A promising route toward quantum networking is via photons as information carriers, requiring deterministic quantum nonlinear optical operations and single-photon routing. Here, we demonstrate a direction-switchable single-photon emitter using a Rydberg polariton. The Rydberg component of the stored photon is changed using a stimulated Raman transition with a specific intermediate state. By adjusting the direction of the retrieval laser, we can redirect the emitted photon into a rich variety of alternative modes. We experimentally demonstrate a redirection angle of ∼100 ∘ . Building upon this scheme, we propose a quantum routing of single photons with N output channels by rotation of the retrieval laser, where all directions have identical routing efficiency. In addition, the protocol reduces the effect of motional dephasing, increasing the photon lifetime to >10µs (>20 times the photon processing time), enabling functional quantum devices based on Rydberg polaritons.
A promising route toward quantum networking is via photons as information carriers, requiring deterministic quantum nonlinear optical operations and single-photon routing. Here, we demonstrate a direction-switchable single-photon emitter using a Rydberg polariton. The Rydberg component of the stored photon is changed using a stimulated Raman transition with a specific intermediate state. By adjusting the direction of the retrieval laser, we can redirect the emitted photon into a rich variety of alternative modes. We experimentally demonstrate a redirection angle of ∼100 ∘ . Building upon this scheme, we propose a quantum routing of single photons with N output channels by rotation of the retrieval laser, where all directions have identical routing efficiency. In addition, the protocol reduces the effect of motional dephasing, increasing the photon lifetime to >10µs (>20 times the photon processing time), enabling functional quantum devices based on Rydberg polaritons.
Quantum nonlinear optics by Rydberg polaritons can enable single-photon transistor and switch, single-photon source, and deterministic quantum information processing. A major hindrance in this study is the fast motional decoherence. Here, we devise a scheme to significantly enhance the coherence of Rydberg polariton by letting the atoms {\it remember} their velocities, or, alternatively, by {\it changing} the phase of Rydberg polariton according to its storage time. After the Rydberg polariton is prepared with a Rydberg state ∣r1⟩, i.e., during the storage time, two laser fields induce a transition between ∣r1⟩ and a nearby Rydberg state ∣r2⟩ via a low-lying intermediate state ∣f⟩ which is largely detuned. In particular, we find that either a 2πN protocol, a π-wait-π protocol, or a wait-π protocol, along with an appropriate choice of ∣f⟩ can lead to a phase-coherent Rydberg polariton upon its retrieval. Importantly, the coherent transition between ∣r1⟩ and ∣r2⟩ ensures that the Rydberg polariton can block the Rydberg excitation of nearby atoms as in usual applications of Rydberg polaritons. Numerics show that the theory can nearly completely eliminate the motional dephasing, leaving Rydberg-state decay as the only fundamental channel of decoherence. This sheds light on a broad application of Rydberg-mediated quantum nonlinear optics.
Mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons enables the realization of optical nonlinearities which can modify light on the level of individual photons.This novel approach forms the basis of a growing Rydberg quantum optics toolbox, which already contains photonic logic building-blocks such as single-photon sources, switches, transistors, and conditional π-phase shifts.This thesis reports on two experiments investigating strong photon-photon interactions mediated by Rydberg interactions.First, applying a ladder-type EIT scheme to Rydberg atoms in D-states with high principal quantum number results in the Rydberg interaction mediated nonlinearity accompanied by a time-dependent decay of transmission of probe light through the medium.In a joint experimental and theoretical analysis, this effect is attributed to the dephasing of propagating polaritons into stationary Rydberg excitations caused by the state mixing interaction occurring with Rydberg D-state atoms.Second, via a two-photon Raman excitation scheme Rydberg atoms are efficiently excited in a small atomic cloud.As the size of the Rydberg blockade exceeds the dimension of the medium, only a single Rydberg excitation can be present at a time.By fast engineered dephasing this Rydberg excitation is decoupled from the light field.Measurement of the transmitted light and the amount of excited Rydberg atoms gives evidence for the realization of a deterministic single-photon absorber.
