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arXiv:2503.11802 · Physical Review Letters

Nonequilibrium Critical Scaling of a Squeezing Phase Transition

Arman Duha, Samuel E. Begg, Thomas Bilitewski

Published Sep 11, 2025• 2 citations
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Abstract

We investigate phase transitions in the nonequilibrium dynamics of power-law interacting spin-1/2 bilayer XXZ models, which have recently been shown to allow generation of entanglement in the form of two-mode squeezing. We find a transition between a collective phase characterized by Heisenberg limited squeezing and a partially collective phase with scalable squeezing. We identify universal scaling of the squeezing dynamics in terms of system parameters and a divergent timescale, establishing these as distinct dynamical phases within the framework of nonequilibrium critical phenomena. Our Letter demonstrates a novel dynamical phase transition with potential applications in quantum sensing and quantum simulation in cold-atomic, molecular, or Rydberg platforms.

DOI
10.1103/7g55-lpff

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We investigate phase transitions in the nonequilibrium dynamics of power-law interacting spin-1/2 bilayer XXZ models, which have recently been shown to allow generation of entanglement in the form of two-mode squeezing. We find a transition between a collective phase characterized by Heisenberg limited squeezing and a partially collective phase with scalable squeezing. We identify universal scaling of the squeezing dynamics in terms of system parameters and a divergent timescale, establishing these as distinct dynamical phases within the framework of nonequilibrium critical phenomena. Our Letter demonstrates a novel dynamical phase transition with potential applications in quantum sensing and quantum simulation in cold-atomic, molecular, or Rydberg platforms.
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Non-equilibrium phase transitions of open quantum systems generically exhibit diverging classical but not quantum correlations. Still entanglement -- characterizing the latter correlations -- can be sensitive to the phase transition. Furthermore, mutual information, bounding the total correlations, should exhibit critical scaling at the transition. In this work, we study these quantities in the steady state of open quantum Ising chains with power-law interactions (with the exponent 0≤α≤30\le α\le 30≤α≤3) where spins are subject to spontaneous emission. The bulk of this paper is dedicated to a detailed analytical as well as numerical analysis of the infinite-range model (α=0α=0α=0), a model that is closely related to the paradigmatic open Dicke model. Our main findings are that the entanglement, while being finite, peaks, exhibits a kink and takes a universal value at the transition, while the mutual information exhibits critical scaling not only at the transition but well into the ordered phase, underscoring a hidden criticality that is not captured by (two-point) correlations. We consider three distinct entanglement measures: logarithmic negativity; quantum Fisher information; and, spin squeezing. Specifically, we show that the collective spin operator that maximizes the quantum Fisher information can be identified with the \textit{gapless} mode of the phase transition, while the squeezed direction is that of the \textit{gapped} mode. Finally, we investigate power-law interacting models using matrix product states where we find comparable bounds on squeezing even when no phase transition is expected (for larger ααα), thus the connection to the phase transition does not appear to hold for shorter-range interactions.
We demonstrate a general mechanism to generate scalable, metrologically useful entanglement in the form of generalized spin squeezing in multi-level (qudit) spin systems with power-law interactions. We demonstrate this for spin-changing dynamics, extending the physics of spin-nematic squeezing known from spinor BECs to spatially extended lattice geometries. In the absence of all-to-all connectivity, the dynamics generally suffers from leakage into non-collective finite-momentum modes, destroying Heisenberg scaling. We show that introducing local su(D)\mathfrak{su}(D)su(D) exchange interactions establishes an energy gap that protects the fully symmetric collective manifold, suppressing non-collective excitations, and achieving Heisenberg scaling ξ2∝1/Nξ^2\propto1/Nξ2∝1/N in one to three dimensions for any power-law exponent. We provide an analytical understanding of the mechanism via the analysis of the Bogoliubov excitation spectrum, and demonstrate its effectiveness via numerical simulations of the quantum many-body dynamics. Our findings more broadly apply to other spin-squeezing Hamiltonians, and directly generalize to larger internal spin dimensions. Our results provide a practical pathway towards scalable Heisenberg-limited qudit entanglement generation in experimental platforms such as arrays of (polar) molecules, magnetic atoms, and Rydberg atoms realizing multi-level spin systems.
Universality and scaling laws are hallmarks of equilibrium phase transitions and critical phenomena. However, extending these concepts to non-equilibrium systems is an outstanding challenge. Despite recent progress in the study of dynamical phases, the universality classes and scaling laws for non-equilibrium phenomena are far less understood than those in equilibrium. In this work, using a trapped-ion quantum simulator with single-spin resolution, we investigate the non-equilibrium nature of critical fluctuations following a quantum quench to the critical point. We probe the scaling of spin fluctuations after a series of quenches to the critical Hamiltonian of a long-range Ising model. With systems of up to 50 spins, we show that the amplitude and timescale of the post-quench fluctuations scale with system size with distinct universal critical exponents, depending on the quench protocol. While a generic quench can lead to thermal critical behavior, we find that a second quench from one critical state to another (i.e. a double quench) results in a new universal non-equilibrium behavior, identified by a set of critical exponents distinct from their equilibrium counterparts. Our results demonstrate the ability of quantum simulators to explore universal scaling beyond equilibrium.