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arXiv:2412.10954 · Physical Review Applied

Structured position-momentum-entangled two-photon fields

Radhika Prasad, Sanjana Wanare, Suman Karan, Mritunjay K. Joshi, Abhinandan Bhattacharjee, Anand K. Jha

Published Dec 10, 2024• 5 citations
arXivHTMLPDF

Abstract

Structured optical fields have led to several ground-breaking techniques in classical imaging and microscopy. At the same time, in the quantum domain, position-momentum entangled photon fields have been shown to have several unique features that can lead to beyond-classical imaging and microscopy capabilities. Therefore, it is natural to expect that position-momentum entangled two-photon fields that are structured can push the boundaries of quantum imaging and microscopy even further beyond. Nonetheless, the existing experimental schemes are able to produce either structured two-photon fields without position-momentum entanglement, or position-momentum entangled two-photon fields without structured correlations. In this article, by manipulating the phase-matching condition of the spontaneous parametric down-conversion process, we report experimental generation of two-photon fields with various structures in their spatial correlations. We experimentally measure the minimum bound on the entanglement of formation and thereby verify the position-momentum entanglement of the structured two-photon field. We expect this work to have important implications for quantum technologies related to imaging and sensing.

DOI
10.1103/physrevapplied.22.064034

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Structured optical fields have led to several ground-breaking techniques in classical imaging and microscopy. At the same time, in the quantum domain, position-momentum entangled photon fields have been shown to have several unique features that can lead to beyond-classical imaging and microscopy capabilities. Therefore, it is natural to expect that position-momentum entangled two-photon fields that are structured can push the boundaries of quantum imaging and microscopy even further beyond. Nonetheless, the existing experimental schemes are able to produce either structured two-photon fields without position-momentum entanglement, or position-momentum entangled two-photon fields without structured correlations. In this article, by manipulating the phase-matching condition of the spontaneous parametric down-conversion process, we report experimental generation of two-photon fields with various structures in their spatial correlations. We experimentally measure the minimum bound on the entanglement of formation and thereby verify the position-momentum entanglement of the structured two-photon field. We expect this work to have important implications for quantum technologies related to imaging and sensing.
Biphoton systems exhibiting entanglement in position-momentum variables, known as spatial entanglement, are among the most intriguing and well-studied phenomena in quantum optics. A notable subset of these are phase entangled states, where entanglement manifests purely through correlations in the spatial phase of the wavefunction. While the generation of such states from biphotons via spontaneous parametric down-conversion has been explored, their physical implications and applications remain under-investigated. In this work, we theoretically and experimentally examine a unique form of phase entanglement known as `pure' phase entanglement. This state exhibits the unusual feature that the position of one photon is correlated with the momentum of the other. Unlike typical spatially entangled states, it shows no direct correlation in position or momentum between the two photons, underscoring that all correlations arise purely from the spatial phase of the wavefunction. We delve deeper into the theory of this state and experimentally construct it from known phase-entangled states. To certify its properties, we propose a setup that performs a "one-particle momentum measurement" and explore the various tunable parameters. We also highlight potential applications of this state in quantum optics and imaging experiments.
Entanglement, a key resource of emerging quantum technologies, describes correlations between particles that defy classical physics. It has been studied extensively on various platforms, but has remained elusive in electron microscopy. Transmission electron microscopes are well-established tools for materials characterisation with unparalleled spatial resolution. They provide control over the preparation and detection of high energy electrons, with largely unexploited potential in the study of many-body quantum correlations. Here, we demonstrate entanglement in electron-photon pairs generated via cathodoluminescence in a transmission electron microscope. Employing coincidence imaging techniques adapted from photonic quantum optics, we reconstruct both near- and far-field ``ghost'' images of periodic transmission masks. By measuring spatial and momentum correlations, we show a violation of the classical uncertainty bound: Δx−2Δk+2=0.502±0.047<1Δx_-^2 Δk_+^2 = 0.502 \pm 0.047<1Δx−2​Δk+2​=0.502±0.047<1. Hence, we demonstrate entanglement in position and momentum -- the continuous variables at the base of most imaging methods, bridging the fields of electron microscopy and quantum optics. Our work paves the way for exploring quantum correlations in free-electron systems and their application to quantum-enhanced imaging techniques on the nanoscale.
We experimentally demonstrate how the two-photon field generated by spontaneous parametric down-conversion contains an intriguing fine structure associated with the positional spread within the photon pair. The obtained results provide a three-dimensional picture of the near-field correlations, which are determined by the phase-matching conditions. These correlations are compared with previous results on second-harmonic generation, spatial antibunching, and transverse entanglement in parametric down-conversion.
Abstract The measurement of the position–momentum Einstein–Podolsky–Rosen (EPR) correlations of a two-photon state is important for many quantum information applications ranging from quantum key distribution to coincidence imaging. However, all the existing techniques for measuring the position–momentum EPR correlations involve coincidence detection and thus suffer from issues that result in less accurate measurements. In this article, we propose and demonstrate an experimental scheme that does not require coincidence detection for measuring the EPR correlations. Our technique works for two-photon states that are pure, irrespective of whether the state is separable or entangled. We theoretically show that if the pure two-photon state satisfies a certain set of conditions then the position–momentum EPR correlations can be obtained by doing the intensity measurements on only one of the photons. We experimentally demonstrate this technique for pure two-photon states produced by type-I spontaneous parametric down-conversion, and to the best of our knowledge, we report the most accurate experimental measurement of position–momentum EPR correlations.
High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also provides access to several intriguing quantum phenomena. One such non-intuitive phenomenon is phase entanglement, in which the biphoton state is correlated in the complex phase of its wavefunction. This state, which emerges during the propagation of the biphoton wavefunction, exhibits neither position nor momentum correlation, yet retains full entanglement. In this work, we experimentally explore this state in two distinct ways. The first is by tracking the vanishing spatial photon number correlation over propagation distances lying in [0,∞)\left[0,\infty\right)[0,∞), folded into a finite range using single-lens imaging. These observations show excellent agreement with our theoretical predictions based on the Double Gaussian (DG) approximation of the biphoton state. The second approach involves performing a two-photon interference experiment using a double slit and this state, which reveals the correlated phase front. We show, both theoretically and experimentally, that the observed two-photon interference structure is markedly different from that produced by position-correlated photons, as confirmed by computing the joint probability distribution of photons (JPD) and related metrics. Such interference using phase-entangled light has not been attempted before and opens avenues for advanced experiments and applications in the field of spatial entanglement.