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arXiv:2502.09068 · Applied Physics Letters

Efficient quantum frequency conversion of ultra-violet single photons from a trapped ytterbium ion

Seungwoo Yu, Kyungmin Lee, Sumin Park, Kyunghye Kim, Junhong Goo, Jeonghyun Park, Taehyun Kim

Published Feb 24, 2025• 3 citations
arXivHTMLPDF

Abstract

Ion trap system is a leading candidate for quantum information science benefitting from its long coherence time, high-fidelity gate operations. In addition, the ion photon entanglement provides a versatile tool to realize quantum networks by generating an ideal pair of a stationary memory qubit and a flying communication qubit. Rapid developments in nonlinear quantum frequency conversion techniques have enhanced the potential for constructing a trapped ion quantum network via optical fiber connections. The generation of long-distance entanglement has been demonstrated with ions such as Ca+ and Ba+, which emit photons in visible or near-infrared range naturally. On the other hand, as the qubit-native photons reside in ultra-violet (UV) spectrum, the Yb+ ion has not been considered as a strong competitor for telecommunication qubits despite extensive research on it. Here, we demonstrate an efficient difference-frequency conversion of UV photons, emitted from a trapped Yb+ ion, into a visible range. We provide experimental evidence that confirms the converted photons are radiated from the Yb+ ion. Our results provide a crucial step toward realizing a long-distance trapped ion quantum network based on Yb+ ions through quantum frequency conversion.

