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arXiv:2502.12105

Interplay of Quantum Coherence and Nonequilibrium Quantum Transport: An Exact Density Matrix Formulation in the Heisenberg Framework

Saikumar Krithivasan, Thingujam Yaiphalemba Meitei, Arijit Sen, Md. Manirul Ali

Published Feb 17, 2025• 0 citations
arXivHTMLPDF

Abstract

We aim to bridge the gap between quantum coherence, quantum correlations, and nonequilibrium quantum transport in a quantum double-dot (QDD) system interacting with fermionic reservoirs. The system-reservoir coupling is modeled using a Fano-Anderson-type Hamiltonian. The density operator elements of the QDD system are expressed in terms of expectation values involving various combinations of the fermionic creation and annihilation operators associated with the system. By utilizing the quantum Langevin equation and the Heisenberg equation of motion, we derive the precise temporal behavior of these operator averages in terms of nonequilibrium Green's functions and subsequently obtain the time evolution of the density operator elements. Our approach is valid in both the strong coupling and non-Markovian regimes. Additionally, we examine the time evolution of quantum coherence in the QDD system, quantifying it using standard measures such as the l1-norm and the relative entropy of coherence. As observed, coherence reaches a non-zero steady-state value, highlighting its significant potential for applications in quantum information processing and quantum technologies. Furthermore, we establish a connection between quantum coherence and transport current in a QDD system serially coupled to fermionic reservoirs. We then investigate the effects of coupling strength and reservoir memory by tuning the finite spectral width of the reservoir, examining their impact on both transient and steady-state properties, such as quantum coherence and particle current, which could play a crucial role in ultrafast nanodevice applications.

