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arXiv:2501.03661 · Nature Communications

Spin environment of a superconducting qubit in high magnetic fields

Simon Günzler, J. Beck, D. Rieger, Nicolas Gosling, Nicolas Zapata, M. E. Field, Simon Geisert, A. Bacher, Jens Hohmann, Martin Spiecker, Wolfgang Wernsdorfer, Ioan M. Pop

Published Oct 29, 2025• 9 citations
arXivHTMLPDF

Abstract

Superconducting qubits equipped with quantum non-demolition readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a challenge for superconductors and Josephson junctions. Here we demonstrate a granular aluminum nanojunction fluxonium qubit (gralmonium) with spectrum and coherence resilient to fields beyond one Tesla. Sweeping the field reveals a paramagnetic spin-1/2 ensemble, which is the dominant gralmonium loss mechanism when the electron spin resonance matches the qubit. We also observe a suppression of MHz range fast flux noise in magnetic field, suggesting the freezing of surface spins. Using an active state stabilization sequence, the qubit hyperpolarizes long-lived two-level systems (TLSs) in its environment, previously speculated to be spins. Surprisingly, the coupling to these TLSs is unaffected by magnetic fields, leaving the question of their origin open. The robust operation of gralmoniums in Tesla fields offers new opportunities to explore unresolved questions in spin environment dynamics and facilitates hybrid architectures linking superconducting qubits with spin systems.

