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arXiv:2502.11623 · APL Photonics

An ultra-compact deterministic source of maximally entangled photon pairs

M. Langer, Pavel Ruchka, A. Rahimi, Sara Jakovljevic, Yared G. Zena, Sai Abhishikth Dhurjati, A. Danilov, Mandira Pal, Riccardo Bassoli, Frank H. P. Fitzek, Oliver G. Schmidt, Harald W. Giessen, Caspar Hopfmann

Published Jun 1, 2025• 8 citations
arXivHTMLPDF

Abstract

We demonstrate an ultra-compact source of on-demand, maximally entangled photon pairs using single GaAs quantum dots embedded in monolithic microlenses coupled to a lensed single-mode fiber. A 3D-printed micro-objective with a numerical aperture of 0.6 enables efficient fiber coupling and near-diffraction-limited performance with 604(16) nm resolution directly in the cryogenic environment at 3.8 K. The system achieves high single-photon emission rates [392(20) kHz] and purities [99.2(5)%] using two-photon resonant excitation. Leveraging the exciton–biexciton cascade, it produces near-maximally entangled photon pairs with peak entanglement negativities of 2n = 0.96 ± 0.02. The presented quantum light source combines state-of-the-art performance and long-term stability with a dramatically reduced system footprint, making it well-suited for seamless industrial integration.

DOI
10.1063/5.0271023

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We demonstrate an ultra-compact source of on-demand, maximally entangled photon pairs using single GaAs quantum dots embedded in monolithic microlenses coupled to a lensed single-mode fiber. A 3D-printed micro-objective with a numerical aperture of 0.6 enables efficient fiber coupling and near-diffraction-limited performance with 604(16) nm resolution directly in the cryogenic environment at 3.8 K. The system achieves high single-photon emission rates [392(20) kHz] and purities [99.2(5)%] using two-photon resonant excitation. Leveraging the exciton–biexciton cascade, it produces near-maximally entangled photon pairs with peak entanglement negativities of 2n = 0.96 ± 0.02. The presented quantum light source combines state-of-the-art performance and long-term stability with a dramatically reduced system footprint, making it well-suited for seamless industrial integration.
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Abstract In this work, we present a stand-alone and fiber-coupled quantum-light source. The plug-and-play device is based on an optically driven quantum dot delivering single photons via an optical fiber. The quantum dot is deterministically integrated in a monolithic microlens which is precisely coupled to the core of an optical fiber via active optical alignment and epoxide adhesive bonding. The rigidly coupled fiber-emitter assembly is integrated in a compact Stirling cryocooler with a base temperature of 35 K. We benchmark our practical quantum device via photon auto-correlation measurements revealing g(2)(0) = 0.07 ± 0.05 under continuous-wave excitation and we demonstrate triggered non-classical light at a repetition rate of 80 MHz. The long-term stability of our quantum light source is evaluated by endurance tests showing that the fiber-coupled quantum dot emission is stable within 4% over several successive cool-down/warm-up cycles. Additionally, we demonstrate non-classical photon emission for a user-intervention-free 100-hour test run and stable single-photon count rates up to 11.7 kHz with a standard deviation of 4%.
Entangled photon generation from semiconductor quantum dots via the biexciton-exciton cascade underlies various decoherence mechanisms related to the solid-state nature of the quantum emitters. So far, this has prevented the demonstration of nearly-maximally entangled photons without the aid of inefficient and complex post-selection techniques that are hardly suitable for quantum communication technologies. Here, we tackle this challenge using strain-tunable GaAs quantum dots driven under two-photon resonant excitation and with strictly-degenerate exciton states. We demonstrate experimentally that our on-demand source generates polarization-entangled photons with fidelity of 0.978(5) and concurrence of 0.97(1) without resorting to post-selection techniques. Moreover, we show that the remaining decoherence mechanisms can be overcome using a modest Purcell enhancement so as to achieve a degree of entanglement >0.99. Our results highlight that GaAs quantum dots can be readily used in advanced communication protocols relying on the non-local properties of quantum entanglement.
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We demonstrate the on-demand emission of polarisation-entangled photon pairs from the biexciton cascade of a single InAs quantum dot embedded in a GaAs/AlAs planar microcavity. Improvements in the sample design blue shifts the wetting layer to reduce the contribution of background light in the measurements. Results presented show that >70% of the detected photon pairs are entangled. The high fidelity of the (|HxxHx>+|VxxVx>)/2^0.5 state that we determine is sufficient to satisfy numerous tests for entanglement. The improved quality of entanglement represents a significant step towards the realisation of a practical quantum dot source compatible with applications in quantum information.
We report on two-photon interference (TPI) experiments using remote deterministic single-photon sources. Employing 3D in-situ electron-beam lithography, we fabricate quantum-light sources at specific target wavelengths by integrating pre-selected semiconductor quantum dots within monolithic microlenses. The individual single-photon sources show TPI visibilities of 49% and 22%, respectively, under pulsed p-shell excitation at 80 MHz. For the mutual TPI of the remote sources, we observe an uncorrected visibility of 29%, in quantitative agreement with the pure dephasing of the individual sources. Due to its efficient photon extraction within a broad spectral range (>20 nm), our microlens-based approach is predestinated for future entanglement swapping experiments utilizing entangled photon pairs emitted by distant biexciton-exciton radiative cascades.