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arXiv:2504.07814 · Quantum

Estimating the best separable approximation of non-pure spin-squeezed states

Julia Mathé, Ayaka Usui, Otfried Gühne, Giuseppe Vitagliano

Published Apr 21, 2026• 0 citations
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Abstract

We discuss the estimation of the distance of a given mixed many-body quantum state to the set of fully separable states, applied to the concrete scenario of collective spin states. Concretely, we discuss lower bounds to distances from the set of fully separable states based on entanglement criteria and upper bounds to those distances using an iterative algorithm to find the optimal separable state closest to the target. Focusing on collective states of N spin- 1 / 2 particles, we consider spin-squeezing inequalities (SSIs), which provide a complete set of nonlinear entanglement criteria based on collective spin variances. First, we find a lower bound to distance-based entanglement monotones, specifically the so-called best separable approximation (BSA) from the complete set of SSIs, thereby bypassing entirely a numerical optimization over a (potentially very large) set of linear entanglement witnesses. Then, we improve current algorithms to iteratively find the closest separable state to a given target state, exploiting the symmetry of the system. These results allow us to study entanglement quantitatively on thermal states of spin systems on fully-connected graphs at nonzero temperature, as well as potentially similar states arising in out-of-equilibrium situations. We thus apply our methods to investigate entanglement across different phases of a fully-connected XXZ model. We observe that our lower bound becomes often tight for zero temperature as well as for the temperature at which entanglement disappears, both of which are thus precisely captured by the SSIs. We further observe, among other things, that entanglement can arise at nonzero temperature even in the ordered phase, where the ground state is separable, revealing the potential usefulness of entanglement quantification also beyond the ground state paradigm.