Photons are ideal carriers of quantum information: they are fast, low-loss, and compatible with mature photonic infrastructure.Linear optical quantum computing exploits these properties but relies on probabilistic measurements and post-selection, incurring an exponential resource overhead that limits scalability [1].Circumventing this bottleneck requires deterministic quantum logic gates, which in turn demand strong, controllable interactions between individual photons.Photons do not interact in free space or in linear optical media.The standard route to attain effective photonphoton interactions is to hybridise photons with interacting matter excitations, forming polaritons.The matter component introduces an interaction-induced anharmonic level shift U into the ladder of polariton states: when one polariton occupies a mode, the next photon sees a shifted resonance (Fig. 1a).The key figure of merit is U/γ, where γ is the total polariton decoherence rate.For U/γ ≪ 1 the nonlinearity is classical; for U/γ ≳ 1 the system enters the quantum nonlinear regime, enabling photon blockade, large conditional phase shifts, and deterministic photonic gates.Atomic Rydberg systems have provided the clearest demonstration of this regime.Atoms excited to Rydberg states -electronic states with large principal quantum numbers n ≫ 1 -possess unique properties [2].Their lifetimes scale as 1/γ ∝ n 3 and transition dipole moments as µ ∝ n 2 , leading to strong dipole-dipole (U ∝ n 4 /r 3 ) or van der Waals (U ∝ n 11 /r 6 ) interactions over long distances r.These interactions can be imprinted onto photons via electromagnetically induced transparency (EIT) [3]: photons hybridise with collective atomic excitations to form slowly propagating Rydberg polaritons that strongly interact with each other over distances of up to tens of micrometres [4].This mechanism has produced photon blockade [5]
Quantum emitters coupled to nanophotonic structures are an excellent platform for controllable single-photon scattering. The tunable light-matter interaction enables the construction of a single-photon switch -- a device that can route a single photon from an input port to a selected output port. Such single-photon switching devices can be integrated into reconfigurable photonic circuits to actively control the photon propagation direction in a quantum network. Ideally, a single-photon switch should operate with high speed, efficiency, and fidelity, preserving the state of the input photon in the routing process. This review brings together key input-output methods from quantum optics, theoretical proposals of emitter-based single-photon routing mechanisms, and experimental demonstrations of single-photon switching devices across different physical platforms, including semiconductor quantum dots, neutral atoms, superconducting qubits, and color centers. We highlight the need for reporting the key figures of merit (speed/efficiency/fidelity) in future single-photon switch demonstrations to support further developments in the field.
For several decades, scientists have been aware of significant benefits allowing quantum information processing technologies to surpass their classical counterparts. Recent technological development allows these benefits to be tested experimentally and in some cases also implemented in practical devices. So far the majority of experimental quantum networks was limited to peer-to-peer communications between two parties. Practical implementation of quantum communications networks, however, needs to address the problem of scalability to serve large numbers of users. Similarly to classical computer networks, their quantum counterparts would require routing protocols to direct the signal from its source to destination. Devices implementing these routing protocols are called quantum routers and have recently been subject of an intense research. In this paper, we report on experimental implementation of a linear-optical quantum router. Our device allows single-photon polarization-encoded qubits to be routed coherently into two spatial output modes depending on the state of two identical control qubits. The polarization qubit state of the routed photon is maintained during the routing operation. The success probability of our scheme can be increased up to 25% making it the most efficient linear-optical quantum router developed to this date.
Single-photons of well-defined polarization that are deterministically generated in a single spatio-temporal field mode are the key to the creation of multi-partite entangled states in photonic networks. Here, we present a novel scheme to produce such photons from a single atom in an optical cavity, by means of vacuum-stimulated Raman transitions between the Zeeman substates of a single hyperfine state. Upon each transition, a photon is emitted into the cavity, with a polarization that depends on the direction of the Raman process.