Rydberg atom triangular arrays in an optical cavity serve as an ideal platform for understanding the interplay between geometric frustration and quantized photons. Using a large-scale quantum Monte Carlo method, we obtain a rich ground state phase diagram. Around half-filling, the infinite long-range light-matter interaction lifts the ground state degeneracy, resulting in a novel order-coexisted superradiant clock phase that completely destroys the fragile order-by-disorder phase observed in classical light fields. According to the Ginzburg-Landau theory, this replacement may result from the competition between threefold and sixfold clock terms. Similar to the spin supersolid, the clear first-order phase transition at the Z_{2} symmetry line is attributed to the nonzero photon density, which couples to the threefold clock term. Finally, we discuss the low-energy physics in the dimer language and propose that cavity-mediated nonlocal ring exchange interactions may play a critical role in the rich physics induced by the attachment of cavity QED. Our Letter opens a new arena of research on the emergent phenomena of quantum phase transitions in many-body quantum optics.
Rydberg atom triangular arrays in an optical cavity serve as an ideal platform for understanding the interplay between geometric frustration and quantized photons. Using a large-scale quantum Monte Carlo method, we obtain a rich ground state phase diagram. Around half-filling, the infinite long-range light-matter interaction lifts the ground state degeneracy, resulting in a novel order-coexisted superradiant clock phase that completely destroys the fragile order-by-disorder phase observed in classical light fields. According to the Ginzburg-Landau theory, this replacement may result from the competition between threefold and sixfold clock terms. Similar to the spin supersolid, the clear first-order phase transition at the Z_{2} symmetry line is attributed to the nonzero photon density, which couples to the threefold clock term. Finally, we discuss the low-energy physics in the dimer language and propose that cavity-mediated nonlocal ring exchange interactions may play a critical role in the rich physics induced by the attachment of cavity QED. Our Letter opens a new arena of research on the emergent phenomena of quantum phase transitions in many-body quantum optics.
We study the two-dimensional Rydberg atom array in an optical cavity with the help of a variational method and large-scale quantum Monte Carlo simulations. The strong dipole-dipole interactions between Rydberg atoms can make the system exhibit a crystal structure, and the coupling between a two-level atom and a cavity photon mode can result in the formation of a polariton. The interplay between them provides a rich quantum phase diagram including the Mott, solid-1/2, superradiant, and superradiant solid (SRS) phases. As a two-order coexisted phase, the superradiant solid breaks both translational and U(1) symmetries. Different from the fragile SRS phase in a one-dimensional system [Zhang et al., Phys. Rev. Lett. 110, 090402 (2013)], the SRS phase stays in a larger parameter region. Thus, it is more feasible to detect a SRS phase and corresponding quantum criticality in the real system involving dissipations. Our work not only extends the understanding of the light-atom interacting system, but also provides the guidelines and benchmark for the future experiments.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
Confinement is a pivotal phenomenon in numerous models of high-energy and statistical physics. In this study, we investigate the emergence of confined meson excitations within a one-dimensional system, comprising Rydberg-dressed atoms trapped and coupled to a cavity field. This system can be effectively represented by an Ising-Dicke Hamiltonian model. The observed ground-state phase diagram reveals a first-order transition from a ferromagnetic-subradiant phase to a paramagnetic-superradiant phase. Notably, a quench near the transition point within the ferromagnetic-subradiant phase induces meson oscillations in the spins and leads to the creation of squeezed-vacuum light states. We suggest a method for the photonic characterization of these confined excitations, utilizing homodyne detection and single-site imaging techniques to observe the localized particles. The methodologies and results detailed in this Letter are feasible for implementation on existing cavity-QED platforms, employing Rydberg-atom arrays in deep optical lattices or optical tweezers.
We study an optical cavity coupled to a lattice of Rydberg atoms, which can be represented by a generalized Dicke model. We show that the competition between the atom-atom interaction and atom-light coupling induces a rich phase diagram. A novel superradiant solid (SRS) phase is found, where both the superradiance and crystalline orders coexist. Different from the normal second order superradiance transition, here both the solid-1/2 and SRS to SR phase transitions are first order. These results are confirmed by large scale quantum Monte Carlo simulations.
Locality is a transversal principle that governs quantum dynamics of many-body systems. However, for cavity-embedded systems, such a fundamental notion is hindered by the presence of nonlocal cavity modes, leaving space for new possible dynamical behavior. Here, we investigate the real-time dynamics of low-energy excitations in one-dimensional Rydberg atom arrays coupled to a global cavity mode. We derive an effective description in terms of a Tavis-Cummings-Ising model, whose phase diagram features ordered and disordered phases. The nonlocal nature of the cavity mode drastically affects the emergent meson and string dynamics. Mesons hybridize coherently with the cavity photons, leading to composite meson-polariton excitations. Strings, differently from local interacting theories, acquire a finite kinetic energy thanks to nonlocal cavity-mediated interactions between the underlying domain walls. We then conclude by presenting a new concrete experimental blueprint for a cavity QED Rydberg atom array simulator where the physics outlined in this Letter can be realized.
We study the properties of a generalized Dicke-Ising model realized with an array of Rydberg atoms, driven by microwave electric fields and coupled to an optical cavity. As this platform allows for a precisely tunable anisotropy parameter, the model exhibits a rich landscape of phase transitions and critical phenomena, induced by the interplay of rotating-wave, counter-rotating-wave, and Ising interactions. We develop an improved quantum Monte Carlo algorithm based on the stochastic series expansion that explicitly tracks the Fock state of the quantum cavity. In the superradiant (SR) phase, this allows us to determine, through data collapse, the scaling laws of the photon number. We also demonstrate the vanishing of parity symmetry in finite-size simulations and show that the Rydberg blockade leads to a significant suppression of cavity occupation. Notably, stronger quantum fluctuations induced by the counter-rotating wave terms slightly favor the superradiant solid (SRS) phase over the Solid-1/2 state. Finally, we confirm that the SR phase transition and the transition from the Solid-1/2 to the SRS are second-order. In contrast, the transitions from the Solid-1/2 or SRS to the SR phase are both first-order for any value of the normalized anisotropy parameter.