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arXiv:2501.02784 · Physical Review Letters

Overcoming Quantum Metrology Singularity through Sequential Measurements

Yaoling Yang, Víctor Montenegro, Abolfazl Bayat

Published May 27, 2025• 11 citations
arXivHTMLPDF

Abstract

The simultaneous estimation of multiple unknown parameters is the most general scenario in quantum sensing. Quantum multiparameter estimation theory provides fundamental bounds on the achievable precision of simultaneous estimation. However, these bounds can become singular (no finite bound exists) in multiparameter sensing due to parameter interdependencies, limited probe accessibility, and insufficient measurement outcomes. Here, we address the singularity issue in quantum sensing through a simple mechanism based on a sequential measurement strategy. This sensing scheme overcomes the singularity constraint and enables the simultaneous estimation of multiple parameters with a local and fixed measurement throughout the sensing protocol. This is because sequential measurements, involving consecutive steps of local measurements followed by probe evolution, inherently produce correlated measurement data that grows exponentially with the number of sequential measurements. Finally, through two different examples, namely a strongly correlated probe and a light-matter system, we demonstrate how such singularities are reflected when inferring the unknown parameters through Bayesian estimation.

DOI
10.1103/gsyv-jllq

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The simultaneous estimation of multiple unknown parameters is the most general scenario in quantum sensing. Quantum multiparameter estimation theory provides fundamental bounds on the achievable precision of simultaneous estimation. However, these bounds can become singular (no finite bound exists) in multiparameter sensing due to parameter interdependencies, limited probe accessibility, and insufficient measurement outcomes. Here, we address the singularity issue in quantum sensing through a simple mechanism based on a sequential measurement strategy. This sensing scheme overcomes the singularity constraint and enables the simultaneous estimation of multiple parameters with a local and fixed measurement throughout the sensing protocol. This is because sequential measurements, involving consecutive steps of local measurements followed by probe evolution, inherently produce correlated measurement data that grows exponentially with the number of sequential measurements. Finally, through two different examples, namely a strongly correlated probe and a light-matter system, we demonstrate how such singularities are reflected when inferring the unknown parameters through Bayesian estimation.
Estimating multiple unknown parameters simultaneously is essential for practical quantum sensing. However, it faces a fundamental challenge: the optimal strategy for estimating one parameter is often incompatible with that for another, making it impossible to simultaneously achieve the ultimate precision limits for all parameters. Here we develop a general and efficient computational framework that jointly optimizes probe states, control operations, and measurements across different strategy families, including parallel, sequential, and those with indefinite causal order. Our approach provides exact semidefinite-program formulations for several precision bounds, including the Holevo, Nagaoka-Hayashi, and quantum Cramér-Rao bounds. We demonstrate the capabilities of the framework in multiparameter magnetometry and frequency estimation, identifying optimal protocols within each class and revealing a strict hierarchy among the achievable performances of different classes in the multiparameter regime. The framework also directly incorporates resource constraints, such as energy budgets, enabling systematic investigation of experimentally realistic sensing scenarios. Furthermore, we develop a finite-memory optimization method for sequential strategies with restricted ancillary-memory dimension. By decomposing the protocol into initial probe preparation and intermediate control operations, this method provides a practical route to designing resource-constrained sequential sensing schemes. Our work establishes a versatile computational tool for determining fundamental precision limits and designing optimal quantum-sensing protocols in complex multiparameter settings.