DOI
10.22331/q-2026-04-21-2078

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We discuss the estimation of the distance of a given mixed many-body quantum state to the set of fully separable states, applied to the concrete scenario of collective spin states. Concretely, we discuss lower bounds to distances from the set of fully separable states based on entanglement criteria and upper bounds to those distances using an iterative algorithm to find the optimal separable state closest to the target. Focusing on collective states of N spin- 1 / 2 particles, we consider spin-squeezing inequalities (SSIs), which provide a complete set of nonlinear entanglement criteria based on collective spin variances. First, we find a lower bound to distance-based entanglement monotones, specifically the so-called best separable approximation (BSA) from the complete set of SSIs, thereby bypassing entirely a numerical optimization over a (potentially very large) set of linear entanglement witnesses. Then, we improve current algorithms to iteratively find the closest separable state to a given target state, exploiting the symmetry of the system. These results allow us to study entanglement quantitatively on thermal states of spin systems on fully-connected graphs at nonzero temperature, as well as potentially similar states arising in out-of-equilibrium situations. We thus apply our methods to investigate entanglement across different phases of a fully-connected XXZ model. We observe that our lower bound becomes often tight for zero temperature as well as for the temperature at which entanglement disappears, both of which are thus precisely captured by the SSIs. We further observe, among other things, that entanglement can arise at nonzero temperature even in the ordered phase, where the ground state is separable, revealing the potential usefulness of entanglement quantification also beyond the ground state paradigm.
Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteria provide for two relevant entanglement measures: the best separable approximation and the generalized robustness. This yields a practical method for quantifying entanglement in realistic experimental situations, in particular, when only few measurements of simple observables are available. As a concrete application of this method, we quantify bipartite and multipartite entanglement in spin-squeezed Bose-Einstein condensates of ∼500 atoms, by lower bounding the best separable approximation and the generalized robustness only from measurements of first and second moments of the collective spin operator.
Spin squeezing inequalities (SSI) represent a major tool to probe quantum entanglement among a collection of few-level atoms, and are based on collective spin measurements and their fluctuations. Yet, for atomic ensembles of spin- j atoms and ultracold spinor gases, many experiments can image the populations in all Zeeman sublevels s=−j,−j+1,…,j , potentially revealing finer features of quantum entanglement not captured by SSI. Here we present a systematic approach which exploits Zeeman-sublevel population measurements in order to construct novel entanglement criteria, and illustrate our approach on ground states of spin-1 and spin-2 Bose-Einstein condensates. Beyond these specific examples, our approach allows one to infer, in a systematic manner, the optimal permutationally-invariant entanglement witness for any given set of collective measurements in an ensemble of d -level quantum systems.
Generalizing the well-known spin-squeezing inequalities, we study the relation between squeezing of collective N -particle s u ( d ) operators and many-body entanglement geometry in multi-particle systems. For that aim, we define the set of pseudo-separable states, which are mixtures of products of single-particle states that lie in the ( d 2 − 1 ) -dimensional Bloch sphere but are not necessarily positive semidefinite. We obtain a set of necessary conditions for states of N qudits to be of the above form. Any state that violates these conditions is entangled. We also define a corresponding s u ( d ) -squeezing parameter that can be used to detect entanglement in large particle ensembles. Geometrically, this set of conditions defines a convex set of points in the space of first and second moments of the collective N -particle s u ( d ) operators. We prove that, in the limit N ≫ 1 , such set is filled by pseudo-separable states, while any state corresponding to a point outside of this set is necessarily entangled. We also study states that are detected by these inequalities: We show that states with a bosonic symmetry are detected if and only if the two-body reduced state violates the positive partial transpose (PPT) criterion. On the other hand, highly mixed states states close to the s u ( d ) singlet are detected which have a separable two-body reduced state and are also PPT with respect to all possible bipartitions. We also provide numerical examples of thermal equilibrium states that are detected by our set of inequalities, comparing the spin-squeezing inequalities with the s u ( 3 ) -squeezing inequalities.
We present criteria to detect the depth of entanglement in macroscopic ensembles of spin- j particles using the variance and second moments of the collective spin components. The class of states detected goes beyond traditional spin-squeezed states by including Dicke states and other unpolarized states. The criteria derived are easy to evaluate numerically even for systems of very many particles and outperform past approaches, especially in practical situations where noise is present. We also derive analytic lower bounds based on the linearization of our criteria, which make it possible to define spin-squeezing parameters for Dicke states. In addition, we obtain spin squeezing parameters also from the condition derived in (Sørensen and Mølmer 2001 Phys. Rev. Lett. 86 4431 ). We also extend our results to systems with fluctuating number of particles.
What is the relation between spin squeezing and entanglement? To clarify this, we derive the full set of generalized spin squeezing inequalities for the detection of entanglement. These are inequalities for the mean values and variances of the collective angular momentum components. They can be used for the experimental detection of entanglement in a system of spin‐12 particles in which the spins cannot be individually addressed. We also show how to obtain the complete set of entanglement conditions if the mean spin and the spin correlation matrix are known. Finally, we apply our criteria for entanglement detection in spin models, showing that they can be used to detect bound entanglement in the thermal state of these systems.
How can we analyze quantum correlations in large and noisy systems without quantum state tomography? An established method is to measure total angular momenta and employ the so-called spin-squeezing inequalities based on their expectations and variances. This allows detection of metrologically useful entanglement, but efficient strategies for estimating such nonlinear quantities have yet to be determined. In this paper we show that spin-squeezing inequalities can not only be evaluated by measurements of the total angular momentum but also by two-qubit correlations, either involving all pair correlations or randomly chosen pair correlations. Then we analyze the estimation errors of our approaches in terms of a hypothesis test. For this purpose, we discuss how error bounds can be derived for nonlinear estimators with the help of their variances, characterizing the probability of falsely detecting a separable state as entangled. We focus on the spin-squeezing inequalities in multiqubit systems. Our methods, however, can also be applied to spin-squeezing inequalities for qudits or for the statistical treatment of other nonlinear parameters of quantum states.