The bottom-up design of strongly interacting quantum materials with prescribed ground-state properties is a highly nontrivial task, especially if only simple constituents with realistic two-body interactions are available on the microscopic level. Here we study two- and three-dimensional structures of two-level systems that interact via a simple blockade potential in the presence of a coherent coupling between the two states. For such strongly interacting quantum many-body systems, we introduce the concept of to construct symmetric blockade structures with strong quantum fluctuations that lead to equal-weight superpositions of tailored states. Drawing from these results, we design a quasi-two-dimensional periodic quantum system that—as we show rigorously—features a topological Z 2 spin liquid as its ground state. Our construction is based on the implementation of a local symmetry on the microscopic level in a system with only two-body interactions.
The bottom-up design of strongly interacting quantum materials with prescribed ground-state properties is a highly nontrivial task, especially if only simple constituents with realistic two-body interactions are available on the microscopic level. Here we study two- and three-dimensional structures of two-level systems that interact via a simple blockade potential in the presence of a coherent coupling between the two states. For such strongly interacting quantum many-body systems, we introduce the concept of to construct symmetric blockade structures with strong quantum fluctuations that lead to equal-weight superpositions of tailored states. Drawing from these results, we design a quasi-two-dimensional periodic quantum system that—as we show rigorously—features a topological Z 2 spin liquid as its ground state. Our construction is based on the implementation of a local symmetry on the microscopic level in a system with only two-body interactions.
Exactly solvable models of topologically ordered phases with non-abelian anyons typically require complicated many-body interactions which do not naturally appear in nature. This motivates the "inverse problem" of quantum many-body physics: given microscopic systems with experimentally realistic two-body interactions, how to design a Hamiltonian that realizes a desired topological phase? Here we solve this problem on a platform motivated by Rydberg atoms, where elementary two-level systems couple via simple blockade interactions. Within this framework, we construct Hamiltonians that realize topological orders described by non-abelian quantum double models. We analytically prove the existence of topological order in the ground state, and present efficient schemes to prepare these states. We also introduce protocols for the controlled adiabatic braiding of anyonic excitations to probe their non-abelian statistics. Our construction is generic and applies to quantum doubles D(G) for arbitrary finite groups G. We illustrate braiding for the simplest non-abelian quantum double D(S3).
Excitation gap of a blockade structure with Z2 topological order
Mathematically rigorous statements on the spectral gap of quantum many-body systems in the thermodynamic limit are notoriously difficult to prove -- yet they are of fundamental importance for classifying quantum phases of matter. Here we prove the existence of a finite excitation gap for a particular Hamiltonian which was proposed in [T. F. Maier et al., PRX Quantum 6, 030340 (2025)] and is motivated by the Rydberg platform. The Hamiltonian exhibits only two-body blockade interactions between two-level systems and has a topologically ordered ground state in the toric code phase. We show that our result also applies to a broader class of blockade Hamiltonians which realize non-Abelian quantum double phases and were proposed in [H. P. Büchler et al., Phys. Rev. B 114, 065113 (2026)]. The proof builds on known gap stability results and exploits the local symmetry of the studied models.
