionality but also expanding the number of particles that are entangled. We present an experimental study demonstrating multi-partite quantum non-locality beyond qubit constraints, thus moving into the realm of strongly entangled high-dimensional multi-particle quantum systems. In the experiment, quantum states were encoded in the path degree of freedom (DoF) and controlled via polarization, enabling efficient operations in a two-dimensional plane to prepare three- and four-particle Greenberger-Horne-Zeilinger (GHZ) states in three-level systems. Our experimental results reveal ways in which high-dimensional systems can surpass qubits in terms of violating local-hidden-variable theories. Our realization of multiple complex and high-quality entanglement technologies is an important primary step for more complex quantum computing and communication protocols. Experimental demonstrations of genuine high-dimensional multipartite quantum nonlocality have been lacking so far. Here, the authors fill this gap using entangled photons, surpassing qubit-based limits and paving the way for device-independent quantum information processing in more complex systems.

DOI: 10.1038/s41467-025-59717-y

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High-dimensional quantum systems, known as qudits with dimension

d>2

, possess the capability to encode and process more information than traditional two-dimensional qubits. Entangled states serve as crucial resources for both quantum computation and quantum communication. On the basis of circuit quantum electrodynamics (QED) systems, we introduce an efficient scheme to deterministically generate high-dimensional multipartite entangled states of hybrid qutrits (

d=3

). Assuming a simple initial state has already been prepared with the use of local operations, our method requires only a single step to produce hybrid Greenberger-Horne-Zeilinger (GHZ) entangled states among circuit QED systems consisting of superconducting qutrits and a superconducting cavity. Remarkably, the number of steps and the operational time remain constant as the number of qutrits increases, highlighting the efficiency and scalability of our approach. Using numerical simulations for a three-dimensional hybrid GHZ state of seven qutrits, we demonstrate the feasibility of our scheme and study the effects of various parameters on the fidelity. The importance of this research is in directing the experimental creation of multipartite, high-dimensional, and hybrid GHZ states, which can then be used to enhance quantum communication protocols and computational processes.

Characterizing entanglement of systems composed of multiple particles is a very complex problem that is attracting increasing attention across different disciplines related to quantum physics. The task becomes even more complex when the particles have many accessible levels, i.e., they are of high dimension, which leads to a potentially high-dimensional multipartite entangled state. These are important resources for an ever-increasing number of tasks, especially when a network of parties needs to share highly entangled states, e.g., for communicating more efficiently and securely. For these applications, as well as for purely theoretical arguments, it is important to be able to certify both the high-dimensional and the genuine multipartite nature of entangled states, possibly based on simple measurements. Here we derive a novel method that achieves this and improves over typical entanglement witnesses like the fidelity with respect to states of a Greenberger-Horne-Zeilinger (GHZ) form, without needing more complex measurements. We test our condition on paradigmatic classes of high-dimensional multipartite entangled states like imperfect GHZ states with random noise, as well as on purely randomly chosen ones and find that, in comparison with other available criteria our method provides a significant advantage and is often also simpler to evaluate.

High-dimensional qudit (i.e.,

d

-level or

d

-state) systems outperform two-dimensional qubit (i.e., 2-level or 2-state) systems in some quantum information processing tasks. We exploit entanglement purification protocols (EPPs) for extracting a subset of high quality arbitrary

d

-dimensional

n

-partite Greenberger-Horne-Zeilinger (GHZ) states from a large set of less entangled GHZ states. In our protocols, qudit-flip and phase-flip errors can be corrected, and the fidelity of the output state can be asymptotically improved to unity by iterating the EPP process. Moreover, the schemes are immune to the number of polluted photons, the fidelity thresholds of the proposed EPPs are developed, and the spatial-based single-qudit operations can be well manipulated with a range of balanced beam splitters, and phase shifters. These features make the proposed schemes offer an alternative method for high-dimensional multipartite entanglement purification.

Entanglement states serve as the central resource for a number of important applications in quantum information science, including quantum key distribution, quantum precision measurement, and quantum computing. In pursuit of more promising applications, efforts have been made to generate entangled states with more qubits. However, the efficient creation of a high-fidelity multiparticle entanglement remains an outstanding challenge due to the difficulty that increases exponentially with the number of particles. We design an interferometer that is capable of coupling the polarization and spatial paths of photons and prepare 2-D four-qubit GHZ entanglement states. Using quantum state tomography, entanglement witness, and the violation of Ardehali inequality against local realism, the properties of the prepared 2-D four-qubit entangled state are analyzed. The experimental results show that the prepared four-photon system is an entangled state with high fidelity.

High-dimensional entanglement is of great importance in quantum communications and can be realized by encoding information on multiple degrees of freedom (DoFs) of the photons. Conventionally, the realization of such high-dimensional entanglement involves different combinations of bulky optical elements. In this work, we present the use of a single dielectric metasurface to generate high-dimensional entanglement by modulating multi-DoFs of photons. By sending one of the polarization-entangled photons to interact with the metasurface, we encode path, spin angular momentum, and orbital angular momentum information to the original state. We achieve a four-qubit quantum state in the experiment. To verify it, we experimentally demonstrate the nonlocal correlations between the two photons by recording the correlated images, and we also perform a quantum state tomography measurement. This scheme can be applied to on-chip quantum state manipulation, which is promising in quantum communication with integrated components.