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arXiv:2502.09930 · npj Quantum Information

Long-lived photon blockade with weak optical nonlinearity

You Wang, Zheng Gang Xu, T. C. H. Liew, Y. D. Chong

Published Jun 20, 2026• 2 citations
arXivHTMLPDF

Abstract

Abstract In conventional photon blockade, the occupation of a cavity mode by more than one photon is suppressed via strong optical nonlinearity. An alternative, called unconventional photon blockade, can occur under weak nonlinearity by relying on quantum interference between fine-tuned cavities. A serious limitation to this approach is the very short antibunching time window, orders of magnitude less than the cavity lifetime. We present a scheme to achieve photon blockade over a large time window of several cavity lifetimes, even exceeding that of conventional photon blockade, while still requiring only weak nonlinearity. This “long-lived photon blockade” (LLPB) occurs when the single-particle Green’s function exhibits a zero at a large cavity loss rate, which is satisfied by an exemplary configuration of four coupled cavities under weak driving. Our analytical results agree well with wavefunction Monte Carlo simulations. The LLPB phenomenon may aid the development of single-photon sources utilizing materials with weak optical nonlinearities.

DOI
10.1038/s41534-026-01293-0

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Abstract In conventional photon blockade, the occupation of a cavity mode by more than one photon is suppressed via strong optical nonlinearity. An alternative, called unconventional photon blockade, can occur under weak nonlinearity by relying on quantum interference between fine-tuned cavities. A serious limitation to this approach is the very short antibunching time window, orders of magnitude less than the cavity lifetime. We present a scheme to achieve photon blockade over a large time window of several cavity lifetimes, even exceeding that of conventional photon blockade, while still requiring only weak nonlinearity. This “long-lived photon blockade” (LLPB) occurs when the single-particle Green’s function exhibits a zero at a large cavity loss rate, which is satisfied by an exemplary configuration of four coupled cavities under weak driving. Our analytical results agree well with wavefunction Monte Carlo simulations. The LLPB phenomenon may aid the development of single-photon sources utilizing materials with weak optical nonlinearities.
The photon blockade based on weak nonlinearities is called the unconventional photon blockade. The study of the unconventional photon blockade in recent decades has mainly focused on the ${\ensuremath{\chi}}^{(3)}$ Kerr nonlinearity. In this paper, we study the photon blockade in two weakly coupled nonlinear cavities via ${\ensuremath{\chi}}^{(2)}$ nonlinearity, where ${\ensuremath{\chi}}^{(2)}$ mediates the conversion of a single photon in the cavity with high frequency into two photons with low frequency in another cavity. When the two cavity modes are driven simultaneously, our calculations show that the strong photon antibunching can be obtained in the cavity. The optimal condition for strong antibunching is found by analytic calculations and numerical simulations, and discussions of the optimal condition are presented. The differences between the present scheme and that with ${\ensuremath{\chi}}^{(3)}$ nonlinearity are discussed. This scheme is not sensitive to the change of decay rates, which makes the experimental realization easy.
In this paper, we show that photon blockade can be observed in a system with weak Kerr nonlinearities. The system consists of two spatially overlapping single-mode semiconductor cavities with tunable one- and two-photon tunneling. We find that both conventional and unconventional single-photon blockades are controllable by manipulating the phase in the hopping regardless of the weakness of nonlinearity. We refer to the photon blockade with weak nonlinearities as an unconventional photon blockade. The unconventional photon blockade effect originates from the destructive interference between different paths from the ground state to two-photon states. We analytically derive the exact optimal conditions for strong antibunching, which are in good agreement with those obtained by numerical simulations. The optimal parameters for photon blockade are derived. Based on these parameters, the semiconductor cavity systems can be used as a single-photon source in regimes of both weak and strong nonlinearities.
Photon blockades are traditionally classified into conventional and unconventional types, depending on distinct physical mechanisms. Regarding the cavity decay rate κ, the conventional photon blockade takes place under strong nonlinearity condition (g>κ), whereas the unconventional photon blockade occurs in the regime of weak nonlinearity (g<κ). We here propose how to derive an optimal condition for photon blockade utilizing a two-photon Jaynes-Cummings model. Under this condition, the equal-time second-order correlation function reaches its minimum, leading to photon antibunching in both conventional and unconventional photon blockade regimes (g>κ and g<κ), even in g∼κ. This characteristic is termed universal photon blockade. By comparing it with the conventional and the unconventional photon blockades in the weak-driving limit, the advantages of universal photon blockade are revealed. Our proposal paves an avenue towards the future study of photon blockades and has potential applications in generating antibunched photons.
The photon blockade based on weak nonlinearities is called unconventional photon blockade. The studies of the unconventional photon blockade in recent decades are all limited to Markovian approximation. In this paper, we propose a scheme to achieve a strong photon antibunching in non-Markovian reservoir. An exact non-Markovian master equation for the optical cavity coupled with a degenerate optical parametric amplifier (DOPA) is derived. We show that this unconventional photon blockade originates from the destructive interference between two paths which are formed by the DOPA pump and a driving field. Unconventional single-photon blockades that exhibit a transition from the non-Markovian to Markovian regime by controlling environmental spectral width regardless of the weakness of DOPA gain and driving field are found. We analytically derive an optimal condition for strong antibunching, which is in good agreement with that obtained by the full numerical simulation. The presented results then are compared with that given by Markovian approximation in the weak-coupling limit. Our scheme might have paved an avenue towards the investigations of unconventional photon blockades in many other non-Markovian quantum systems in quantum optics.
We propose a scheme of photon blockade in a system comprising of coupled cavities embedded in Kerr nonlinear material, where two cavities are driven and dissipated. We analytically derive the exact optimal conditions for strong photon antibunching, which are in good agreement with those obtained by numerical simulations. We find that conventional and unconventional photon blockades have controllable flexibilities by tuning the strength ratio and relative phase between two complex driving fields. Such unconventional photon-blockade effects are ascribed to the quantum interference effect to avoid two-photon excitation of the coupled cavities. We also discuss the statistical properties of the photons under given optimal conditions. Our results provide a promising platform for the coherent manipulation of photon blockade, which has potential applications for quantum information processing and quantum optical devices.
Abstract The unconventional photon blockade, which relies on the physical mechanism of quantum interference, is primarily investigated using a general master equation, where a weak nonlinearity must be presented in the system to achieve photon antibunching. In this study, we explore the unconventional photon blockade using an alternative master equation known as the two-photon absorption master equation, which is derived from the system and environment interaction via two-photon absorption. Specifically, we find that the unconventional photon blockade can be triggered in two-coupled cavities, where each cavity interacts with a two-photon absorption environment. Different from unconventional photon blockade via the general master equation, we show that the two-photon absorption acts as the weak nonlinearity, and this photon blockade corresponds to a large average photon number. To derive optimal conditions for achieving this blockade, we propose a non-Hermitian Hamiltonian method to describe the mode loss caused by the two-photon absorption. In addition, we highlight the distinctions between our proposal and other approaches for generating single-photon states based on two-photon absorption.