The Schrödinger equation is nearly a century old, yet we are still in the midst of uncovering the remarkable phenomena emerging in many-body quantum systems. From superconductivity to anyonic quasiparticles, nature consistently surprises with its rich self-organization. To elucidate and grasp this variety, it is paramount to understand the phases of matter that can occur in many-body ground states, as well as their emergent collective excitations. Of particular interest are topological phases of matter, characterized by exotic excitations or edge phenomena. There exist by now several universal frameworks for gapped systems, i.e., those with an energy gap above the ground state. However, in the last decade, a multitude of gapless quantum wires---effectively one-dimensional systems---have been reported to be topologically non-trivial. A framework for their understanding and classification is missing. In addition to ground state order---topological or otherwise---a more complete picture involves the properties of excitations above the ground state. Alas, little is known about excitations beyond the universal low-energy regime. In part, this is due to a lack of analytical and numerical methods able to describe excitations at finite energies, especially in strongly-interacting systems beyond one dimension. In this thesis, we address these issues: firstly, we build a general understanding of topological phases in one dimension, including both gapped and gapless cases. In particular, we unify previously studied examples into a single framework. Secondly, we develop a novel numerical method for obtaining spectral functions in two dimensions---these give direct insight into the properties of excitations and are moreover experimentally measurable. Using this numerical method, we uncover a variety of robust properties of excitations at finite energies. Part I of this thesis concerns gapped and gapless topological phases in one dimension. In Chapter 2, we first treat the case of non-interacting fermions. Therein, we review the known classification of gapped phases before extending it to the gapless case, showing that exponentially-localized Majorana zero modes can still emerge at the edge when the bulk is gapless. Interacting gapped phases are discussed in Chapter 3, with a focus on symmetry-protected topological order. These have already been classified; our contribution is to provide a non-technical review of this classification as well as showing that many paradigmatic model Hamiltonians can be related to one another. Finally, Chapter 4 introduces the notion of symmetry-enriched quantum criticality, which we propose as a framework for classifying gapless phases. The key message is that in the presence of symmetries, a universality class can divide into distinct phases, characterized by the symmetry action on the low-energy scaling operators. This includes gapless topological phases, with examples hiding in plain sight; we clarify their stability and reinterpret previously studied examples. Part II studies the excitations above the ground states of two-dimensional quantum spin models. The main object of our study is the dynamic spin structure factor; this type of spectral function is reviewed in the first part of Chapter 5. The second part of this chapter introduces a novel matrix-product-state-based algorithm to efficiently compute it, opening a new window on the dynamics of two-dimensional quantum systems. We benchmark this numerical method in Chapter 6 on the exactly-solvable Kitaev model---a paradigmatic topological model realizing a quantum spin liquid. By adding non-integrable Heisenberg perturbations, we identify the first unequivocal theoretical realization of a proximate spin liquid: the ground state becomes conventionally ordered, yet the high-energy spectral properties are structurally similar to those of the nearby Kitaev spin liquid. The latter agrees with aspects of recent inelastic neutron scattering experiments on alpha-RuCl3. In Chapter 7, we turn to one of the oldest models in many-body quantum physics: the spin-1/2 Heisenberg antiferromagnet on the square lattice. Despite its venerable history, there is still disagreement about the physical origin of high-energy spectral features which low-order spin wave theory cannot account for. We provide a simple picture for this strongly-interacting-magnon feature by connecting it to a simple Ising limit. Lastly, Chapter 8 discusses the stability of quasiparticles---collective excitations behaving like a single emergent entity, of which magnons are a prime example. These are often known to be stable at the lowest energies and are presumed to decay whenever this is seemingly allowed by energy and momentum conservation. However, we show that strong interactions can prevent this from happening. We numerically confirm this principle of avoided decay in the (slightly-detuned) Heisenberg antiferromagnet on the triangular lattice. Moreover, we can even identify its fingerprints in existing experimental data on Ba3CoSb2O9 and superfluid helium. In this thesis, we thus enlarge our understanding of quantum phases and their excitations. The identification of the key principles of gapless topological phases in one dimension calls for direct analogues in higher dimensions, waiting to be uncovered. With regard to the robust properties of the excitations identified in this thesis, we are hopeful that these can be extended into a theory of quasiparticle properties away from the universal low-energy regime.
