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arXiv:2502.01480

Two-particle quantum interference in a nonlinear optical medium: a witness of timelike indistinguishability

Chao Chen, Shu-Tian Xue, Shi, Yu-Peng, Wang, Jing, Zi-Mo Cheng, Wan, Pei, Zhi‐Cheng Ren, Michael G. Jabbour, Nicolas J. Cerf, Xi‐Lin Wang, Hui‐Tian Wang

Published Feb 3, 2025• 0 citations

Abstract

The Hong-Ou-Mandel effect is a paradigmatic quantum phenomenon demonstrating the interference of two indistinguishable photons that are linearly coupled at a 50:50 beam splitter. Here, we transpose such a two-particle quantum interference effect to the nonlinear regime, when two single photons are impinging on a parametric down-conversion crystal. Formally, this transposition amounts to exchanging space and time variables, giving rise to an unknown form of timelike quantum interference. The two-photon component of the output state is a superposition of the incident photons being either transmitted or reborn, that is, replaced by indistinguishable substitutes due to their interaction with the nonlinear crystal. We experimentally demonstrate the suppression of the probability of detecting precisely one photon pair when the amplification gain is tuned to 2, which arises from the destructive interference between the transmitted and reborn photon pairs. This heretofore unobserved quantum manifestation of indistinguishability in time pushes nonlinear quantum interference towards a new regime with multiple photons. Hence, composing this effect with larger linear optical circuits should provide a tool to generate multimode quantum non-Gaussian states, which are essential resources for photonic quantum computers.

DOI: 10.48550/arxiv.2502.01480

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The Hong-Ou-Mandel effect is a paradigmatic quantum phenomenon demonstrating the interference of two indistinguishable photons that are linearly coupled at a 50:50 beam splitter. Here, we transpose such a two-particle quantum interference effect to the nonlinear regime, when two single photons are impinging on a parametric down-conversion crystal. Formally, this transposition amounts to exchanging space and time variables, giving rise to an unknown form of timelike quantum interference. The two-photon component of the output state is a superposition of the incident photons being either transmitted or reborn, that is, replaced by indistinguishable substitutes due to their interaction with the nonlinear crystal. We experimentally demonstrate the suppression of the probability of detecting precisely one photon pair when the amplification gain is tuned to 2, which arises from the destructive interference between the transmitted and reborn photon pairs. This heretofore unobserved quantum manifestation of indistinguishability in time pushes nonlinear quantum interference towards a new regime with multiple photons. Hence, composing this effect with larger linear optical circuits should provide a tool to generate multimode quantum non-Gaussian states, which are essential resources for photonic quantum computers.

The celebrated Hong-Ou-Mandel effect is the paradigm of two-particle quantum interference. It has its roots in the symmetry of identical quantum particles, as dictated by the Pauli principle. Two identical bosons impinging on a beam splitter (of transmittance 1/2) cannot be detected in coincidence at both output ports, as confirmed in numerous experiments with light or even matter. Here, we establish that partial time reversal transforms the beam splitter linear coupling into amplification. We infer from this duality the existence of an unsuspected two-boson interferometric effect in a quantum amplifier (of gain 2) and identify the underlying mechanism as time-like indistinguishability. This fundamental mechanism is generic to any bosonic Bogoliubov transformation, so we anticipate wide implications in quantum physics.

Two-photon interference effects arise because photons are indistinguishable particles. In the wellknown Hong-Ou-Mandel (HOM) effect, the transmission of two photons at a beam splitter interferes destructively with the reflection of both photons, requiring both photons to "bunch up" by leaving the beam splitter on the same side. Here, we show that the interference between locally propagating photons and photons exchanged by a mode swap can be implemented by post-selecting spatially separated photon outputs of a four-path interferometer. Even though the photons detected at spatially separated locations must have travelled along paths that never met up at the same beam splitter, the Hong-Ou-Mandel effect can be observed in correlations between the output ports that originate from the association of detection events with non-local output modes defined by the two single photon inputs. Local phase shifts can be used to map out non-classical correlations between the photons detected at different output locations, clarifying the role of linear optics in generating entanglement between spatially separated photons. Our work thus establishes a fundamental relation between multiphoton interference and entanglement, opening the door to new possibilities in optical quantum technologies.

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The bunching of two single photons on a beam splitter is a fundamental quantum effect, first observed by Hong, Ou, and Mandel. It is a unique interference effect that relies only on the photons' indistinguishability and not on their relative phase. We generalize this effect by demonstrating the bunching of two Bell states, created in two passes of a nonlinear crystal, each composed of two photons. When the two Bell states are indistinguishable, phase-insensitive destructive interference prevents the outcome of fourfold coincidence between the four spatial-polarization modes. For certain combinations of the two Bell states, we demonstrate the opposite effect of antibunching. We relate this result to the number of distinguishable modes in parametric down-conversion.

The two-photon Hong-Ou-Mandel (HOM) interference is a pure quantum effect which indicates the degree of indistinguishability of photons. The four-photon HOM interference exhibits richer dynamics in comparison to the two-photon interference and simultaneously is more sensitive to the input photon states. We demonstrate theoretically and experimentally an explicit dependency of the four-photon interference on the number of temporal modes, created in the process of parametric down-conversion. Moreover, we exploit the splitting ratio of the beam splitter to manipulate the interference between bunching and antibunching. Our results reveal that the temporal mode structure (multimodeness) of the quantum states shapes many-particle interference.

The bunching of two single photons on a beam-splitter is a fundamental quantum effect, first observed by Hong, Ou and Mandel. It is a unique interference effect that relies only on the photons' indistinguishability and not on their relative phase. We generalize this effect by demonstrating the bunching of two Bell states, created in two passes of a nonlinear crystal, each composed of two photons. When the two Bell states are indistinguishable, phase insensitive destructive interference prevents the outcome of four-fold coincidence between the four spatial-polarization modes. For certain combinations of the two Bell states, we demonstrate the opposite effect of anti-bunching. We relate this result to the number of distinguishable modes in parametric down-conversion.