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arXiv:2501.01891 · Optica Quantum

Two-cavity-mediated photon-pair emission by one atom

Gianvito Chiarella, Tobias Frank, Pau Farrera, Gerhard Rempe

Published Oct 15, 2024• 4 citations
arXivHTMLPDF

Abstract

Photon-pair sources are widely used in quantum optics and quantum information experiments. Despite their broad deployment, there has not yet been an on-demand implementation with efficient into-fiber photon generation and high single-photon purity. Here we report on such a source based on a single atom with three energy levels in ladder configuration and coupled to two optical fiber cavities. We efficiently generate photon pairs with an in-fiber emission efficiency of η pair =16(1)% and study their temporal correlation properties. We simulate theoretically a regime with strong atom–cavity coupling and find that photons are directly emitted from the ground state, i.e., without atomic population in any intermediate state. We propose a scenario to observe such a double-vacuum-stimulated effect experimentally.

DOI
10.1364/opticaq.529241

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Photon-pair sources are widely used in quantum optics and quantum information experiments. Despite their broad deployment, there has not yet been an on-demand implementation with efficient into-fiber photon generation and high single-photon purity. Here we report on such a source based on a single atom with three energy levels in ladder configuration and coupled to two optical fiber cavities. We efficiently generate photon pairs with an in-fiber emission efficiency of η pair =16(1)% and study their temporal correlation properties. We simulate theoretically a regime with strong atom–cavity coupling and find that photons are directly emitted from the ground state, i.e., without atomic population in any intermediate state. We propose a scenario to observe such a double-vacuum-stimulated effect experimentally.
A single atom strongly coupled to a high-finesse optical-cavity is a versatile tool for quantum information processing. Utilized as a single-photon source, it allows one to generate single photons very efficiently in a well defined spatio-temporal mode. In a first experiment, polarization-control over the photons is shown. A time-resolved two-photon interference experiment proves the indistinguishability of these photons - required in various quantum information processing schemes. Moreover, in a second experiment, entanglement between the polarization of the emitted photon and the population of the atomic Zeeman levels is created. Subsequent state mapping of the atomic state onto another photon results in a pair of polarization-entangled photons emitted one after the other from the cavity. Although these schemes are in principle possible in free space, the cavity boosts the efficiency by several orders of magnitude.
A single rubidium atom trapped within a high-finesse optical cavity is an efficient source of single photons. We theoretically and experimentally study single-photon generation using a vacuum stimulated Raman adiabatic passage. We experimentally achieve photon generation efficiencies of up to 34% and 56% on the D1{D}_{1}D1​ and D2{D}_{2}D2​ line, respectively. Output coupling with 89% results in record-high efficiencies for single photons in one spatiotemporally well-defined propagating mode. We demonstrate that the observed generation efficiencies are constant in a wide range of applied pump laser powers and virtual level detunings. This allows for independent control over the frequency and wave packet envelope of the photons without loss in efficiency. In combination with the long trapping time of the atom in the cavity, our system constitutes a significant advancement toward an on-demand, highly efficient single-photon source for quantum information processing tasks.
We describe a cavity-QED scheme to deterministically generate polarization entangled photon pairs by using a single atom successively coupled to two single longitudinal mode cavities presenting polarization degeneracy. The cavities are initially prepared either in the vacuum state or in a single photon Fock state for each orthogonal polarization. Sharing the same basic elements, the source can operate on different physical processes. For a V -type three-level atom initially prepared in the ground state two implementations of the source are possible using either: i) two truncated Rabi Oscillations, or ii) a counterintuitive Stimulated Raman Adiabatic Passage process. Although slower than the former implementation, this second one is very efficient and robust under fluctuations of the experimental parameters and, particularly interesting, almost insensitive to atomic decay. For a four-level atom in a diamond configuration initially prepared in the upper state, the source can produce entangled photon pairs even in the bad cavity limit via an adiabatic passage process. We have performed Monte Carlo wave function simulations to characterize these sources by means of: i) the success probability P of producing the desired entangled state, ii) the fidelity F in the reduced space of two emitted cavity photons, and iii) the S parameter of the Clauser-Horne-Shimony-Holt (CHSH) inequality to quantify the entanglement capability.
We propose a component-selective scheme for improving two-photon sources in a cavity-coupled two-atom system, where a single cavity mode interacts with two two-level atoms driven by phase-controlled classical fields of the same frequency. By controlling the atomic detunings and driving phase, the system can be tailored toward optimized cavity-field two-photon blockade or strongly correlated fluorescence photon-pair emission. When the two-cavity-photon component is enhanced, the cavity field exhibits optimized two-photon blockade with simultaneous suppression of unwanted one- and three-photon components at a comparable two-photon population. In another parameter regime, strongly correlated fluorescence photon pairs can also be generated from the two atoms by selecting the double-atomic-excitation component in the same two-excitation manifold. This approach provides a route toward high-quality and versatile two-photon sources, with potential applications in few-photon quantum optics and quantum information processing.
Abstract Spontaneous two-photon emission is a process in which the transition between two quantum states happens via simultaneous emissions of two identical photons. Such second-order quantum radiation is of paramount importance in astrophysics, atomic physics, and quantum technology. In particular, on-demand spontaneous two-photon emission from single quantum emitters has long been envisioned to revolutionize photonic quantum science and technology. To date, experimental realizations of two-photon emission at the single quanta level are still highly challenging yet elusive due to their low probabilities. In this work, we explore spontaneous two-photon emission from a single semiconductor quantum dot deterministically coupled to a high-quality microcavity in which the cavity resonances greatly enhance both excitation and emission processes. When the cavity is resonant to the half energy of the biexciton, the strong vacuum field in the cavity mode drives the biexciton to the ground state and simultaneously emits two photons into the cavity mode, resulting in two-photon emissions with a record brightness comparable to the competing single-photon process and sub-nanowatt power consumption. For the first time, the quantum nature associated with spontaneous two-photon emissions in the cavity quantum electrodynamics regime has been investigated via photon statistics measurements. Furthermore, spontaneous two-photon emission is exploited to build unconventional entangled quantum light sources with the unique advantage of combining the best of two worlds: near-unity entanglement fidelity for spontaneous parametric down-conversion source and on-demand photon emissions for atomic quantum emitters. Our work provides unprecedented insights into the two-photon process in the quantum regime and opens an unexplored avenue for pursuing optically reconfigurable quantum light sources with nonlinear quantum radiations.
A sequence of single photons is emitted on demand from a single three-level atom strongly coupled to a high-finesse optical cavity. The photons are generated by an adiabatically driven stimulated Raman transition between two atomic ground states, with the vacuum field of the cavity stimulating one branch of the transition, and laser pulses deterministically driving the other branch. This process is unitary and therefore intrinsically reversible, which is essential for quantum communication and networking, and the photons should be appropriate for all-optical quantum information processing.