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arXiv:2412.05480 · Optica Quantum

Efficient storage of multidimensional telecom photons in a solid-state quantum memory

Zongfeng Li, Yisheng Lei, Trevor Kling, Mahdi Hosseini

Published May 28, 2025• 3 citations
arXivHTMLPDF

Abstract

Efficient storage of telecom-band quantum optical information represents a crucial milestone for establishing distributed quantum optical networks. Erbium ions in crystalline hosts provide a promising platform for telecom quantum memories; however, their practical applications have been hindered by demanding operational conditions, such as ultra-high magnetic fields and ultra-low temperatures. In this work, we demonstrate the storage of telecom photonic qubits encoded in polarization, frequency, and time-bin bases. Using the atomic frequency comb protocol in an Er 3+ -doped crystal, we developed a memory initialization scheme that improves storage efficiency by over an order of magnitude. The observed results were made possible by the deliberate selection of the pumping sequence and the minimization of lattice interactions, to the extent possible without the use of dilution refrigerators or superconducting magnets.

DOI
10.1364/opticaq.564321

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Efficient storage of telecom-band quantum optical information represents a crucial milestone for establishing distributed quantum optical networks. Erbium ions in crystalline hosts provide a promising platform for telecom quantum memories; however, their practical applications have been hindered by demanding operational conditions, such as ultra-high magnetic fields and ultra-low temperatures. In this work, we demonstrate the storage of telecom photonic qubits encoded in polarization, frequency, and time-bin bases. Using the atomic frequency comb protocol in an Er 3+ -doped crystal, we developed a memory initialization scheme that improves storage efficiency by over an order of magnitude. The observed results were made possible by the deliberate selection of the pumping sequence and the minimization of lattice interactions, to the extent possible without the use of dilution refrigerators or superconducting magnets.
Optical quantum memories will enable technologies including long distance quantum communication and modular quantum computing. Rare earth ion doped crystals provide an excellent solid state platform for optical quantum memories. Among rare earths, erbium is particularly appealing due to its long-lived telecom-wavelength resonance, allowing integration with silicon photonics and with existing optical communication technology and infrastructure. We present an on-chip all-optical quantum memory at telecom wavelengths using a nanobeam photonic crystal cavity fabricated directly in erbium-167 doped yttrium orthosilicate. Using an atomic frequency comb protocol, we store coherent pulses for memory times as long as 10 µs, albeit with low efficiency. For shorter memory times, we achieve a memory efficiency of 0.4%, which is limited by the coupling rate between the resonator and the ensemble of ions. By working at dilution refrigerator temperatures, we are able to access a regime where the ions have long optical coherence times and good spectral holeburning properties using only a moderate magnetic field applied with permanent magnets. We characterize the multimode properties and fidelity of the quantum memory in this device, and outline a path toward higher efficiency.
The quantum internet is envisioned to enable transformative applications such as distributed quantum computing, quantum-enhanced distributed sensing, precise clock distribution, and secure communication. However, the development of the envisioned quantum internet hinges upon high performance quantum memories (QMs). Rare-earth ions doped in solids are among the promising candidates for realizing QMs due to high multimode storage capability, long coherence time and high storage efficiency. In this work, we demonstrate a practical solid-state memory using Erbium ions (Er3+), operating at telecom wavelengths (1536 nm) compatible with existing fiber-optic infrastructure. We showcase on-demand storage and retrieval of weak coherent pulses for up to 1 ms, the longest storage time using Er\textsuperscript{3+} reported in the literature. Crucially, our storage protocol operates without involving spin-level transitions, simplifying the system design and improving its robustness. We further showcase a temporal and spectral multimode capacity with selective recall capabilities, essential for a scalable quantum repeater architecture.
Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realizations of photonic quantum information technologies due to the ease of performing single qubit manipulations, the availability of polarization-entangled photon-pair sources, and the possibility of leveraging existing fiber-optic links for distributing qubits over long distances. An optical quantum memory compatible with this platform could serve as a building block for these technologies. Here we present the first experimental demonstration of an atomic quantum memory that directly allows for reversible mapping of quantum states encoded in the polarization degree of freedom of a telecom-wavelength photon. We show that heralded polarization qubits at a telecom wavelength are stored and retrieved with near-unity fidelity by implementing the atomic frequency comb protocol in an ensemble of erbium atoms doped into an optical fiber. Despite remaining limitations in our proof-of-principle demonstration such as small storage efficiency and storage time, our broadband light-matter interface reveals the potential for use in future quantum information processing.
The realization of scalable quantum networks for distribution of entanglement over long distances hinges on quantum repeaters. To outperform the exponential transmission loss in optical fibers, quantum repeaters must employ multiplexing schemes in the temporal, spectral, or spatial domain. The performance of such a multiplexed scheme is contingent on efficient quantum memories offering both extended storage times and large multimode capacities. Towards this goal, we experimentally demonstrate a memory platform operating at telecom wavelength using an Er3+^{3+}3+:Y2_{2}2​SiO5_{5}5​ crystal. We record on-demand storage and recall of weak coherent pulses for up to 111 ms, exceeding by an order of magnitude that of previously reported demonstrations based on Er3+^{3+}3+. The memory exhibits an efficiency of 10.36 % at 300 μμμs storage time with a signal-to-noise ratio of 10.910.910.9, mainly limited by spontaneous emission noise. We also store two spectral modes representing a frequency-bin encoding and retrieve the state with an overlap of 81.8 %. Furthermore, we demonstrate multimode capacity by simultaneously storing 20 temporal and 3 spectral modes with on-demand and selective recall capabilities, serving as a promising step toward a scalable quantum repeater architecture.
Quantum memories at telecom wavelengths are crucial for the construction of large-scale quantum networks based on existing fiber networks. On-demand storage of telecom photonic qubits is an essential request for such networking applications but yet to be demonstrated. Here we demonstrate the storage and on-demand retrieval of telecom photonic qubits using a laser-written waveguide fabricated in an ^{167}Er^{3+}:Y_{2}SiO_{5} crystal. Both ends of the waveguide memory are directly connected with fiber arrays with a fiber-to-fiber efficiency of 51%. Storage fidelity of 98.3(1)% can be obtained for time-bin qubits encoded with single-photon-level coherent pulses, which is far beyond the maximal fidelity that can be achieved with a classical measure and prepared strategy. This device features high reliability and easy scalability, and it can be directly integrated into fiber networks, which could play an essential role in fiber-based quantum networks.
Quantum memory devices with high storage efficiency and bandwidth are essential elements for future quantum networks. Here, we report a storage efficiency greater than 28% in a Tm\mathrm{Tm}Tm3+{}^{3+}3+:YAG crystal (where YAG is yttrium aluminum garnet) at elevated temperatures, achieving this milestone without relying on optical cavities and without compromising memory bandwidth. We introduce different pumping techniques for Tm\mathrm{Tm}Tm-based memories that enable multifrequency-window storage and high memory bandwidth reaching 630 MHz, significantly surpassing previous Tm\mathrm{Tm}Tm-based memory demonstrations, considering the operating temperature of 3.5 K. Furthermore, we propose a general method for large-bandwidth atomic frequency memory using non-Kramers rare-earth ions (REIs) in solids, paving the way for storage efficiencies and bandwidths approaching fundamental limits. The compatibility of Tm\mathrm{Tm}Tm memories with neutral-atom quantum processors and their seamless integration with scalable photonic platforms, such as lithium niobate on insulator, underscore their potential for distributed quantum computing, hybrid quantum networks, and space-based quantum communication. Our study represents a significant advancement toward practical high-performance quantum memories based on REI-doped crystals, where we predict that gigahertz bandwidth and storage efficiencies exceeding 30% are achievable at lower temperatures.