The most general strategy for estimating parameters of a quantum channel is to probe the channel many times sequentially with the help of coherent ancillary systems. However, finding the strategy that minimizes the mean-squared error (MSE) is a notoriously hard problem, requiring optimization over the initial probe state, intermediate evolutions, final measurement, and classical postprocessing. In this work, we study how the minimum attainable MSE can be bounded from below in this setting. We propose a lower bound for the MSE of any physically implementable sequential sensing strategy that applies to estimating parameters of any physical quantum evolution, including quantum channels probed over multiple time steps under temporally correlated noise and general temporally correlated quantum processes. We show that this lower bound can be formulated as a semidefinite program (SDP). Our bound generalizes the Nagaoka-Hayashi lower bound (that applies to parameter estimation tasks with separable measurements) to the regime where the quantum channel can be accessed sequentially multiple times. For regular finite-dimensional single-parameter sequential estimation tasks admitting an optimal strategy, we show that our SDP bound is tight and provide a procedure to obtain a locally optimal strategy from the SDP optimizer. Using our optimization bound, we compute the MSE lower bound and derive new protocols for several other physically motivated problems including error-corrected quantum sensing under an unknown correlated noise model, multiparameter estimation, and estimation with qudit systems.
Conventional multiparameter quantum sensing relies on joint estimation, but this approach faces two key limitations: theoretical bounds may be unattainable due to measurement incompatibility, and sensing may fail due to parameter interdependencies. We propose stepwise estimation and identify regimes where it outperforms joint estimation. For multiple quantum sensors, this scheme achieves far lower error bounds than joint estimation. With many-body probes, stepwise sensing retains a quantum-enhanced scaling advantage often lost in joint estimation due to parameter correlations. We demonstrate its concrete advantages through Bayesian implementations across diverse examples.
For single-parameter sensing, Greenberger-Horne-Zeilinger (GHZ) probes achieve optimal quantum-enhanced precision across the unknown parameter range, solely relying on parameter-independent separable measurement strategies for all values of the unknown parameter. However, in the multiparameter setting, a single GHZ probe not only fails to achieve quantum advantage but also the corresponding optimal measurement becomes complex and dependent on the unknown parameters. Here, we provide a recipe for multiparameter sensing with GHZ probes using quantum error correction techniques by treating all but one unknown parameters as noise, whose effects can be corrected. This strategy restores the core advantage of single parameter GHZ-based quantum sensing, namely reaching optimally quantum-enhanced precision for all unknown parameter values while keeping the measurements separable and fixed. Specifically, given one shielded ancilla qubit per GHZ probe, our protocol extracts optimal possible precision for any probe size. While this optimal precision is shot-noise limited for a single GHZ probe, we recover the Heisenberg scaling through use of multiple complementary GHZ probes. We demonstrate the effectiveness of the protocol with Bayesian estimation.
A longstanding problem in quantum metrology is how to extract as much information as possible in realistic scenarios with not only multiple unknown parameters, but also limited measurement data and some degree of prior information. Here we present a practical solution to this: We derive a Bayesian multi-parameter quantum bound, construct the optimal measurement when our bound can be saturated for a single shot, and consider experiments involving a repeated sequence of these measurements. Our method properly accounts for the number of measurements and the degree of prior information, and we illustrate our ideas with a qubit sensing network and a model for phase imaging, clarifying the nonasymptotic role of local and global schemes. Crucially, our technique is a powerful way of implementing quantum protocols in a wide range of practical scenarios that tools such as the Helstrom and Holevo Cram\'er-Rao bounds cannot normally access.
Abstract The theoretical foundation of quantum sensing is rooted in the Cramér–Rao formalism, which establishes quantitative precision bounds for a given quantum probe. In many practical scenarios, where more than one parameter is unknown, the multi-parameter Cramér–Rao bound (CRB) applies. Since this is a matrix inequality involving the inverse of the quantum Fisher information matrix (QFIM), the formalism breaks down when the QFIM is singular. In this paper, we examine the physical origins of such singularities, showing that they result from an over-parameterization on the metrological level. This is itself caused by emergent metrological symmetries , whereby the same set of measurement outcomes are obtained for different combinations of system parameters. Although the number of effective parameters is equal to the number of non-zero QFIM eigenvalues, the Cramér–Rao formalism typically does not provide information about the effective parameter encoding. Instead, we demonstrate through a series of concrete examples that Bayesian estimation can provide deep insights. In particular, the metrological symmetries appear in the Bayesian posterior distribution as lines of persistent likelihood running through the space of unknown parameters. These lines are contour lines of the effective parameters which, through suitable parameter transformations, can be estimated and follow their own effective CRBs.