Whether a photon exhibits wavelike or particlelike behaviour depends on the observation method, as clearly demonstrated by Wheeler's delayed choice (DC) experiments. A key aspect of such experiments is the random determination of the observation device's status, typically controlled by a random number generator or a quantum-controlling apparatus. Here, we propose a novel version of the quantum delayed choice (QDC) experiment by tailoring the quantum state of the single photon into an arbitrary polarization superposition. In this experiment, the "choice" can be considered as being made by the photon's state itself at the moment of observation, thereby violating classical causality. Additionally, we observe the morphing behaviour of the single photon between wavelike and particlelike characteristics, which challenges the classical picture of waves and particles. Utilizing the quantum state of the photon rather than the quantum-controlling devices not only facilitates the implementation of the QDC experiment but also helps deepen the understanding of Bohr's complementarity principle.
Whether a photon exhibits wavelike or particlelike behaviour depends on the observation method, as clearly demonstrated by Wheeler's delayed choice (DC) experiments. A key aspect of such experiments is the random determination of the observation device's status, typically controlled by a random number generator or a quantum-controlling apparatus. Here, we propose a novel version of the quantum delayed choice (QDC) experiment by tailoring the quantum state of the single photon into an arbitrary polarization superposition. In this experiment, the "choice" can be considered as being made by the photon's state itself at the moment of observation, thereby violating classical causality. Additionally, we observe the morphing behaviour of the single photon between wavelike and particlelike characteristics, which challenges the classical picture of waves and particles. Utilizing the quantum state of the photon rather than the quantum-controlling devices not only facilitates the implementation of the QDC experiment but also helps deepen the understanding of Bohr's complementarity principle.
Whether a photon exhibits wavelike or particlelike behavior depends on the observation method, as clearly demonstrated by the quantum erasure (QE) experiments. Here, we propose a novel, to the best of our knowledge, version of the QE experiment that leverages a single photon prepared in an arbitrary polarization superposition state. Unlike traditional approaches that have a definite erasure method, the erasure in our experiment is determined intrinsically by the photon's quantum state at the moment of measurement. Furthermore, we observe continuous morphing between wave and particle behavior, enabled by continuous path information erasure in the photon's transverse mode. This dynamic transition challenges the classical dichotomy of waves and particles. These findings provide deeper insight into Bohr's complementarity principle and expand the conceptual framework of quantum mechanics.
Bohr's complementarity notion is at the heart of quantum physics. It suggests that quantum systems are observed as waves or particles depending on the type of measurement, i.e., the experimental arrangement, they are subjected to. For instance, sending single photons to an open or closed Mach-Zehnder interferometer (MZI) leads to the observation of particle or wave behaviours, respectively. In 1984, Wheeler proposed a "Gedanken" delayed-choice experiment in which the interferometer configuration is chosen at will by the experimentalist only after the photon has already passed the input beam-splitter (BS_in) of the device. This experiment was realized using a single photon source and showed that Bohr's complementarity notion was still obeyed.It was recently proposed to take Wheeler's experiment one step further by employing an output "quantum beam-splitter" (QBS), i.e.,preparing BS_out in a coherent superposition of being absent and present. This allows choosing the type of measurement, i.e., wave or particle, only after having determined the state of the QBS, which can be (in principle) infinitely delayed.We realized such an experiment by exploiting the resource of entanglement, in this case pairs of polarization entangled photons. The behaviour of one of the paired photons, called the test photon, is analysed using a MZI having a QBS at its output. This QBS is enabled by entanglement and made of a polarization dependent beam-splitter. The other photon, called the corroborative photon, allows determining the state of the QBS, and consequently, which test photon behaviour (wave, particle, or both) is observed.By manipulating the corroborative photon polarization state, we demonstrate a continuous morphing of the test photon from wave to particle behaviour. This refutes simple models of single photons behaving exclusively as waves or particles. The state of the QBS is determined via the measurement of the corroborative photon only after the test photon has already been detected. The space-like separation between the two measurements invalidates local-hidden variable models associated with pre-existing information about the measurement outcomes. In other words, when the test photon is detected, no information is available about the type of measurement it underwent. These results still perfectly obey Bohr's complementarity notion and its extension.
Wheeler's delayed-choice experiment delays the decision to observe either the wave or particle behavior of a photon until after it has entered the interferometer, and the quantum delayed-choice experiment provides the possibility of observing the wave and particle behaviors with a single experimental setup by introducing quantum control. We here propose a modified quantum delayed-choice experiment without quantum control or entanglement assistance, in which a photon can be prepared in a wave-particle superposition state and the morphing behavior of wave-to-particle transition can be observed easily. It is demonstrated that the presented scheme can allow us to rule out classical hidden-variable models in a device-independent manner via violating dimension witness. We also extend the scheme to the situation of two degrees of freedom, first constructing a hybrid quantum delayed-choice experiment which enables a photon respectively exhibits wave and particle behaviors in different degrees of freedom, and then proposing a scheme to prepare the single-photon wave-particle entanglement. This study is not only meaningful to explore the wave-particle complementarity of photons, but also provides potential for the research of the single-particle nonlocality from the perspective of the wave-particle degree of freedom.