DOI
10.1063/5.0241469

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Ion trap system is a leading candidate for quantum information science benefitting from its long coherence time, high-fidelity gate operations. In addition, the ion photon entanglement provides a versatile tool to realize quantum networks by generating an ideal pair of a stationary memory qubit and a flying communication qubit. Rapid developments in nonlinear quantum frequency conversion techniques have enhanced the potential for constructing a trapped ion quantum network via optical fiber connections. The generation of long-distance entanglement has been demonstrated with ions such as Ca+ and Ba+, which emit photons in visible or near-infrared range naturally. On the other hand, as the qubit-native photons reside in ultra-violet (UV) spectrum, the Yb+ ion has not been considered as a strong competitor for telecommunication qubits despite extensive research on it. Here, we demonstrate an efficient difference-frequency conversion of UV photons, emitted from a trapped Yb+ ion, into a visible range. We provide experimental evidence that confirms the converted photons are radiated from the Yb+ ion. Our results provide a crucial step toward realizing a long-distance trapped ion quantum network based on Yb+ ions through quantum frequency conversion.
Generating entangled states of quantum memories over a long distance is an essential component for scalable quantum communication and its application such as quantum key distribution. Generation of entangled ion pairs mediated by photonic qubits has been demonstrated with trapped ytterbium (Yb) ions [1] and is a promising approach. However the wavelength of a single photon emitted by most trapped ions is in the ultraviolet (UV) or short-wavelength visible range where the maximum distribution distance of the photons is severely limited due to high absorption coefficient in a single mode optical fiber. To overcome this limitation, we are currently developing a frequency down-conversion scheme [2,3] which can coherently transfer a qubit stored in a 370 nm photon emitted by a Yb ion to another photon at 1310 nm which coincides with the low loss window of a telecom fiber.
Fiber-based quantum networks require photons at telecommunications wavelengths to interconnect qubits separated by long distances. Trapped ions are leading candidates for quantum networking with high-fidelity two-qubit gates, long coherence times, and the ability to readily emit photons entangled with the ion's internal qubit states. However, trapped ions typically emit photons at wavelengths incompatible with telecommunications fiber. Here, we demonstrate frequency conversion of visible photons, emitted from the S–P dipole transition of a trapped Ba+ ion into the telecommunications C-band. These results are an important step toward enabling a long-distance trapped ion quantum internet.
Trapped ions are excellent candidates for quantum nodes, as they possess many desirable features of a network node including long lifetimes, on-site processing capability, and production of photonic flying qubits. However, unlike classical networks in which data may be transmitted in optical fibers and where the range of communication is readily extended with amplifiers, quantum systems often emit photons that have a limited propagation range in optical fibers and, by virtue of the nature of a quantum state, cannot be noiselessly amplified. Here, we first describe a method to extract flying qubits from a Ba+ trapped ion via shelving to a long-lived, low-lying D-state with higher entanglement probabilities compared with current strong and weak excitation methods. We show a projected fidelity of ≈89% of the ion–photon entanglement. We compare several methods of ion–photon entanglement generation, and we show how the fidelity and entanglement probability varies as a function of the photon collection optic’s numerical aperture. We then outline an approach for quantum frequency conversion of the photons emitted by the Ba+ ion to the telecommunication range for long-distance networking and to 780 nm for potential entanglement with rubidium-based quantum memories. Our approach is significant for extending the range of quantum networks and for the development of hybrid quantum networks compromised of different types of quantum memories.
Trapped ions are one of the leading candidates for scalable and long-distance quantum networks because of their long qubit coherence time, high-fidelity single- and two-qubit gates, and their ability to generate photons entangled with the qubit state of the ion. One method for creating ion-photon entanglement is to exploit optical transitions from the 6 P 1/2 to 6 S 1/2 levels, which naturally emit spin-photon entangled states. But these optical transitions typically lie in the ultraviolet and visible wavelength regions of the spectrum. These wavelengths exhibit significant fiber-optic propagation loss, thereby limiting the transfer of quantum information to tens of meters. Quantum frequency conversion is essential to convert these photons to telecom wavelengths so that they can propagate over long distances in fiber-based networks, as well as for compatibility with the vast number of telecom-based optoelectronic components. Here, we generate O-band telecom photons via a low-noise quantum frequency conversion scheme from photons emitted from the 6 P 1/2 to 6 S 1/2 dipole transition of a trapped barium ion. We use a two-stage quantum frequency conversion scheme to achieve a frequency shift of 375.4 THz between the input visible photon and the output telecom photon, achieving a conversion efficiency of 11%. We attain a signal-to-background ratio of over 100 for the converted O-band telecom photon with background noise of less than 15 counts/s. These results are an important step toward achieving trapped ion quantum networks over long distances for distributed quantum computing and quantum communication.
Efficiently scaling quantum networks to long ranges requires local processing nodes to perform basic computation and communication tasks. Trapped ions have demonstrated all the properties required for the construction of such a node, storing quantum information for up to 12 min, implementing deterministic high fidelity logic operations on one and two qubits, and ion–photon coupling. While most ions suitable for quantum computing emit photons in visible to near ultraviolet (UV) frequency ranges poorly suited to long-distance fibre optical based networking, recent experiments in frequency conversion provide a technological solution by shifting the photons to frequencies in the telecom band with lower attenuation for fused silica fibres. Encoding qubits in frequency rather than polarization makes them more robust against decoherence from thermal or mechanical noise due to the conservation of energy. To date, ion–photonic frequency qubit entanglement has not been directly shown. Here we demonstrate a frequency encoding ion–photon entanglement protocol in 171 Yb + with correlations equivalent to 92.4(8)% fidelity using a purpose-built UV hyperfine spectrometer. The same robustness against decoherence precludes our passive optical setup from rotating photonic qubits to unconditionally demonstrate entanglement, however it is sufficient to allow us to benchmark the quality of ion–UV photon correlations prior to frequency conversion to the telecom band.
Abstract Entanglement between a stationary quantum system and a flying qubit is an essential ingredient of a quantum-repeater network. It has been demonstrated for trapped ions, trapped atoms, color centers in diamond, or quantum dots. These systems have transition wavelengths in the blue, red or near-infrared spectral regions, whereas long-range fiber-communication requires wavelengths in the low-loss, low-dispersion telecom regime. A proven tool to interconnect flying qubits at visible/NIR wavelengths to the telecom bands is quantum frequency conversion. Here we use an efficient polarization-preserving frequency converter connecting 854 nm to the telecom O-band at 1310 nm to demonstrate entanglement between a trapped 40Ca+ ion and the polarization state of a telecom photon with a high fidelity of 98.2 ± 0.2%. The unique combination of 99.75 ± 0.18% process fidelity in the polarization-state conversion, 26.5% external frequency conversion efficiency and only 11.4 photons/s conversion-induced unconditional background makes the converter a powerful ion–telecom quantum interface.