This dissertation establishes and investigates new phenomena in diverse interacting many-body quantum systems guided by three distinct, but complementary, themes: (i) symmetry and topology, (ii) localization, and (iii) non-Fermi liquids. The first theme concerns how the interplay of symmetry and topology can offer robust protection for a many-body system. We investigate low-dimensional quantum fermionic models from a general structural perspective. These phases can exhibit fractionalized Majorana zero-energy modes on their boundary. We devise experimentally relevant nonlocal measurements that can be used to detect these topological phases. While our primary focus is on quantum systems, topologically protected behavior can arise in classical mechanical models as well. We extend a recent connection between the topological band theory of electrons and classical physics by proposing a mechanical analogue of a topological nodal semimetal.The second theme concerns that of many-body localization. We demonstrate that the combination of localization, symmetry, and topology can have radical consequences for quantum systems at high energies, such as the existence of protected gapless boundary modes. We show that, even at these high energies, quantum information can be preserved, and quantum coherence recovered. Quantum coherent dynamics in this regime is unexpected and of great interest for quantum computation.The third direction in our study of interacting many-body systems concerns non-Fermi liquids. We construct a non-Fermi liquid by bringing together a spin-orbit coupled Fermi surface and fluctuating magnetic order. Using newly developed analytic tools for strongly coupled systems, we demonstrate the stability of the non-Fermi liquid to ordering. This identifies an experimentally accessible candidate for exploring physics that lies beyond Fermi liquid theory.
This dissertation establishes and investigates new phenomena in diverse interacting many-body quantum systems guided by three distinct, but complementary, themes: (i) symmetry and topology, (ii) localization, and (iii) non-Fermi liquids. The first theme concerns how the interplay of symmetry and topology can offer robust protection for a many-body system. We investigate low-dimensional quantum fermionic models from a general structural perspective. These phases can exhibit fractionalized Majorana zero-energy modes on their boundary. We devise experimentally relevant nonlocal measurements that can be used to detect these topological phases. While our primary focus is on quantum systems, topologically protected behavior can arise in classical mechanical models as well. We extend a recent connection between the topological band theory of electrons and classical physics by proposing a mechanical analogue of a topological nodal semimetal.The second theme concerns that of many-body localization. We demonstrate that the combination of localization, symmetry, and topology can have radical consequences for quantum systems at high energies, such as the existence of protected gapless boundary modes. We show that, even at these high energies, quantum information can be preserved, and quantum coherence recovered. Quantum coherent dynamics in this regime is unexpected and of great interest for quantum computation.The third direction in our study of interacting many-body systems concerns non-Fermi liquids. We construct a non-Fermi liquid by bringing together a spin-orbit coupled Fermi surface and fluctuating magnetic order. Using newly developed analytic tools for strongly coupled systems, we demonstrate the stability of the non-Fermi liquid to ordering. This identifies an experimentally accessible candidate for exploring physics that lies beyond Fermi liquid theory.
Interactions among atoms can lead to emergent phenomena, one of the most fascinating being topological order. Topological phases are important in understanding high-temperature superconductors and fault-tolerant quantum computing. Quantum spin liquids, a key example of topologically ordered phases, exhibit unique properties such as long-range entanglement in the ground state and support of anyonic excitations, making them an exciting focus in the study of strongly correlated systems. This thesis explores the detection and learning of topological phases in quantum many-body systems, including quantum spin models, cuprate superconductors and ultracold atomic platform of Rydberg atom arrays. Guided by the experiments on Kitaev materials, we begin by using spinon mean-field theory of quantum spin liquids to explain the transition from a quantized thermal Hall effect to an unquantized values. Making closer connections to experiments in cuprates, we include additional interactions with phonons present in the system. We examine how spinon-phonon interactions, characterized by symmetry analysis, give rise to a chiral phonon Hall viscosity and can also contribute to the thermal Hall effect. In the second part, we turn to Rydberg atom arrays, which have recently been shown to realize a Z2 quantum spin liquid phase—an elusive state in conventional solid-state materials. We study how Rydberg interactions and lattice geometries lead to the emergence of Z2 gauge theories and distinct classes of topological quantum spin liquids. Finally, we study a variational tensor network tomography method for learning topological states from randomized measurements on Rydberg atom arrays. We demonstrate its efficiency in characterizing complex two-dimensional states that could be realized in future experiments.