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arXiv:2501.08917 · Physical Review Research

Spectral and temporal properties of type-II parametric down-conversion: The impact of losses during state generation

Denis A. Kopylov, Michael Stefszky, Torsten Meier, Christine Silberhorn, Polina R. Sharapova

Published Jun 18, 2025• 4 citations
arXivHTMLPDF

Abstract

In this paper, we theoretically study the spectral and temporal properties of pulsed spontaneous parametric down-conversion (SPDC) generated in lossy waveguides. Our theoretical approach is based on the formalism of Gaussian states and the Langevin equation, which is elaborated for weak parametric down-conversion and photon-number-unresolved click detection. Using the example of frequency-degenerate type-II SPDC generated under the pump-idler group-velocity-matching condition, we show how the joint-spectral intensity, mode structure, normalized second-order correlation function, and Hong-Ou-Mandel interference pattern depend on internal losses of the SPDC process. We found that the joint-spectral intensity is almost insensitive to internal losses, while the second-order correlation function shows a strong dependence on them, being different for the signal and idler beams in the presence of internal losses. Based on the sensitivity of the normalized second-order correlation function, we show how its measurement can be used to experimentally determine internal losses.

DOI
10.1103/zp72-7qwl

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In this paper, we theoretically study the spectral and temporal properties of pulsed spontaneous parametric down-conversion (SPDC) generated in lossy waveguides. Our theoretical approach is based on the formalism of Gaussian states and the Langevin equation, which is elaborated for weak parametric down-conversion and photon-number-unresolved click detection. Using the example of frequency-degenerate type-II SPDC generated under the pump-idler group-velocity-matching condition, we show how the joint-spectral intensity, mode structure, normalized second-order correlation function, and Hong-Ou-Mandel interference pattern depend on internal losses of the SPDC process. We found that the joint-spectral intensity is almost insensitive to internal losses, while the second-order correlation function shows a strong dependence on them, being different for the signal and idler beams in the presence of internal losses. Based on the sensitivity of the normalized second-order correlation function, we show how its measurement can be used to experimentally determine internal losses.
Parametric down-conversion (PDC) is mostly known in the low-gain (spontaneous) regime, in which the correlated photon pairs are produced. Spontaneous PDC (SPDC) plays a very important role for quantum optics as a variety of quantum states is produced via SPDC. In the high-gain case PDC leads to generation of bright states having up to hundreds mW mean power. With such states almost any nonlinear optical interaction or light-matter interaction becomes more efficient. Even being macroscopically bright, the produced states maintain nonclassical properties as, for example, the fluctuations of electric field quadratures are squeezed below the shot-noise level. The high-gain PDC could be used not only in the same applications as SPDC, it also can provide new ones. Apart from that the high-gain PDC has many remarkable spectral and statistical properties, which are in the focus of this work. The description starts from the PDC generation in normal and anomalous group velocity dispersion ranges. The spectrum and mode content of high-gain PDC is considered as well as their change with the parametric gain are demonstrated. Then, there are the interference effects emerging from the PDC correlations presented, namely the macroscopic analogue of the Hong-Ou-Mandel interference. In addition, it is shown how spatial and temporal walk-off matching could be used for the generation of giant narrowband twin beams. Finally, the statistical properties of high-gain PDC are reviewed as well as their use for multiphoton effects is demonstrated. Photon-number fluctuations of PDC are studied via normalized correlation functions and probability distributions. These fluctuations enhance the generation efficiency for multiphoton effects by orders of magnitude and lead to tremendously fluctuating light described by heavy-tailed photon-number probability distributions.
We derive frequency correlation and exit probability expressions for photons generated via spontaneous parametric downconversion (SPDC) in nonlinear waveguides that exhibit linear scattering loss.Such loss is included within a general Hamiltonian formalism by connecting waveguide modes to reservoir modes with a phenomenological coupling Hamiltonian, the parameters of which are later related to the usual loss coefficients.In the limit of a low probability of SPDC pair production, the presence of loss requires that we write the usual lossless generated pair state as a reduced density operator, and we find that this density operator is naturally composed of two photon, one photon, and zero photon contributions.The biphoton probability density, or joint spectral intensity (JSI), associated with the two-photon contribution is determined not only by a phase matching term, but also by a loss matching term.The relative sizes of the loss coefficients within this term lead to three qualitatively different regimes of SPDC JSIs.If either the pump or generated photon loss is much higher than the other, the side lobes of the phase matching squared sinc function are washed out.On the other hand, if pump and generated photon loss are appropriately balanced, the lossy JSI is identical to the lossless JSI.Finally, if the generated photon loss is frequency dependent, the shape of the JSI can be altered more severely, potentially leading to generated photons that are less frequency correlated though also produced less efficiently when compared to photons generated in low-loss waveguides.
Photon sources based on spontaneous parametric down-conversion (SPDC) are central to experimental quantum optics and quantum technologies. Their performance is commonly quantified by three metrics: pair-collection probability, heralding efficiency, and spectral purity. In bulk-crystal SPDC, these metrics are known to be mutually constrained, yet the physical origin of the resulting trade-offs is often obscured. We show that these trade-offs originate from the frequency-dependent population of discrete spatial modes in the SPDC emission. By performing a Laguerre-Gauss mode decomposition at each frequency component, we show how spectral-spatial non-separability impacts collection probability, heralding efficiency, and purity. We apply this framework to two widely used quasi-phase-matching configurations: collinear degenerate type-0 and type-II SPDC in periodically poled bulk crystals, and quantify how different phase-matching functions shape the spectral-spatial mode structure. In particular, for type-II SPDC we compare standard periodically poled and aperiodically poled Gaussian phase matching. We experimentally validate some of our theoretical results using spatial- and spectral-projection measurements. This spectral-spatial mode analysis provides a quantitative and predictive framework for understanding and engineering bulk-crystal photon sources, enabling systematic multi-parameter optimization beyond qualitative design guidelines.
Spontaneous parametric down-conversion (SPDC) is the most often used source of entangled photon states in quantum optics. Recently, it has been suggested in theory that the reduction of polarization entanglement between the photon pair generated via the type-II SPDC process pumped by a ultrafast laser is due to the asymmetry in the joint spectrum function, which is the indicative of the frequency entanglement between the two photons. In this paper, we report the measurement of the joint spectrum function (i.e., direct observation of the degree of frequency entanglement) of the two-photon state of type-II SPDC in both cw- and ultrafast-laser pumping conditions. We observed that, in agreement with the theory, the degree of frequency entanglement (the shape of the joint spectrum function) is indeed different for cw- and ultrafast-pumped type-II SPDC. Our results are of importance in "engineering" the two-photon state for specific quantum applications, such as quantum cryptography.
Spectral properties of entangled photons generated via type-I frequency-nondegenerate spontaneous parametric down-conversion are studied theoretically and experimentally. For monochromatic pumping, the joint spectral intensity function for the photon pair is found to be symmetric even though each photon has a different central wavelength. The single-photon (first-order) interference shows the familiar triangular interferogram, usually associated with the cw-pumped frequency-degenerate type-II spontaneous parametric down-conversion. For broadband (ultrafast) pumping, on the other hand, the joint spectral intensity function is shown to be asymmetric, similar to the case of ultrafast-pumped frequency-degenerate type-II spontaneous parametric down-conversion. The spectral studies reported here are expected to play an important role in developing ultrabright two-color entangled photon sources.