DOI
10.48550/arxiv.2502.12105

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We aim to bridge the gap between quantum coherence, quantum correlations, and nonequilibrium quantum transport in a quantum double-dot (QDD) system interacting with fermionic reservoirs. The system-reservoir coupling is modeled using a Fano-Anderson-type Hamiltonian. The density operator elements of the QDD system are expressed in terms of expectation values involving various combinations of the fermionic creation and annihilation operators associated with the system. By utilizing the quantum Langevin equation and the Heisenberg equation of motion, we derive the precise temporal behavior of these operator averages in terms of nonequilibrium Green's functions and subsequently obtain the time evolution of the density operator elements. Our approach is valid in both the strong coupling and non-Markovian regimes. Additionally, we examine the time evolution of quantum coherence in the QDD system, quantifying it using standard measures such as the l1-norm and the relative entropy of coherence. As observed, coherence reaches a non-zero steady-state value, highlighting its significant potential for applications in quantum information processing and quantum technologies. Furthermore, we establish a connection between quantum coherence and transport current in a QDD system serially coupled to fermionic reservoirs. We then investigate the effects of coupling strength and reservoir memory by tuning the finite spectral width of the reservoir, examining their impact on both transient and steady-state properties, such as quantum coherence and particle current, which could play a crucial role in ultrafast nanodevice applications.
Quantum discord captures quantum correlations beyond entanglement and can remain finite even when the entanglement vanishes. We investigate the transient nonequilibrium dynamics and steady-state behavior of quantum discord and classical correlations in a double quantum dot (DQD) system coupled to fermionic reservoirs. By employing a quantum Langevin equation formalism, we obtain the exact reduced density matrix of the system, enabling a comprehensive analysis of its quantum and classical correlations under nonequilibrium conditions. The influence of system-reservoir coupling strength, spectral bandwidth, thermal bias, and varying initial state on both the transient dynamics and steady-state correlations is systematically analyzed. Quantum discord remains finite in the nonequilibrium steady state over a broad parameter range. Although thermal gradients reduce the overall magnitude of correlations, quantum discord persists and exhibits greater resilience. These results demonstrate that nonequilibrium electronic transport, together with the environmental spectral properties and reservoir asymmetry, provides an effective means of controlling nonclassical correlations in mesoscopic systems and establishes quantum discord as a robust hallmark of open fermionic quantum devices.
We consider a finite quantum system under slow driving and weakly coupled to thermal reservoirs at different temperatures. We present a systematic derivation of the quantum master equation for the density matrix and the out-of-time-order correlators. We start from the microscopic Hamiltonian and we formulate the equations ruling the dynamics of these quantities by recourse to the Schwinger-Keldysh nonequilibrium Green's function formalism, performing a perturbative expansion in the coupling between the system and the reservoirs. We focus on the adiabatic dynamics, which corresponds to considering the linear response in the ratio between the relaxation time due to the system-reservoir coupling and the time scale associated to the driving. We calculate the particle and energy fluxes. We illustrate the formalism in the case of a qutrit coupled to bosonic reservoirs and of a pair of interacting quantum dots attached to fermionic reservoirs, also discussing the relevance of coherent effects.
Transport in open quantum systems can be explored through various theoretical frameworks, including the quantum master equation, scattering matrix, and Heisenberg equation of motion. The choice of framework depends on factors such as the presence of interactions, the coupling strength between the system and environment, and whether the focus is on steady-state or transient regimes. Existing literature mainly treats these frameworks independently. Our work establishes connections between them by clarifying the role and status of these approaches using two paradigmatic models for single and multipartite quantum systems in a two-terminal setup under voltage and temperature biases. We derive analytical solutions in both steady-state and transient regimes for the populations, currents, and current correlation functions. Exact results from the Heisenberg equation are shown to align with scattering matrix and master equation approaches within their respective validity regimes. Crucially, we establish a protocol for the weak-coupling limit, bridging the applicability of master equations at weak-coupling with Heisenberg or scattering matrix approaches at arbitrary coupling strength. Published by the American Physical Society 2024
In this review article, we present a non-equilibrium quantum transport theory for transient electron dynamics in nanodevices based on exact Master equation derived with the path integral method in the fermion coherent-state representation. Applying the exact Master equation to nanodevices, we also establish the connection of the reduced density matrix and the transient quantum transport current with the Keldysh nonequilibrium Green functions. The theory enables us to study transient quantum transport in nanostructures with back-reaction effects from the contacts, with non-Markovian dissipation and decoherence being fully taken into account. In applications, we utilize the theory to specific quantum transport systems, a variety of quantum decoherence and quantum transport phenomena involving the non-Markovian memory effect are investigated in both transient and stationary scenarios at arbitrary initial temperatures of the contacts.
We analytically and numerically investigate the steady-state entanglement and coherence of two coupled qubits, each interacting with a local boson or fermion reservoir, based on the Bloch-Redfield master equation beyond the secular approximation. We find that there is nonvanishing steady-state coherence in the nonequilibrium scenario, which grows monotonically with the nonequilibrium condition quantified by the temperature difference or chemical potential difference of the two baths. The steady-state entanglement, in general, is a nonmonotonic function of the nonequilibrium condition as well as the bath parameters in the equilibrium setting. We also discover that weak interqubit coupling and high base temperature or chemical potential of the baths can strongly suppress the steady-state entanglement and coherence, regardless of the strength of the nonequilibrium condition. On the other hand, the energy detuning of the two qubits, when used in a compensatory way with the nonequilibrium condition, can lead to significant enhancement of the steady-state entanglement in some parameter regimes. In addition, the qubits typically have a stronger steady-state entanglement when coupled to fermion baths exchanging particles with the system than boson baths exchanging energy with the system, under similar conditions. We also identify a close connection between the energy current flowing through the system and the steady-state coherence. Preliminary investigations suggest that these results are insensitive to the form of the reservoir spectral densities in the Markovian regime. Feasible experimental realization of measuring the steady-state entanglement and coherence is discussed for the coupled qubit system in nonequilibrium environments. Our findings offer some general guidelines for optimizing the steady-state entanglement and coherence in the coupled qubit system and may find potential applications in quantum information technology.
We derive a non-Markovian master equation for the evolution of a class of open quantum systems consisting of quadratic fermionic systems coupled to wideband reservoirs. This is done by providing an explicit correspondence between master equations and nonequilibrium Green's function approaches. Our findings permit us to address non-Markovian regimes characterized by negative decoherence rates and to characterize the dynamics with respect to a recently proposed measurement of ``non-Markovianity.'' We study the real-time dynamics and the steady-state solution of two illustrative models: a tight-binding electronic model and XY\mathit{XY}XY spin chains. The rich set of nonequilibrium steady-state phases encountered extends previous results to the non-Markovian regime.