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arXiv:2412.13418 · Optics Express

Characterization of near-infrared to telecom frequency conversion in a rubidium-filled hollow-core photonic-crystal fiber

Jed A. Rowland, Christopher Perrella, Rachel F. Offer, Andre Nicholas Luiten, Ben M. Sparkes, Till J. Weinhold

Published Mar 7, 2025• 6 citations
arXivHTMLPDF

Abstract

We experimentally investigate near-infrared to telecommunications frequency conversion via a diamond four-wave mixing scheme in rubidium vapor contained within a hollow-core photonic-crystal fiber. The strong light-atom interaction in the fiber results in lower pump power requirements and higher conversion efficiency than can be achieved under equivalent conditions in a rubidium vapor cell. We also observe non-intuitive pump and signal frequency dependence of the four-wave mixing efficiency in the fiber due to the large nonlinearities present in the system. These results indicate the potential for hollow-core fibers to provide a scalable solution for quantum information network infrastructure, with additional modelling required for a full understanding of the extreme atom-light interaction effects present.

DOI
10.1364/oe.549459

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We experimentally investigate near-infrared to telecommunications frequency conversion via a diamond four-wave mixing scheme in rubidium vapor contained within a hollow-core photonic-crystal fiber. The strong light-atom interaction in the fiber results in lower pump power requirements and higher conversion efficiency than can be achieved under equivalent conditions in a rubidium vapor cell. We also observe non-intuitive pump and signal frequency dependence of the four-wave mixing efficiency in the fiber due to the large nonlinearities present in the system. These results indicate the potential for hollow-core fibers to provide a scalable solution for quantum information network infrastructure, with additional modelling required for a full understanding of the extreme atom-light interaction effects present.
We demonstrate extremely efficient four-wave mixing with gains greater than 100 at microwatt pump powers and signal-to-idler conversion of 50% in Rb vapor confined to a hollow-core photonic band-gap fiber. We present a theoretical model that demonstrates such efficiency is consistent with the dimensions of the fiber and the optical depths attained. This is, to our knowledge, the largest four-wave mixing gain observed at such low total pump powers and the first demonstrated example of four-wave mixing in an alkali-metal vapor system with a large (approximately 30 MHz) ground state decoherence rate.
Large-area quantum networks based on optical fibers allow photons at near-infrared wavelengths to travel with minimal loss. Quantum frequency conversion is a method to alter the wavelength of a single photon while maintaining its quantum state. Most commonly, nonlinear crystals are employed for this conversion process, where near-unity conversion efficiency at high fidelity has been demonstrated. Still, the crystal-based conversion process is plagued by strong background noise, very limited spectral bandwidth, and inhomogeneous temperature profiles at strong pump fields. In the previous work, we have demonstrated frequency conversion in hydrogen-filled hollow-core fibers and claimed that this conversion process does not compromise performance at strong pump fields, is essentially free of background noise, and is intrinsically broadband. Here, we demonstrate that these three claims are justified: we demonstrate the quadratic scaling with pump field intensity, quantify the background level, and present coarse tuning over a range of 10 nm.
Quantum information networks will facilitate the use of a broad range of quantum technologies including quantum computers, quantum sensors, and quantum communication systems, among others. An important component of these networks are devices that enable light-atom interactions, as they interface photons from communication channels with the matter-based nodes, allowing for processing of photonic quantum information. These devices will need to be scalable and easily integrated to expand the size of networks. One platform of interest is vapour-filled hollow-core fibres (HCF). By overlapping light and atomic vapour within the same volume, strong interactions can occur, including important nonlinear effects such as cross-phase modulation and wave mixing processes. HCFs can be directly integrated into fibre systems, making them a convenient technology for the expansion of quantum networks. This thesis reports on three projects themed around scalable technologies for quantum networks. The first project involved the injection-locking of a diode laser. Nanosecond long pulses had their 20 GHz frequency chirps reduced to near the Fourier-transform limit, enabling them to interact efficiently with rubidium vapour. This project demonstrated that the mature, cost effective, and scalable technology of diode lasers can be compatible with essential atomic ensemble quantum networking devices such as quantum memories and quantum frequency converters. In the second project, a high-bandwidth quantum memory protocol called off-resonant cascaded absorption (ORCA) was investigated. The ORCA memory can be used to synchronise high speed photonic operations that occur in optical quantum information processing. This project used a Kagom´e HCF to enhance the light-atom interactions, resulting in two orders of magnitude reduction in optical power requirements. The third project again used the HCF platform, this time to facilitate a quantum frequency conversion scheme that converts rubidium-compatible, near-IR wavelengths to the telecommunications C-band, which is ideal for long distance fibre transmission. This project demonstrated the FWM process has reduced optical pump powers and higher efficiency in the HCF when compared to a rubidium-filled cell. The research described in this thesis presents a strong argument for the use of HCFs as a scalable technology that could be implemented in quantum networks.
We present an experimental realization of a noise-free and high-bandwidth quantum memory scheme using a rubidium vapor that is confined within the hollow core of a photonic crystal fiber. We achieve the same internal efficiencies as similar free-space experiments (30%) for 4.5-ns-long optical pulses but with a 100-fold reduction in the control-field power required. Modeling indicates that this efficiency could be improved to 88% with higher control powers and the implementation of techniques such as light-induced atomic desorption to increase the optical depth. The compactness, robustness, and low drive power of this approach lends itself to direct integration into large-scale fiber-based quantum processors.