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arXiv:2502.19479 · Physical Review Letters

Probing Green’s Function Zeros by Cotunneling through Mott Insulators

Carl Lehmann, Lorenzo Crippa, Giorgio Sangiovanni, Jan Carl Budich

Published Aug 8, 2025• 5 citations
arXivHTMLPDF

Abstract

Quantum tunneling experiments have provided deep insights into basic excitations occurring as Green's function poles in the realm of complex quantum matter. However, strongly correlated quantum materials also allow for Green's functions zeros (GFZs) that may be seen as an antidote to the familiar poles and have so far largely eluded direct experimental study. Here, we propose and investigate theoretically how cotunneling through Mott insulators enables direct access to the shadow band structure of GFZs. In particular, we derive an effective Hamiltonian for the GFZ that is shown to govern the cotunneling amplitude and reveal fingerprints of many-body correlations clearly distinguishing the GFZ structure from the underlying free Bloch band structure of the system. Our perturbative analytical results are corroborated by numerical data in the framework of both exact diagonalization and matrix product state simulations for a one-dimensional model system consisting of a Su-Schrieffer-Heeger-Hubbard model coupled to two single-level quantum dots.

DOI
10.1103/jnq4-sykq

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Quantum tunneling experiments have provided deep insights into basic excitations occurring as Green's function poles in the realm of complex quantum matter. However, strongly correlated quantum materials also allow for Green's functions zeros (GFZs) that may be seen as an antidote to the familiar poles and have so far largely eluded direct experimental study. Here, we propose and investigate theoretically how cotunneling through Mott insulators enables direct access to the shadow band structure of GFZs. In particular, we derive an effective Hamiltonian for the GFZ that is shown to govern the cotunneling amplitude and reveal fingerprints of many-body correlations clearly distinguishing the GFZ structure from the underlying free Bloch band structure of the system. Our perturbative analytical results are corroborated by numerical data in the framework of both exact diagonalization and matrix product state simulations for a one-dimensional model system consisting of a Su-Schrieffer-Heeger-Hubbard model coupled to two single-level quantum dots.
Topology without quasiparticles has emerged as a key framework for understanding Mott insulators, where Green's-function zeros encode nontrivial topological structure. Yet, experimental detection of these zeros represents a challenge. Using exact diagonalization of the one-dimensional Hubbard model with an impurity and Zeeman field, supported by exact analytic results, we show that Green's-function zeros manifest as an in-gap spectral weight in the unitary scattering regime. In this limit, we map the impurity problem onto a doped Mott insulator and identify the resulting in-gap state as a "zeron" excitation which is a localized doublon (holon) for an attractive (repulsive) potential. The zeron spectral weight and its associated zero vanish above a critical Zeeman field. Our results imply that Green's function zeros have in fact already been observed in experiments, and establish impurity and magnetic-field tuning as practical tools for controlling their topology.
The topological classification of electronic band structures is based on symmetry properties of Bloch eigenstates of single-particle Hamiltonians. In parallel, topological field theory has opened the doors to the formulation and characterization of non-trivial phases of matter driven by strong electron-electron interaction. Even though important examples of topological Mott insulators have been constructed, the relevance of the underlying non-interacting band topology to the physics of the Mott phase has remained unexplored. Here, we show that the momentum structure of the Green's function zeros defining the "Luttinger surface" provides a topological characterization of the Mott phase related, in the simplest description, to the one of the single-particle electronic dispersion. Considerations on the zeros lead to the prediction of new phenomena: a topological Mott insulator with an inverted gap for the bulk zeros must possess gapless zeros at the boundary, which behave as a form of "topological antimatter" annihilating conventional edge states. Placing band and Mott topological insulators in contact produces distinctive observable signatures at the interface, revealing the otherwise spectroscopically elusive Green's function zeros.
While correlated insulators are devoid of low-energy quasiparticle poles, their Green functions retain clean momentum structure through zeros. However, precisely what zeros imply is not clear. By studying the extended Hubbard model both analytically and numerically, we establish a new paradigm for strongly correlated matter: the dispersion of Green function zeros is determined by both microscopic spin-spin correlations and defect kinematics. In fact, we find that the dispersion changes discontinuously across the transition between the Mott and the checkerboard charge-density wave phases as is expected for a first-order transition. This physics is robust to the inclusion of further neighbor hopping which simply fine tunes the spin-correlation or charge-defect kinematics. We conclude that it is the {\it dispersion} of the Green-function zeros that encode the physics of ordering resultant from the strong correlations.