Bohr's complementarity notion is at the heart of quantum physics, and suggests that in a quantum experiment, the observed phenomena are inherently linked to the type of measurement that is performed. For example, sending single photons to an open or closed Mach-Zehnder interferometer leads to the observation of particle or wave behaviours. In 1984, Wheeler proposed a 'Gedanken' experiment in which the experimentalist chooses the interferometer configuration, at will, only after the photon has already passed the input beam-splitter (BSin) of the device. This experiment was realized using a diamond-based single photon source, and it was shown that Bohr's complementarity notion was still obeyed, as expected. It was recently proposed theoretically to take Wheeler's experiment one step further by employing a 'quantum beam-splitter' (QBS) at the interferometer output. In this case, the output beam-splitter (BSout) is placed in a coherent superposition of being absent and present, which also allows to further delay the choice of the measurement type. The type of measurement is determined only after having measured the state of the QBS, which can be (in principle) infinitely delayed. We demonstrate the realization of such an experiment by exploiting entanglement. In particular, we take advantage of pairs of polarization entangled photons. The behaviour of one of the paired photons, called the test photon, is analysed by sending it to a Mach-Zehnder interferometer having an entanglement-enabled QBS at its output. This device is made of a polarization dependent beam-splitter followed by polarization state erasers. The other photon, called the corroborative photon, allows determining the actual state of the QBS, and consequently, which test photon behaviour (wave, particle, or both) is measured. By manipulating the corroborative photon, we demonstrate a continuous morphing from wave to particle behaviour, which refutes too simple views of single photons behaving exclusively as waves or particles. The measurements on the test photon and the interferometer configuration are performed in a strictly delayed manner. The state of the QBS is measured only after the test photon already left the interferometer, and is detected, which means that it is destroyed before the type of measurement it under- goes is determined. We find that even in this configuration, Bohr's complementarity notion, and its extension, are perfectly obeyed. The space-like separation between the measurements invalidates local-hidden variable models associated with pre-existing information about the measurement out- comes. In other words, when the test photon is detected, no information is available about the type of measurement that was performed. This assertion is confirmed by the violation of the Bell's inequalities with more than 10 standard deviations. The presence of entanglement shows furthermore that genuine quantum behaviour for the test photons has been observed. As a conclusion, we have demonstrated the experimental realization of the quantum version of Wheeler's experiment. Trying to explain our observations in classical terms causes severe contradictions, but the results are in perfect agreement with quantum physics, in which the measurement timing order does not matter. The beauty in such experiments is that space and time do not seem to play any role.
Gedanken experiments help to reconcile our classical intuition with quantum mechanics and nowadays are routinely performed in the laboratory. An important open question is the quantum behavior of the controlling devices in such experiments. We propose a framework to analyze quantum-controlled experiments and illustrate it by discussing a quantum version of Wheeler's delayed-choice experiment. Using a quantum control has several consequences. First, it enables us to measure complementary phenomena with a single experimental setup, pointing to a redefinition of complementarity principle. Second, it allows us to prove there are no consistent hidden-variable theories having "particle" and "wave" as realistic properties. Finally, it shows that a photon can have a morphing behavior between particle and wave. The framework can be extended to other experiments (e.g., Bell inequality).
Wave-particle duality constitutes one of the most intriguing features in quantum physics. A well-known gedanken experiment that provides evidence for this is Wheeler's delayed-choice experiment based on a Mach-Zehnder interferometer [J. A. Wheeler, in Mathematical Foundations of Quantum Theory, edited by A. R. Marlow (Academic, New York, 1978), pp. 9--48; in Quantum Theory and Measurement, edited by J. A. Wheeler and W. H. Zurek (Princeton University Press, Princeton, 1984), pp. 182--213]. Many different versions of delayed-choice experiments have been conducted with both classical and quantum detecting devices. Recently, it was proposed that the delayed-choice experiment could be devised from the perspective of a device-independent prepare-and-measure scenario [R. Chaves et al., Causal Modeling the Delayed-Choice Experiment, Phys. Rev. Lett. 120, 190401 (2018)]. In our work, we experimentally realize this modified version with a deterministic single-photon source and examine the wave-particle objective in a causal-modeled scheme without the assistance of entanglement, which is achieved by violating the dimension-witness inequalities. Our experiment also provides an intriguing perspective and exhibits the benefits of studying quantum theory from the casual model point of view.