Single atoms trapped in optical cavities exhibit immense potential as key nodes in future quantum information processing. They have already demonstrated significant advancement in various quantum technologies, particularly regarding the generation of nonclassical light. Here, we efficiently produce genuine photonic Bell states through the inelastic scattering process off single two-level intracavity atoms. An experimental violation of the Bell inequality, arising from the interference between the probability amplitudes of two photons, validates the intrinsic nature of energy-time entanglement. Coupling atoms with an optical cavity in the Purcell regime substantially enhances the two-photon scattering. This Bell state generation process does not require atomic spin control, thereby rendering it inherently immune to decoherence effects. This work advances the comprehension of resonance fluorescence and has the potential to broaden the landscape of quantum technologies and facilitate the application of photonic Bell states.
Single atoms trapped in optical cavities exhibit immense potential as key nodes in future quantum information processing. They have already demonstrated significant advancement in various quantum technologies, particularly regarding the generation of nonclassical light. Here, we efficiently produce genuine photonic Bell states through the inelastic scattering process off single two-level intracavity atoms. An experimental violation of the Bell inequality, arising from the interference between the probability amplitudes of two photons, validates the intrinsic nature of energy-time entanglement. Coupling atoms with an optical cavity in the Purcell regime substantially enhances the two-photon scattering. This Bell state generation process does not require atomic spin control, thereby rendering it inherently immune to decoherence effects. This work advances the comprehension of resonance fluorescence and has the potential to broaden the landscape of quantum technologies and facilitate the application of photonic Bell states.
Abstract Entanglement, the non-local correlations present in multipartite quantum systems, is a curious feature of quantum mechanics and the fuel of quantum technology. It is therefore a major priority to develop energy-conserving and simple methods for generating high-fidelity entangled states. In the case of light, entanglement can be realized by interactions with matter, although the required nonlinear interaction is typically weak, thereby limiting its applicability. Here, we show how a single two-level emitter deterministically coupled to light in a nanophotonic waveguide is used to realize genuine photonic quantum entanglement for excitation at the single photon level. By virtue of the efficient optical coupling, two-photon interactions are strongly mediated by the emitter realizing a giant nonlinearity that leads to entanglement. We experimentally generate and verify energy-time entanglement by violating a Bell inequality (Clauder-Horne-Shimony-Holt Bell parameter of S = 2.67(16)>2) in an interferometric measurement of the two-photon scattering response. As an attractive feature of this approach, the two-level emitter acts as a passive scatterer initially prepared in the ground state, i.e., no advanced spin control is required. This experiment is a fundamental advancement that may pave a new route for ultra-low energy-consuming synthesis of photonic entangled states for quantum simulators or metrology.
Single photons and single-photon pairs, inherently nonclassical in their nature, are fundamental elements of quantum sciences and technologies. Here, we propose to realize the nonclassical correlated deterministic photon pairs at the single-photon level for a single atom trapped in bimodal cavities. It is shown that the photon emissions for bimodal cavities exhibit a high single-photon purity and relatively large intracavity photon numbers, which are ascribed to the combination of optical Stark-shift enhanced energy-spectrum anharmonicity and quantum interference suppressed two-photon excitation. Our scheme generates photon-photon pairs with strong photon blockade for cavity modes via constructing a highly tunable cavity-enhanced deterministic parametric down-conversion process. Furthermore, we show that the cross-correlation function between the two cavity modes vastly violates the Cauchy-Schwarz inequality of the classical boundary, which unambiguously demonstrates the nonclassicality of the single-photon pairs. Our result reveals a prominent strategy to generate the high-quality two-mode single-photon sources with strong nonclassical correlation, which could provide versatile applications in distribution of quantum networks, long-distance quantum communication, and fundamental tests of quantum physics.
