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arXiv:2504.02256

A direct algebraic proof for the non-positivity of Liouvillian spectral values and controlling the dissipative gap of systems with normal Lindblad operators

Yikang Zhang, Thomas Barthel

Published Apr 3, 2025• 0 citations
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Abstract

Markovian open quantum systems are described by the Lindblad master equation $\partial_tρ=\mathcal{L}(ρ)$, where $ρ$ denotes the system's density operator and $\mathcal{L}$ the Liouville super-operator, which is also known as the Liouvillian. For systems with a finite-dimensional Hilbert space, it is a fundamental property of the Liouvillian that the real parts of all its eigenvalues are non-positive. Analogously, for infinite-dimensional Hilbert spaces, the Liouvillian as a map on trace-class operators only has spectral values with non-positive real parts. The usual arguments for these properties are indirect, using that $\mathcal{L}$ generates a quantum channel and that quantum channels are contractive. We provide a direct algebraic proof based on the Lindblad form of Liouvillians. Subtleties for infinite-dimensional systems are highlighted. For example, unbounded operators can then be eigenvectors of the adjoint Liouvillian with positive eigenvalues, corresponding to a physical instability of the system. As an illustrative application of the algebraic approach, we prove that a strict minimum can be imposed on the dissipative gap of any Markovian spin-$s$ or fermionic many-particle system with normal Lindblad operators by adding simple local dissipators. The added dissipators comprise Pauli or generalized Pauli Lindblad operators for spin systems and Majorana Lindblad operators for fermionic systems.

DOI
10.48550/arxiv.2504.02256

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We study generic open quantum systems with Markovian dissipation, focusing on a class of stochastic Liouvillian operators of Lindblad form with independent random dissipation channels (jump operators) and a random Hamiltonian. We perform a thorough numerical study, focusing on global spectral features, the spectral gap, and the steady-state purity and statistics. We establish that all properties follow three different regimes as a function of the dissipation strength, whose boundaries depend on the particular observable. Within each regime, we determine the scaling exponents with the dissipation strength and system size. On the analytical side, we compute the average spectral gap at arbitrary dissipation and provide simple closed-form expressions for the asymptotic values at strong and weak dissipation strength. We also consider spectral correlations in generic complex spectra, such as that of the Liouvillian. We introduce and study, both analytically and numerically, the complex ratio of the nearest-neighbor spacing by next-to-nearest-neighbor spacing. Besides the usual level repulsion, we find that complex spacing ratios have a nontrivial angular dependence which offers a distinct signature of quantum chaos. It distinguishes integrable systems, which support the flat ratio distribution characteristic of Poisson statistics, and chaotic dissipative quantum systems, which conform to Random Matrix Theory statistics. We apply this new signature of quantum chaos to random Liouvillians and boundary-driven dissipative spin-chains. The results of this thesis can help understand the long-time dynamics, steady-state properties, and spectral correlations of generic dissipative systems.
Strong dynamical symmetries provide an algebraic description of persistent oscillations in open quantum systems governed by the Lindblad equation. For finite-dimensional systems with a full-rank stationary state, such symmetries are necessary and sufficient for non-decaying oscillatory modes to appear in the Liouvillian's spectrum. These modes can be directly constructed by acting on stationary states with the identified symmetry operators. Here we establish an asymptotic counterpart of this algebra for collective spins. Taking a single spin SSS in a magnetic field, subject to dissipation through linear jump operators, we identify the exact conditions on the field and dissipative couplings under which non-decaying oscillatory modes emerge as S→∞S \rightarrow \inftyS→∞. We then write down a simple, closed form for the corresponding `symmetry' operator which can be applied to the steady state to construct these modes, which are eigenvectors of the Liouvillian, with imaginary eigenvalues, up to O(1/S)O(1/S)O(1/S) corrections. A second operator, an emergent conserved quantity, completes the algebra, and its slow relaxation determines how quantum noise selects the stationary state. The construction can be directly extended to a pair of interacting spins sharing a common reservoir, with the resulting quantum algebra making the entanglement during a quench analytically accessible.
Abstract The dynamics of Markovian open quantum systems are described by Lindblad master equations. For fermionic and bosonic systems that are quasi-free, i.e. with Hamiltonians that are quadratic in the ladder operators and Lindblad operators that are linear in the ladder operators, we derive the equation of motion for the covariance matrix. This determines the evolution of Gaussian initial states and the steady states, which are also Gaussian. Using ladder super-operators (a.k.a. third quantization), we show how the Liouvillian can be transformed to a many-body Jordan normal form which also reveals the full many-body spectrum. Extending previous work by Prosen and Seligman, we treat fermionic and bosonic systems on equal footing with Majorana operators, shorten and complete some derivations, also address the odd-parity sector for fermions, give a criterion for the existence of bosonic steady states, cover non-diagonalizable Liouvillians also for bosons, and include quadratic systems. In extension of the quasi-free open systems, quadratic open systems comprise additional Hermitian Lindblad operators that are quadratic in the ladder operators. While Gaussian states may then evolve into non-Gaussian states, the Liouvillian can still be transformed to a useful block-triangular form, and the equations of motion for k -point Green’s functions form a closed hierarchy. Based on this formalism, results on criticality and dissipative phase transitions in such models are discussed in a companion paper.
We study spectral and steady-state properties of generic Markovian dissipative systems described by quadratic fermionic Liouvillian operators of the Lindblad form. The Hamiltonian dynamics is modeled by a generic random quadratic operator, i.e., as a featureless superconductor of class D, whereas the Markovian dissipation is described by M M random linear jump operators. By varying the dissipation strength and the ratio of dissipative channels per fermion, m=M/(2N_F) m = M / ( 2 N F ) , we find two distinct phases where the support of the single-particle spectrum has one or two connected components. In the strongly dissipative regime, this transition occurs for m=1/2 m = 1 / 2 and is concomitant with a qualitative change in both the steady-state and the spectral gap that rules the large-time dynamics. Above this threshold, the spectral gap and the steady-state purity qualitatively agree with the fully generic (i.e., non-quadratic) case studied recently. Below m=1/2 m = 1 / 2 , the spectral gap closes in the thermodynamic limit and the steady-state decouples into an ergodic and a nonergodic sector yielding a non-monotonic steady-state purity as a function of the dissipation strength. Our results show that some of the universal features previously observed for fully random Liouvillians are generic for a sufficiently large number of jump operators. On the other hand, if the number of dissipation channels is decreased the system can exhibit nonergodic features, rendering it possible to suppress dissipation in protected subspaces even in the presence of strong system-environment coupling.