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arXiv:2412.08724 · Physical Review A

Separability Lindblad equation for dynamical open-system entanglement

Julien Pinske, Laura Ares, Benjamin Hinrichs, Martin Kolb, Jan Sperling

Published Dec 3, 2025• 5 citations
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Abstract

Providing entanglement for the design of quantum technologies in the presence of noise constitutes today's main challenge in quantum information science. A framework is required that assesses the build-up of entanglement in realistic settings. In this work, we put forth a new class of nonlinear quantum master equations in Lindblad form that unambiguously identify dynamical entanglement in open quantum systems via deviations from a separable evolution. This separability Lindblad equation restricts quantum trajectories to classically correlated states only. Unlike many conventional approaches, here the entangling capabilities of a process are not characterized by input-output relations, but separability is imposed at each instant of time. We solve these equations for crucial examples, thereby quantifying the dynamical impact of entanglement in non-equilibrium scenarios. Our results allow to benchmark the engineering of entangled states through dissipation. The separability Lindblad equation provides a unique path to characterizing quantum correlations caused by arbitrary system-bath interactions, specifically tailored for the noisy intermediate-scale quantum era.

DOI
10.1103/kd3b-bfxq

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Providing entanglement for the design of quantum technologies in the presence of noise constitutes today's main challenge in quantum information science. A framework is required that assesses the build-up of entanglement in realistic settings. In this work, we put forth a new class of nonlinear quantum master equations in Lindblad form that unambiguously identify dynamical entanglement in open quantum systems via deviations from a separable evolution. This separability Lindblad equation restricts quantum trajectories to classically correlated states only. Unlike many conventional approaches, here the entangling capabilities of a process are not characterized by input-output relations, but separability is imposed at each instant of time. We solve these equations for crucial examples, thereby quantifying the dynamical impact of entanglement in non-equilibrium scenarios. Our results allow to benchmark the engineering of entangled states through dissipation. The separability Lindblad equation provides a unique path to characterizing quantum correlations caused by arbitrary system-bath interactions, specifically tailored for the noisy intermediate-scale quantum era.
We develop an extension of the Monte Carlo wave function approach that unambiguously identifies dynamical entanglement in general composite, open systems. Our algorithm performs tangential projections onto the set of separable states, leading to classically correlated quantum trajectories. By comparing this restricted evolution with the unrestricted one, we can characterize the entangling capabilities of quantum channels without making use of input-output relations. Moreover, applying this method is equivalent to solving the nonlinear master equation in Lindblad form introduced in \cite{PAH24} for two-qubit systems. We here extend these equations to multipartite systems of qudits, describing non-entangling dynamics in terms of a stochastic differential equation. We identify the impact of dynamical entanglement in open systems by applying our approach to several correlated decay processes. Therefore, our methodology provides a complete and ready-to-use framework to characterize dynamical quantum correlations caused by arbitrary open-system processes.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
Open quantum system dynamics is efficiently described by the quantum master equation formalism. Therein, quantum master equations in Lindblad form constitute an important subclass describing Markovian dynamics. When an open quantum system is in an out-of-equilibrium state, an exchange of particles between the open system and reservoirs takes place yielding to a non-zero average net current and associated current fluctuations, which can be characterised with the quantum jump formalism for quantum master equations expressed in Lindblad form. However, a large class of quantum master equations cannot be described by Lindblad dynamics. Here we assess the validity and the effectiveness of the quantum jump formalism when the dissipators in the quantum master equation describe a non-additive, open quantum system dynamics. We find that an additive unravelling of the non-additive quantum master equation does not generate a completely-positive dynamics in the scenario of perfect jump detection. Nevertheless, allowing for an imperfect jump detection scenario, we find that an additive unravelling is possible that reproduces the current and the fluctuations obtained via the Landauer-Büttiker formalism.
In the framework of the theory of open systems based on completely positive quantum dynamical semigroups, we study the continuous variable entanglement for a system consisting of two independent harmonic oscillators interacting with a general environment. We solve the Kossakowski-Lindblad master equation for the time evolution of the considered system and describe the entanglement in terms of the covariance matrix for an arbitrary Gaussian input state. Using Peres–Simon necessary and sufficient criterion for separability of two-mode Gaussian states, we show that for certain values of diffusion and dissipation coefficients describing the environment, the state keeps for all times its initial type: separable or entangled. In other cases, entanglement generation, entanglement sudden death or a periodic collapse and revival of entanglement take place. We analyze also the time evolution of the logarithmic negativity, which characterizes the degree of entanglement of the quantum state.
The role of quantum entanglement in thermodynamical systems remains elusive. Does entanglement result in thermodynamic advantages or does it impose fundamental limitations? Here, we unambiguously quantify the amount of heat and work in a quantum system that is due to the presence of entanglement. This is achieved by constraining the system's non-equilibrium dynamics to separable states, thereby isolating the impact entanglement has on thermodynamic effects. Unlike thermodynamic entanglement measures, which signify a loose connection between entanglement and thermodynamic properties, imposing a constraint constitutes an active intervention into a system -- answering how much of a system's thermodynamics is caused by (not correlated with) its quantumness. We benchmark our theory by applying the constrained dynamics to several multipartite systems, including quantum batteries and quantum refrigerators.
Reservoir engineering has proven to be a practical approach to control open quantum systems, preserving quantum coherence by appropriately manipulating the reservoir and system-reservoir interactions. In this context, for systems comprised of different parts, it is common to describe the dynamics of a subsystem of interest by performing an adiabatic elimination of the remaining components of the system. This procedure often leads to an effective master equation for the subsystem that is not in the diagonal form of the Gorini-Kossakowski-Lindblad-Sudarshan master equation (here called diagonal Lindblad form). Instead, it has a more general structure (here called non-diagonal Lindblad form), which explicitly reveals the dissipative coupling between the various components of the subsystem. In this work, we present a set of dynamical equations for the first and second moments of the canonical variables for linear Gaussian systems, bosonic and fermionic, described by non-diagonal Lindblad master equations. Our method is efficient and allows one to obtain analytical solutions for the steady state. We supplement our findings with a review of covariance matrix methods, focusing on those related to the measurement of entanglement. Notably, our exploration yields a surprising byproduct: the Duan criterion, commonly applied to bosonic systems for verification of entanglement, is found to be equally valid for fermionic systems. We conclude with a practical example, where we revisit two-mode mechanical entanglement in an optomechanical setup. Our approach, which employs adiabatic elimination for systems governed by time-dependent Hamiltonians, opens the door to examine physical regimes that have not been explored before.