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arXiv:2505.09292 · Optics Letters

Robust transfer of a quantum state from an absorbed photon into a diamond spin

Daisuke Ito, Yuhei Sekiguchi, Raustin Reyes, Taichi Fujiwara, Toshiharu Makino, Hiromitsu Kato, Hideo Kosaka

Published Jul 16, 2025• 1 citation
arXivHTMLPDF

Abstract

Conversion of a quantum state from a flying qubit to a memory qubit is crucial for distributed quantum computing. However, this requires precise spatiotemporal or frequency/phase alignment. Here, we experimentally demonstrate quantum teleportation-based state transfer from a photon into a spin in a nitrogen-vacancy center in diamond robust against both spectral and temporal errors. The achieved fidelity exceeds 0.94 within a frequency error of 100 MHz and 0.93 within an arrival-time error of 100 ns. This achievement could enable extraordinarily robust entanglement generation between remote quantum memories compared with the conventional photon-interference-based approaches and paves the way for stable quantum networks.

DOI
10.1364/ol.567933

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Conversion of a quantum state from a flying qubit to a memory qubit is crucial for distributed quantum computing. However, this requires precise spatiotemporal or frequency/phase alignment. Here, we experimentally demonstrate quantum teleportation-based state transfer from a photon into a spin in a nitrogen-vacancy center in diamond robust against both spectral and temporal errors. The achieved fidelity exceeds 0.94 within a frequency error of 100 MHz and 0.93 within an arrival-time error of 100 ns. This achievement could enable extraordinarily robust entanglement generation between remote quantum memories compared with the conventional photon-interference-based approaches and paves the way for stable quantum networks.
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Abstract Quantum networks can enable quantum communication and modular quantum computation. A powerful approach is to use multi-qubit nodes that provide quantum memory and computational power. Nuclear spins associated with defects in diamond are promising qubits for this role. However, dephasing during optical entanglement distribution hinders scaling to larger systems. Here, we show that a 13C-spin quantum memory in isotopically engineered diamond is robust to the optical link operation of a nitrogen-vacancy centre. The memory lifetime is improved by two orders-of-magnitude upon the state-of-the-art, surpassing reported times for entanglement distribution. Additionally, we demonstrate that the nuclear-spin state can survive ionisation and recapture of the nitrogen-vacancy electron. Finally, we use simulations to show that combining this memory with previously demonstrated entanglement links and gates can enable key network primitives, such as deterministic non-local two-qubit gates, paving the way for test-bed quantum networks capable of investigating complex algorithms and error correction.
Abstract Quantum teleportation is a key principle for quantum information technology. It permits the transfer of quantum information into an otherwise inaccessible space, while also permitting the transfer of photon information into a quantum memory without revealing or destroying the stored quantum information. Here, we show reliable quantum state transfer of photon polarization into a carbon isotope nuclear spin coupled to a nitrogen-vacancy center in diamond based on photon-electron Bell state measurement by photon absorption. The carbon spin is first entangled with the electron spin, which is then permitted to absorb a photon into a spin-orbit correlated eigenstate. Detection of the electron after relaxation into the spin ground state allows post-selected transfer of arbitrary photon polarization into the carbon memory. The quantum state transfer scheme allows individual addressing of integrated quantum memories to realize scalable quantum repeaters for long-haul quantum communications, and distributed quantum computers for large-scale quantum computation and metrology.
Quantum repeaters are essential for overcoming the exponential photon loss that limits entanglement generation over long distances in quantum networks. An absorption-emission-based quantum repeater exploits the fundamental light-matter interactions of a diamond nitrogen-vacancy (NV) center---photon absorption and photon emission---to transfer a quantum state from an absorbed photon to an emitted photon, offering a scalable architecture that operates without photon interference between remote nodes. Here we demonstrate an absorption-emission-based quantum repeater node using a single NV center, realizing the complete single-node operation in which heralded photon-to-memory quantum state transfer, repeat-until-success (RUS) emission of a spin-entangled photon, and quantum teleportation of the memory state onto the emitted photon constitute the essential repeater operation. By characterizing the complete repeater operation as a quantum channel from the absorbed photon to the emitted photon via quantum process tomography, we obtain a process fidelity of 78%. This demonstration establishes the absorption-emission approach as a fundamental building block for scalable quantum repeater architectures and paves the way toward practical long-distance quantum networks.
As a kind of hybrid spin system, nitrogen-vacancy (NV) centers in diamond have shown great advantages in implementing quantum registers for quantum information processing (QIP). When scaling up quantum registers to quantum networks for long-distance quantum communication and distributed quantum computation, determining how to entangle two registers in distant nodes is a basic challenge in the absence of direct interactions. In this paper, we present a scheme for entangling two distant NV centers based on the special optical absorption and emission of NV centers. In this demonstration, we transfer the entanglement information of a pair of photons to nuclear spins in NV centers and create remote NV–NV entanglement mediated by entangled photons. We then explain how to extract the entangled information from NV centers to prepare on-demand entangled photons for optical quantum information processing. The strategy of entanglement transfer between spins and photons demonstrated herein may pave the way for an NV-center-based quantum network.
Quantum networks promise secure communication, distributed sensing and modular quantum computing by interconnecting distant quantum nodes through photonic links. Extending such networks beyond metropolitan distances requires quantum repeaters to overcome the exponential attenuation of photons in optical fiber. Across all architectures, a key requirement is the indistinguishability of single photons, which directly impacts the fidelity of photonic operations based on two-photon interference, such as Bell-state measurements and fusion gates. Here, we demonstrate generation of highly indistinguishable single photons from a coherently excited tin-vacancy center in diamond, achieving raw Hong-Ou-Mandel interference visibilities exceeding 0.95. By separating intrinsic emitter properties from technical imperfections, we show that decoherence plays a negligible role and that the remaining limitations are predominantly technical in nature, arriving at an intrinsic indistinguishability of up to 0.999. We further show that quantum frequency conversion to the telecom C-band preserves the photon indistinguishability. In combination with the long-lived electron and nuclear spin coherence times, these results establish tin-vacancy centers in diamond as a competitive platform for long-distance quantum networks and photonic quantum information processing. We further substantiate this potential through Monte Carlo simulations of a quantum-repeater link, demonstrating that the SnV-center platform surpasses the bound set by direct transmission.