Resonance fluorescence, the process in which a single two-level quantum emitter interacts with a near-resonant coherent light, is a cornerstone of quantum optics as a paradigmatic light-matter interaction. Quantum phenomena in resonance fluorescence have been accounted for in terms of one- and two-photon processes; however, the physical processes arising from the interaction of a single two-level atom with higher photon numbers remain unexplored experimentally. Here we experimentally reveal the multiphoton scattering nature of resonance fluorescence, which intrinsically gives rise to multiphoton entanglement. By accessing quantum fluctuations in the field emitted from a cavity-quantum electrodynamics system, we resolve third- and fourth-order photon scattering events from a single two-level atom. In the three-photon component, the scattered photons are shown to be genuinely energy-time entangled, as verified by a violation of Svetlichny's inequality. As a demonstration of an application, a quantum secret sharing protocol (QSS) is implemented using this entangled photon source. Our study refines the descriptive framework of resonance fluorescence and broadens the scope of its investigation. It also establishes a fundamentally simple route for generating multiphoton entangled states for quantum information processing and quantum metrology.
Engineering atom-atom interactions is essential both for controlling novel phases of matter and for efficient preparation of many-body entangled states, which are key resources in quantum communication, computation, and metrology. In this work, we propose a scheme to tailor these interactions by coupling driven atom pairs to optical cavity photons via a molecular state in the dispersive regime, resulting in an effective photon-field-dependent potential. As an illustrative example, by analyzing the quantum Fisher information, we show that such induced interactions can generate robust many-body entanglement in two-mode ultracold bosons in an optical cavity. By tuning the photon-induced interactions through the cavity drive, we identify conditions for preparing highly entangled states on timescales that mitigate decoherence due to photon loss. Our results show that entanglement formation rate scales strongly with both photon and atom number, dramatically reducing the timescale compared to bare atomic interactions. We also identify an optimal measurement for exploiting the metrological potential of the atomic state in an interferometric protocol with significant photon losses, saturating the quantum Cramer-Rao lower bound. Furthermore, we show that despite these losses the atomic state exhibits strong Bell correlations. Our results pave the way for engineering atom-atom interactions to study novel phases of light and matter in hybrid atom-photon systems, as well as for tailoring complex quantum states for new quantum technology protocols and fundamental tests of quantum mechanics.
Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level, which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced dipolar interaction of atoms can be enhanced by a dielectric environment. For this Purcell effect, either a cavity or a waveguide can be used. Here, we combine the high densities achievable in thermal atomic vapors with an efficient coupling to a slot waveguide. In contrast to free-space interactions, atoms aligned within the slot exhibit repulsive interactions that are further enhanced by a factor of 8 due to the Purcell effect. The corresponding blueshift of the transition frequency of atoms arranged in the essentially one-dimensional geometry vanishes above the saturation, providing a controllable nonlinearity at the few-photon level. The experimental results are in good agreement with Monte Carlo simulations that include the dielectric environment, dipolar interactions, and motional effects. The results pave the way towards a robust scalable platform for quantum nonlinear optics and all-optical quantum information processing at room temperature.
Abstract The interaction of light with a single two-level emitter is the most fundamental process in quantum optics, and is key to many quantum applications. As a distinctive feature, two photons are never detected simultaneously in the light scattered by the emitter. This is commonly interpreted by saying that a single two-level quantum emitter can only absorb and emit single photons. However, it has been theoretically proposed that the photon anticorrelations can be thought of as arising from quantum interference between two possible two-photon scattering amplitudes, which one refers to as coherent and incoherent. This picture is in stark contrast to the aforementioned one, in that it assumes that the atom has two different mechanisms at its disposal to scatter two photons at the same time. Here we experimentally validate the interference picture by showing that, when spectrally rejecting only the coherent component of the fluorescence light of a single two-level atom, the remaining light consists of photon pairs that have been simultaneously scattered by the atom. Our results offer fundamental insights into the quantum-mechanical interaction between light and matter and open up novel approaches for the generation of highly non-classical light fields enabling, for example, Fourier-limited photon-pair sources that approach the theoretical limit in brightness.