DOI
10.1038/s41467-025-65528-y

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Superconducting qubits equipped with quantum non-demolition readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a challenge for superconductors and Josephson junctions. Here we demonstrate a granular aluminum nanojunction fluxonium qubit (gralmonium) with spectrum and coherence resilient to fields beyond one Tesla. Sweeping the field reveals a paramagnetic spin-1/2 ensemble, which is the dominant gralmonium loss mechanism when the electron spin resonance matches the qubit. We also observe a suppression of MHz range fast flux noise in magnetic field, suggesting the freezing of surface spins. Using an active state stabilization sequence, the qubit hyperpolarizes long-lived two-level systems (TLSs) in its environment, previously speculated to be spins. Surprisingly, the coupling to these TLSs is unaffected by magnetic fields, leaving the question of their origin open. The robust operation of gralmoniums in Tesla fields offers new opportunities to explore unresolved questions in spin environment dynamics and facilitates hybrid architectures linking superconducting qubits with spin systems.
Superconducting qubits equipped with quantum non-demolition readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a challenge for superconductors and Josephson junctions. Here we demonstrate a granular aluminum nanojunction fluxonium qubit (gralmonium) with spectrum and coherence resilient to fields beyond one Tesla. Sweeping the field reveals a paramagnetic spin-1/2 ensemble, which is the dominant gralmonium loss mechanism when the electron spin resonance matches the qubit. We also observe a suppression of MHz range fast flux noise in magnetic field, suggesting the freezing of surface spins. Using an active state stabilization sequence, the qubit hyperpolarizes long-lived two-level systems (TLSs) in its environment, previously speculated to be spins. Surprisingly, the coupling to these TLSs is unaffected by magnetic fields, leaving the question of their origin open. The robust operation of gralmoniums in Tesla fields offers new opportunities to explore unresolved questions in spin environment dynamics and facilitates hybrid architectures linking superconducting qubits with spin systems.
Understanding the microscopic environment of superconducting qubits is a central challenge for quantum technologies. Parasitic two-level systems (TLSs) of various microscopic origins are ubiquitous and limit qubit performance through decoherence, frequency drifts, and leakage. Recently, long-lived TLSs with lifetimes exceeding those of state-of-the-art qubits have been shown to induce correlated qubit dynamics, with direct implications for quantum error correction. Here, we perform wide-band quantum-jump correlation spectroscopy on flux-tunable transmon qubits and identify microscopic degrees of freedom that outlive the qubit by orders of magnitude. Pump-probe measurements at varying detunings from these objects reveal intrinsic lifetimes exceeding one second. Their weak coupling to the qubit, in the kilohertz range, is consistent with positional defects described by the standard tunneling model, without excluding other microscopic origins such as magnetic spin impurities or trapped quasiparticles. More broadly, these results establish superconducting qubits as a sensitive probe of exceptionally long-lived microscopic degrees of freedom and open a route toward their controlled access and functionalization.
The coherence of superconducting transmon qubits is often disrupted by fluctuations in the energy relaxation time (T1), limiting their performance for quantum computing. While background magnetic fields can be harmful to superconducting devices, we demonstrate that both trapped magnetic flux and externally applied static magnetic fields can suppress temporal fluctuations in T1 without significantly degrading its average value or qubit frequency. Using a three-axis Helmholtz coil system, we applied calibrated magnetic fields perpendicular to the qubit plane during cooldown and operation. Remarkably, transmon qubits based on tantalum-capped niobium (Nb/Ta) capacitive pads and aluminum-based Josephson junctions (JJs) maintained T1 lifetimes near 300 μs even when cooled in fields as high as 600 mG. Both trapped flux up to 600 mG and applied fields up to 400 mG reduced T1 fluctuations by more than a factor of two, while higher field strengths caused rapid coherence degradation. We attribute this stabilization to the polarization of paramagnetic impurities, the role of trapped flux as a sink for non-equilibrium quasiparticles (QPs), and partial saturation of fluctuating two-level systems (TLSs). These findings challenge the conventional view that magnetic fields are inherently detrimental and introduce a strategy for mitigating noise in superconducting qubits, offering a practical path toward more stable and scalable quantum systems.
A hybrid quantum computing architecture combining quantum processors and quantum memory units allows for exploiting each component's unique properties to enhance the overall performance of the total system. However, superconducting qubits are highly sensitive to magnetic fields, while spin ensembles require finite fields for control, creating a major integration challenge. In this work, we demonstrate the first experimental setup that satisfies these constraints and provides verified qubit stability. Our cryogenic setup comprises two spatially and magnetically decoupled sample volumes inside a single dilution refrigerator: one hosting flux-tunable superconducting qubits and the other a spin ensemble equipped with a superconducting solenoid generating fields up to 50 mT. We show that several layers of Cryophy shielding and an additional superconducting aluminum shield suppress magnetic crosstalk by more than eight orders of magnitude, ensuring stability of the qubit's performance. Moreover, the operation of the solenoid adds minimal thermal load on the relevant stages of the dilution refrigerator. Our results enable scalable hybrid quantum architectures with low-loss integration, marking a key step toward scalable hybrid quantum computing platforms.
Hybrid superconducting circuits have been used to investigate mesoscopic superconductivity, but mostly just at low magnetic fields, as typical Al-based circuits are incompatible with magnetic fields, and superconducting circuits are sensitive to external magnetic flux noise. To overcome these challenges, the authors build a hybrid fluxonium system composed of (Nb,Ti)N, with a gradiometric design. They observe the spectrum of the hybrid fluxonium in fields of up to 1T, and probe the ${\ensuremath{\phi}}_{0}$ Josephson effect. These results enable future exploration of topological superconductivity, as well as readout of long-lifetime spin-polarized qubits using superconducting circuitry.
Altermagnets, characterized by vanishing net magnetization and momentum-dependent spin splitting, provide a promising platform for next-generation Josephson devices. Here, we exploit the Josephson effect in superconductor-altermagnet-superconductor junctions and show how to engineer prescribed current-phase relations by device design. Based on these programmable Josephson potentials utilizing altermagnetism, we propose a new class of superconducting qubits that combine large anharmonicity with enhanced robustness against decoherence via coherent two-Cooper-pair tunneling. We show that in the 2φ2φ2φ-junction regime, this kind of qubit is intrinsically protected against both charge and flux noise due to parity protection. Magnetic flux can be used to precisely control the qubit and, under appropriate bias, this architecture further suppresses charge and flux noise. Our results establish altermagnets as a versatile platform for Josephson-potential engineering and open a new route toward high-performance superconducting qubits combining high coherence, large anharmonicity, and broad tunability.