According to Zaanen's interpretation of Homes' empirical law~[Zaanen, {\it Nature} {\bf 430}, 512 (2004)], the superconducting transition temperatures in the cuprates are high because their metallic states are as viscous as quantum mechanics permits. Here, we show that Homes' law in fact implies three key points: (i) the resistivity is linear in temperature in the normal state near the transition temperature; (ii) the dimensionless coefficient of proportionality of the relaxation rate with temperature is of order unity -- the so-called universal Planckian relaxation rate; and (iii) the logarithmically broad applicability of this law arises from an unusually wide range of effective masses throughout the cuprate phase diagram. In fact, a universal Planckian relaxation rate implies Homes' law only if the mechanism of mass renormalization is independent of the Planckian relaxation.
The mysterious metallic phase showing perfect
T-linear resistivity and a universal scattering rate
1/τ=αPkBT/ℏ with a universal prefactor
αP∼1 and logarithmic-in-temperature singular specific heat coefficient, so-called Planckian metal phase was observed in various overdoped high-
Tc cuprate superconductors over a finite range in doping. Here, we propose a microscopic mechanism for this exotic state based on quantum-critical bosonic charge Kondo fluctuations coupled to both spinon and a heavy conduction-electron Fermi surfaces within the heavy-fermion formulation of the slave-boson
t-
J model. Using a controlled perturbative renormalization group (RG) analysis, we examine the competition between the pseudogap phase, characterized by Anderson's Resonating-Valence-Bond spin-liquid, and the Fermi-liquid state, characterized by the electron hoping (effective charge Kondo effect). We find a quantum-critical metallic phase with a universal Planckian
ℏω/kBT scaling in scattering rate near a localized-delocalized (pseudogap-to-Fermi liquid) charge Kondo breakdown transition. Our results are in excellent agreement with the recent experimental observations on optical conductivity (without fine-tuning) in Nat. Commun. 14, 3033 (2023), universal doping-independent field-to-temperature scaling in magnetoresistance in Nature 595, 661 (2021), and the marginal Fermi-liquid spectral function observed in ARPES (Science 366, 1099 (2019)) as well as Hall coefficient in various overdoped cuprates in Nature 595, 661 (2021) and Annu. Rev. Condens. Matter Phys. 10, 409 (2019). Our mechanism offers a microscopic understanding of the quantum-critical Planckian metal phase observed in cuprates d-wave superconducting, and Fermi liquid phases.
Abstract The mysterious metallic phase showing T-linear resistivity and a universal scattering rate 1 / τ = α P k B T / ℏ with a universal prefactor α P ∼ 1 and logarithmic-in-temperature singular specific heat coefficient, the so-called ‘Planckian metal phase’ was observed in various overdoped high- T c cuprate superconductors over a finite range in doping. Revealing the mystery of the Planckian metal state is believed to be the key to understanding the mechanism for high- T c superconductivity. Here, we propose a generic microscopic mechanism for this state based on quantum-critical local bosonic charge Kondo fluctuations coupled to both spinon and a heavy conduction-electron Fermi surface within the heavy-fermion formulation of the slave-boson t–J model. By a controlled perturbative renormalization group analysis, we examine the competition between the pseudogap phase, characterized by Anderson’s Resonating-Valence-Bond spin-liquid, and the Fermi-liquid state, modeled by the electron hopping (effective charge Kondo effect). We find a quantum-critical metallic phase with a universal Planckian ℏ ω / k B T scaling in scattering rate near an extended localized-delocalized (pseudogap-to-Fermi liquid) charge-Kondo breakdown transition. The d-wave superconducting ground state emerges near the transition. Unprecedented qualitative and quantitative agreements are reached between our theoretical predictions and various experiments, including optical conductivity, universal doping-independent field-to-temperature scaling in magnetoresistance, specific heat coefficient, marginal Fermi-liquid spectral function observed in ARPES, and Fermi surface reconstruction observed in Hall coefficients in various overdoped cuprates. Our mechanism offers a microscopic understanding of the quantum-critical Planckian metal phase observed in cuprates and its link to the pseudogap, d-wave superconducting, and Fermi liquid phases. It offers a promising route for understanding how d-wave superconductivity emerges from such a strange metal phase in cuprates–one of the long-standing open problems in condensed matter physics since 1990s–as well as shows a broader implication for the Planckian strange metal states observed in other correlated unconventional superconductors.
Abstract Materials tuned to a quantum critical point display universal scaling properties as a function of temperature T and frequency ω. A long-standing puzzle regarding cuprate superconductors has been the observed power-law dependence of optical conductivity with an exponent smaller than one, in contrast to T-linear dependence of the resistivity and ω-linear dependence of the optical scattering rate. Here, we present and analyze resistivity and optical conductivity of La2−xSrxCuO4 with x = 0.24. We demonstrate ℏω/kBT scaling of the optical data over a wide range of frequency and temperature, T-linear resistivity, and optical effective mass proportional to
∼lnT ~ ln T corroborating previous specific heat experiments. We show that a T, ω-linear scaling Ansatz for the inelastic scattering rate leads to a unified theoretical description of the experimental data, including the power-law of the optical conductivity. This theoretical framework provides new opportunities for describing the unique properties of quantum critical matter.
Understanding the
T-linear normal-state resistivity of cuprates remains a central physics challenge. The associated momentum relaxation rate,
ΓM, saturates near the conjectured ``Planckian" bound
ΓM∼kT/ℏ, but the mechanism underlying the anomalous scattering remains unresolved. Here we employ nonlinear terahertz spectroscopy to systematically study La
2−xSr
xCuO
4 across a broad temperature and doping range. We measure the normal-state third-order susceptibility,
∣χ(3)∣≈6×10−9 m
2/V
2, among the largest in the THz regime, enabling direct access to the rarely measured electronic energy relaxation rate,
ΓE. Strikingly,
ΓE is 10-40 times smaller than
ΓM, revealing that the scatterings responsible for momentum loss and
T-linear resistivity do not remove appreciable energy from the electrons. While
ΓM(T) is consistent with quasi-elastic scattering from bosonic modes above their characteristic energy scale, this is incompatible with the increasing temperature dependence of
ΓE(T). Our results exclude phonons as the source of
T-linear resistivity and impose strong constraints on possible mechanisms.
Relaxational processes for conduction electrons in metals come with characteristic temperature dependences; classic examples at low temperatures are the
1/T2 law for the relaxation time in a Fermi liquid, and the Bloch
1/T5 law for electron-phonon scattering. The strange metal phase of cuprate superconductors is governed instead by the Planckian time, which is given in terms of fundamental constants only. This Colloquium discusses the concept of such a fundamental timescale and the degree to which it provides a lower bound for relaxation times, and illustrates these ideas with examples from conventional and unconventional metals.
The mysterious quantum-critical Planckian bad metal phase with perfect T-linear resistivity persisting beyond the quasi-particle limit and universal T-linear scattering rate has been observed in various high-Tc cuprate superconductors. Here, we develop a realistic theoretical approach to this phase in an analytically solvable large-N multi-channel Kondo lattice model, derived from a heavy-fermion formulated conventionaL t-J model, known for qualitatively describing cuprates. This phase is originated from critical charge Kondo fluctuations where disordered local bosonic charge fluctuations couple to spinon and heavy conduction-electron Fermi surfaces near a charge-Kondo-breakdown local quantum critical point associated with pseudogap-to-Fermi liquid transition. Our results show excellent agreement with experiments and offer broad implications for other unconventional superconductors.