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arXiv:2412.10970 · Optics Express

Experimental investigation of heralded Gaussification of phase-randomized coherent states of light

Martin Dostál, Miroslav Ježek, Jaromı́r Fiurášek, Jan Bílek

Published Nov 14, 2024• 1 citation
arXivHTMLPDF

Abstract

Probabilistic heralded Gaussification of quantum states of light is an important ingredient of protocols for distillation of continuous variable entanglement and squeezing. An elementary step of the heralded Gaussification protocol consists of interference of two copies of the state at a balanced beam splitter, followed by conditioning on the outcome of a suitable Gaussian quantum measurement on one output mode. When iterated, the protocol either converges to a Gaussian state or diverges. Here, we report on experimental investigation of the convergence properties of iterative heralded Gaussification. We experimentally implement two iterations of the protocol, which requires simultaneous processing of four copies of the input state. We utilize the phase-randomized coherent states as the input states, which greatly facilitates the experiment because these states can be generated deterministically, and their mean photon number can easily be tuned. We comprehensively characterize the input and partially Gaussified states by balanced homodyne detection and quantum state tomography. Our experimental results are in good agreement with theoretical predictions and they provide new insights into the convergence properties of heralded quantum Gaussification.

DOI
10.1364/oe.539787

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Probabilistic heralded Gaussification of quantum states of light is an important ingredient of protocols for distillation of continuous variable entanglement and squeezing. An elementary step of the heralded Gaussification protocol consists of interference of two copies of the state at a balanced beam splitter, followed by conditioning on the outcome of a suitable Gaussian quantum measurement on one output mode. When iterated, the protocol either converges to a Gaussian state or diverges. Here, we report on experimental investigation of the convergence properties of iterative heralded Gaussification. We experimentally implement two iterations of the protocol, which requires simultaneous processing of four copies of the input state. We utilize the phase-randomized coherent states as the input states, which greatly facilitates the experiment because these states can be generated deterministically, and their mean photon number can easily be tuned. We comprehensively characterize the input and partially Gaussified states by balanced homodyne detection and quantum state tomography. Our experimental results are in good agreement with theoretical predictions and they provide new insights into the convergence properties of heralded quantum Gaussification.
Distillation of entanglement using only Gaussian operations is an important primitive in quantum communication, quantum repeater architectures, and distributed quantum computing. Existing distillation protocols for continuous degrees of freedom are only known to converge to a Gaussian state when measurements yield precisely the vacuum outcome. In sharp contrast, non-Gaussian states can be deterministically converted into Gaussian states while preserving their second moments, albeit by usually reducing their degree of entanglement. In this work-based on a novel instance of a noncommutative central limit theorem-we introduce a picture general enough to encompass the known protocols leading to Gaussian states, and new classes of protocols including multipartite distillation. This gives the experimental option of balancing the merits of success probability against entanglement produced.
We propose a scheme for purification and distillation of squeezed and entangled continuous-variable states of light transmitted through a channel exhibiting phase fluctuations. The outstanding advantage of the suggested protocol is its experimental feasibility since it only involves an interference of two copies of the decohered state on a balanced beam splitter, a homodyne measurement on one of the output beams, and a conditioning on the measurement outcome. The purification can counteract the detrimental effects of phase fluctuations in optical quantum-communication networks.
The processing of information based on the generation of common quantum optical states (e.g. coherent states) and the measurement of the quadrature components of the light field (e.g. homodyne detection) is often referred to as continuous-variable quantum information processing. It is a very fertile field of investigation, at a crossroads between quantum optics and information theory, with notable successes such as unconditional continuous-variable quantum teleportation or Gaussian quantum key distribution. In quantum optics, the states of the light field are conveniently characterized using a phase-space representation (e.g. Wigner function), and the common optical components effect simple affine transformations in phase space (e.g. rotations). In quantum information theory, one often needs to determine entropic characteristics of quantum states and operations, since the von Neuman entropy is the quantity at the heart of entanglement measures or channel capacities. Computing entropies of quantum optical states requires instead turning to a state-space representation of the light field, which formally is the Fock space of a bosonic mode. This interplay between phase-space and state-space representations does not represent a particular problem as long as Gaussian states (e.g. coherent, squeezed, or thermal states) and Gaussian operations (e.g. beam splitters or squeezers) are concerned. Indeed, Gaussian states are fully characterized by the first- and second-order moments of mode operators, while Gaussian operations are defined via their actions on these moments. The so-called symplectic formalism can be used to treat all Gaussian transformations on Gaussian states, including mixed states of an arbitrary number of modes, and the entropies of Gaussian states are directly linked to their symplectic eigenvalues. This thesis is concerned with the Gaussian