Many strongly correlated electron systems fall outside the conventional quasiparticle paradigm. Their low-energy fermionic excitations need not be adiabatically connected to the bare electrons or appear as poles of the physical electron single-particle Green's function. This thesis investigates to what extent an effective quasiparticle description can nevertheless survive, and which emergent degrees of freedom provide the appropriate low-energy structure. First, the interaction-driven evolution from a quantum spin Hall insulator to a Mott insulator is studied using the dynamical cluster approximation. Dispersive zeros of the single-particle Green's function emerge near the Mott transition and retain a nontrivial topological character. When symmetry breaking is allowed, a nontopological excitonic insulator is found to intrude between quantum spin Hall and Mott insulators. Encoding both poles and zeros within a low-energy quasiparticle Hamiltonian provides a continuous one-body description of the three phases. On the Mott side, its gap evolution supports interpreting the soft excitonic mode as a bound state of quasiparticle and quasihole excitations tied to the Green's function zeros, rather than to the widely separated Hubbard bands. Second, the intrinsic anomalous Hall conductivity of a topological metal is analyzed within a multiband extension of Landau Fermi-liquid theory. Residual interactions among quasiparticles at the Fermi surface dress the dynamic current vertex and generate corrections to the Berry-curvature contribution obtained from the quasiparticle bands alone. Our result supports recent claims that the correct expressions for topological observables include vertex corrections besides the topological invariants built just upon the Green's function. It also demonstrates that such corrections are naturally accounted for by Landau Fermi-liquid theory. Extracting the relevant ingredients for an effective description of material-relevant correlated systems requires computational tools that remain reliable at low temperatures. To this end, a deterministic strong-coupling impurity solver for dynamical mean-field theory is discussed. By providing static, dynamical, and thermodynamic observables without stochastic sampling, it offers a promising route toward multiorbital and spin-orbit coupled problems where conventional Monte Carlo methods currently struggle. Finally, the auxiliary quasiparticle framework underlying the ghost-Gutzwiller Ansatz is investigated. On a model for correlated quantum spin Hall insulators, we show that the topology of the interacting state is encoded in the auxiliary one-body Hamiltonian. The resulting band-structure reveals topological Hubbard bands whose topological character can be tuned through a finite magnetization. When applied to the single-band t-J model, the same framework yields a fractionalized Fermi liquid (FL*). In this phase, dispersive neutral spinons, with vanishing physical-electron spectral weight, coexist with conventional quasiparticles forming a small hole-like Fermi surface, thus violating Luttinger's theorem. The corresponding temperature--doping phase diagram contains a low-doping FL*, a d-wave superconducting dome, and an overdoped conventional Fermi liquid, thereby reproducing key qualitative features of cuprate phenomenology.
A new non-perturbative framework for many-body correlated systems is formulated by extending the operator projection method (OPM). This method offers a systematic expansion which enables us to project into the low-energy structure after extracting the higher-energy hierarchy. This method also opens a way to systematically take into account the effects of collective excitations. The Mott-Hubbard metal-insulator transition in the Hubbard model is studied by means of this projection beyond the second order by taking into account magnetic and charge fluctuations in the presence of the high-energy Mott-Hubbard structure. At half filling, the Mott-Hubbard gap is correctly eproduced between the separated two bands. Near half filling, a strongly renormalized low-energy single-particle excitations coexisting with the Mott-Hubbard bands are shown to appear. Signifcance of momentum-dependent self-energy in the results is stressed.
Luttinger's theorem constrains the particle density of interacting fermions through global properties of the single-particle Green's function, and its violation signals a breakdown of the identification between the quantized Hall response and the Green-function-based Ishikawa-Matsuyama invariant. This phenomenon becomes especially compelling in strongly correlated topological phases, such as fractional Chern insulators, where fractionalized quasiparticles lack an adiabatic connection to electrons, raising the question of how Green's-function-based topological invariants manifest in such phases. Using exact diagonalization of the fermionic Harper-Hofstadter-Hubbard model, we compute bulk single-particle Green's functions deep inside a fractional Chern insulating phase and directly evaluate the Luttinger count, its possible correction (the Luttinger integral), and the Ishikawa-Matsuyama invariant N3[G]N_3[\mathrm{G}]N3​[G]. We demonstrate a clear violation of Luttinger's theorem and show that the fractional nature of the many-body Chern number is encoded in the Středa response of the Luttinger integral, while the integer invariant N3[G]N_3[\mathrm{G}]N3​[G] arises from the Středa response of the Luttinger count. We also analytically prove that N3[G]N_3[\mathrm{G}]N3​[G] is fully determined by the Luttinger count together with the Chern number of the occupied Bloch band, upon neglecting Bloch-band mixing. Finally, we propose an experimental protocol to extract all Green-function-based topological invariants from local density-of-states measurements, experimentally accessible in fractional quantum Hall systems.