transformations applied onto arbitrary states of light, in which case the symplectic formalism is unapplicable and this phase-to-state space interplay becomes highly non trivial. A first motivation to consider arbitrary (non-Gaussian) states of light results from various Gaussian no-go theorems in continuous-variable quantum information theory. For instance, universal quantum computing, quantum entanglement concentration, or quantum error correction are known to be impossible when restricted to the Gaussian realm. A second motivation comes from the fact that several fundamental quantities, such as the entanglement of formation of a Gaussian state or the communication capacity of a Gaussian channel, rely on an optimization over all states, including non-Gaussian states even though the considered state or channel is Gaussian. This thesis is therefore devoted to developing new tools in order to compute state-space properties (e.g. entropies) of transformations defined in phase-space or conversely to computing phase-space properties (e.g. mean-field amplitudes) of transformations defined in state space. Remarkably, even some basic questions such as the entanglement generation of optical squeezers or beam splitters were unsolved, which gave us a nice work-bench to investigate this interplay. In the first part of this thesis (Chapter 3), we considered a recently discovered Gaussian probabilistic transformation called the noiseless optical amplifier. More specifically, this is a process enabling the amplification of a quantum state without introducing noise. As it has long been known, when amplifing a quantum signal, the arising of noise is inevitable due to the unitary evolution that governs quantum mechanics. It was recently realized, however, that one can drop the unitarity of the amplification procedure and trade it for a noiseless, albeit probabilistic (heralded) transformation. The fact that the transformation is probabilistic is mathematically reflected in the fact that it is non trace-preserving. This quantum device has gained much interest during the last years because it can be used to compensate losses in a quantum channel, for entanglement distillation, probabilistic quantum cloning, or quantum error correction. Several experimental demonstrations of this device have already been carried out. Our contribution to this topic has been to derive the action of this device on squeezed states and to prove that it acts quite surprisingly as a universal (phase-insensitive) optical squeezer, conserving the signal-to-noise ratio just as a phase-sensitive optical amplifier but for all quadratures at the same time. This also brought into surface a paradoxical effect, namely that such a device could seemingly lead to instantaneous signaling by circumventing the quantum no-cloning theorem. This paradox was discussed and resolved in our work. In a second step, the action of the noiseless optical amplifier and it dual operation (i.e. heralded noiseless attenuator) on non-Gaussian states has been examined. We have observed that the mean-field amplitude may decrease in the process of noiseless amplification (or may increase in the process of noiseless attenuation), a very counterintuitive effect that Gaussian states cannot exhibit. This work illustrates the above-mentioned phase-to-state space interplay since these devices are defined as simple filtering operations in state space but inferring their action on phase-space quantities such as the mean-field amplitude is not straightforward. It also illustrates the difficulty of dealing with non-Gaussian states in Gaussian transformations (these noiseless devices are probabilistic but Gaussian). Furthermore, we have exhibited an experimental proposal that could be used to test this counterintuitive feature. The proposed set-up is feasible with current technology and robust against usual inefficiencies that occur in optical experiment. Noiseless amplification and attenuation represent new important tools, which may offer interesting perspectives in quantum optical communications. Therefore, further understanding of these transformations is both of fundamental interest and important for the development and analysis of protocols exploiting these tools. Our work provides a better understanding of these transformations and reveals that the intuition based on ordinary (deterministic phase-insensitive) amplifiers and losses is not always applicable to the noiseless amplifiers and attenuators. In the last part of this thesis, we have considered the entropic characterization of some of the most fundamental Gaussian transformations in quantum optics, namely a beam splitter and two-mode squeezer. A beam splitter effects a simple rotation in phase space, while a two-mode squeezer produces a Bogoliubov transformation. Thus, there is a well-known phase-space characterization in terms of symplectic transformations, but the difficulty originates from that one must return to state space in order to access quantum entropies or entanglement. This is again a hard problem, linked to the above-mentioned interplay in the reverse direction this time. As soon as non-Gaussian states are concerned, there is no way of calculating the entropy produced by such Gaussian transformations. We have investigated two novel tools in order to treat non-Gaussian states under Gaussian transformations, namely majorization theory and the replica method. In Chapter 4, we have started by analyzing the entanglement generated by a beam splitter that is fed with a photon-number state, and have shown that the entanglement monotones can be neatly combined with majorization theory in this context. Majorization theory provides a preorder relation between bipartite pure quantum states, and gives a necessary and sufficient condition for the existence of a deterministic LOCC (local operations and classical communication) transformation from one state to another. We have shown that the state resulting from n photons impinging on a beam splitter majorizes the corresponding state with any larger photon number n’ > n, implying that the entanglement monotonically grows with n, as expected. In contrast, we have proven that such a seemingly simple optical component may have a rather surprising behavior when it comes to majorization theory: it does not necessarily lead to states that obey a majorization relation if one varies the transmittance (moving towards a balanced beam splitter). These results are significant for entanglement manipulation, giving rise in particular to a catalysis effect. Moving forward, in Chapter 5, we took the step of introducing the replica method in quantum optics, with the goal of achieving an entropic characterization of general Gaussian operations on a bosonic quantum field. The replica method, a tool borrowed from statistical physics, can also be used to calculate the von Neumann entropy and is the last line of defense when the usual definition is not practical, which is often the case in quantum optics since the definition involves calculating the eigenvalues of some (infinite-dimensional) density matrix. With this method, the entropy produced by a two-mode squeezer (or parametric optical amplifier) with non-trivial input states has been studied. As an application, we have determined the entropy generated by amplifying a binary superposition of the vacuum and an arbitrary Fock state, which yields a surprisingly simple, yet unknown analytical expression. Finally, we have turned to the replica method in the context of field theory, and have examined the behavior of a bosonic field with finite temperature when the temperature decreases. To this end, information theoretical tools were used, such as the geometric entropy and the mutual information, and interesting connection between phase transitions and informational quantities were found. More specifically, dividing the field in two spatial regions and calculating the mutual information between these two regions, it turns out that the mutual information is non-differentiable exactly at the critic
Abstract Entanglement of continuous-variable Gaussian states can be distilled by combination of de-Gaussifying operation such as single-photon subtraction and iterative heralded Gaussification. Here we present and analyze a simplified equivalent version of such entanglement distillation protocol, where the Gaussian measurements utilized in heralded Gaussification are eliminated and are absorbed into the preparation of suitable input Gaussian states of the simplified protocol. The simplified scheme contains less detectors and its overall success probability increases in comparison with the original scheme, while producing completely equivalent outputs. Our simplification of the entanglement distillation protocol closely parallels the recently proposed simplification of a scheme for breeding optical single-mode Gottesman–Kitaev–Preskill states (Aghaee Rad et al 2025 Nature 638 912 ). We investigate operation of the simplified entanglement distillation scheme for both pure and mixed input states and clarify how multicopy distillation of Gaussian entanglement emerges in a setup without any heralding Gaussian measurements.
Coherent state superpositions, also known as Schrödinger cat states, are widely recognized as promising resources in quantum information, quantum metrology, as well as fundamental tests. These states are hard to produce deterministically and most schemes for their probabilistic generation can only attain amplitudes too small for practical use. This is for example the case for photon-subtracted squeezed vacuum (PSSV), which can be used to approximate cat states of amplitude no larger than y = 1.5 if the fidelity is to be maintained above 95%. One way to reach larger amplitudes is to start with pairs of small cats and then to interfere them on a balanced beam splitter. The projective measurement of one of the outputs is used to herald a larger cat resulting from the constructive interference of the initial states. The scheme proposed here uses the projection |x = 0〉〈x = 0| as the heralding condition. Homodyning is proposed, as opposed to photon counting, because homodyne detection has high a quantum efficiency, and - as demonstrated in the paper - can be tuned to increase the success probability of the amplification without heavily compromising the output's fidelity.
Entangled photons are ideally suited to the transmission of photonic quantum information. Mitigating the effects of decoherence is fundamental to distributing photonic entanglement across large distances. One such proposal is entanglement distillation, in which operations on a large ensemble of weakly entangled states generate a smaller ensemble of more strongly entangled states. In this thesis, we experimentally and theoretically analyse various tools required for demonstrating continuous-variable (CV) entanglement distillation, following the proposal by Browne et al., [Phys. Rev. A 67, 062320 (2003)]. Specifically, we propose figures of merit to account for the practical limitations of non-deterministic non-Gaussian operations, and analyse the experimental parameters necessary to optimise them. We develop a source of pulsed two-mode squeezed states, which are the initial states of our entanglement distillation protocol. We use weak-field homodyne detection as a phase-dependent photon counting detector, and demonstrate its utility in conditional state generation. Using these states, we demonstrate sub-binomial light as a tool for benchmarking quantum states. Finally, we applied two-mode weak-field homodyne detection to two entangled states and demonstrate correlations in the photon counting statistics which depend on a joint phase from two independent local oscillators. This setup is sufficient to apply an entanglement witness developed by Puentes et al. [New J. Phys. 12, 033042 (2010)]. Despite encouraging simulations, we do not witness entanglement with this scheme, which we attribute to a noise source unaccounted for in the simulations. Although we do not demonstrate entanglement distillation outright, the tools we develop to do so represent a general, hybrid approach to CV quantum optics. Developing tools such as phase-resolved projective measurement on two-mode states allows us to probe both the wave and particle nature of entangled light at the single-photon level. Using and expanding these techniques to probe larger quantum systems may prove useful in studies of fundamental physics and quantum enhanced technologies.