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arXiv:2412.03698 · Physical review. B./Physical review. B

Non-BCS behavior of the pairing susceptibility near the onset of superconductivity in a quantum-critical metal

Ar. Abanov, Shang-Shun Zhang, Andrey V. Chubukov

Published Feb 21, 2025• 3 citations
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Abstract

In a quantum critical metal, superconductivity out of non-Fermi liquid normal state develops only when the pairing interaction exceeds a certain threshold. The authors show here that the dynamic pairing susceptibility exhibits an unexpected behavior: it diverges at the onset of pairing only for a certain subclass of bare/test pairing amplitudes and remains nonsingular for other amplitudes, and below the instability becomes a nonunique function. The authors argue that this behavior reflects a highly non-BCS nature of the pairing at quantum criticality.

DOI
10.1103/physrevb.111.075157

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In a quantum critical metal, superconductivity out of non-Fermi liquid normal state develops only when the pairing interaction exceeds a certain threshold. The authors show here that the dynamic pairing susceptibility exhibits an unexpected behavior: it diverges at the onset of pairing only for a certain subclass of bare/test pairing amplitudes and remains nonsingular for other amplitudes, and below the instability becomes a nonunique function. The authors argue that this behavior reflects a highly non-BCS nature of the pairing at quantum criticality.
We present a simple phenomenological scaling theory for the pairing instability of a quantum critical metal. It can be viewed as a minimal generalization of the classical Bardeen-Cooper-Schrieffer (BCS) theory of superconductivity (SC) for normal Fermi-liquid metals. We assume that attractive interactions are induced in the fermion system by an external ``bosonic glue'' that is strongly retarded. Resting on the small Migdal parameter, all the required information from the fermion system needed to address the superconductivity enters through the pairing susceptibility. Asserting that the normal state is a strongly interacting quantum critical state of fermions, the form of this susceptibility is governed by conformal invariance and one only has the scaling dimension of the pair operator as free parameter. Within this scaling framework, conventional BCS theory appears as the ``marginal'' case but it is now easily generalized to the (ir)relevant scaling regimes. In the relevant regime an algebraic singularity takes over from the BCS logarithm with the obvious effect that the pairing instability becomes stronger. However, it is more surprising that this effect is strongest for small couplings and small Migdal parameters, highlighting an unanticipated important role of retardation. Using exact forms for the finite-temperature pair susceptibility from 1+1D1+1\text{D}1+1D conformal field theory as models, we study the transition temperatures, finding that the gap to transition temperature ratios is generically large compared to the BCS case, showing, however, an opposite trend as a function of the coupling strength compared to the conventional Migdal-Eliashberg theory. We show that our scaling theory naturally produces the superconducting ``domes'' surrounding the quantum critical points (QCPs), even when the coupling to the glue itself is not changing at all. We argue that hidden relations will exist between the location of the crossover lines to the Fermi liquids away from the quantum critical points and the detailed form of the dome when the glue strength is independent of the zero-temperature control parameter. Finally, we discuss the behavior of the orbital-limited upper critical magnetic field as a function of the zero-temperature coupling constant. Compared to the variation in the transition temperature, the critical field might show a much stronger variation pending the value of the dynamical critical exponent.
Near a quantum critical point in a metal, a strong fermion-fermion interaction, mediated by a soft boson, acts in two different directions: it destroys fermionic coherence and it gives rise to an attraction in one or more pairing channels. The two tendencies compete with each other. We analyze a class of quantum critical models, in which momentum integration and the selection of a particular pairing symmetry can be done explicitly, and the competition between non-Fermi liquid and pairing can be analyzed within an effective model with dynamical electron-electron interaction $V({\mathrm{\ensuremath{\Omega}}}_{m})\ensuremath{\propto}1/{|{\mathrm{\ensuremath{\Omega}}}_{m}|}^{\ensuremath{\gamma}}$ (the $\ensuremath{\gamma}$ model). In this paper, the first in the series, we consider the case T=0T=0T=0 and $0<\ensuremath{\gamma}<1$. We argue that tendency to pairing is stronger, and the ground state is a superconductor. We argue, however, that a superconducting state is highly nontrivial as there exists a discrete set of topologically distinct solutions for the pairing gap ${\mathrm{\ensuremath{\Delta}}}_{n}({\ensuremath{\omega}}_{m})$ ($n=0,1,2,...,\ensuremath{\infty}$). All solutions have the same spatial pairing symmetry, but differ in the time domain: ${\mathrm{\ensuremath{\Delta}}}_{n}({\ensuremath{\omega}}_{m})$ changes sign nnn times as a function of Matsubara frequency ${\ensuremath{\omega}}_{m}$. The n=0n=0n=0 solution ${\mathrm{\ensuremath{\Delta}}}_{0}({\ensuremath{\omega}}_{m})$ is sign preserving and tends to a finite value at ${\ensuremath{\omega}}_{m}=0$, like in BCS theory. The $n=\ensuremath{\infty}$ solution corresponds to an infinitesimally small $\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{m})$, which oscillates down to the lowest frequencies as $\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{m})\ensuremath{\propto}|{\ensuremath{\omega}}_{m}{|}^{\ensuremath{\gamma}/2}cos[2\ensuremath{\beta}\phantom{\rule{0.16em}{0ex}}log(|{\ensuremath{\omega}}_{m}|/{\ensuremath{\omega}}_{0})]$, where $\ensuremath{\beta}=O(1)$ and ${\ensuremath{\omega}}_{0}$ is of order of fermion-boson coupling. As a proof, we obtain the exact solution of the linearized gap equation at T=0T=0T=0 on the entire frequency axis for all $0<\ensuremath{\gamma}<1$, and an approximate solution of the nonlinear gap equation. We argue that the presence of an infinite set of solutions opens up a new channel of gap fluctuations. We extend the analysis to the case where the pairing component of the interaction has additional factor 1/N1/N1/N and show that there exists a critical Ncr>1{N}_{cr}>1Ncr​>1, above which superconductivity disappears, and the ground state becomes a non-Fermi liquid. We show that all solutions develop simultaneously once NNN gets smaller than Ncr{N}_{cr}Ncr​.
We revisit the issue of superconductivity at the quantum-critical point (QCP) between a 2D paramagnet and a spin-density-wave metal with ordering momentum (π, π). This problem is highly nontrivial because the system at criticality displays a non-Fermi-liquid behavior and because the effective coupling constant λ for the pairing is generally of order one, even when the actual interaction is smaller than fermionic bandwidth. Previous study [M. A. Metlitski and S. Sachdev, Phys. Rev. B 82, 075128 (2010)] has found that the renormalizations of the pairing vertex are stronger than in BCS theory and hold in powers of log(2)(1/T). We analyze the full gap equation and argue that summing up of the leading logarithms does not lead to a pairing instability. Yet, we show that superconductivity has no threshold and appears even if λ is set to be small, because subleading logarithmical renormalizations diverge and give rise to a BCS-like result log1/T(c) ∝ 1/λ. We argue that the analogy with BCS is not accidental as at small λ superconductivity at a QCP predominantly comes from fermions that retain Fermi-liquid behavior at criticality. We compute T(c) for the actual λ ∼ O(1), and find that both Fermi-liquid and non-Fermi-liquid fermions contribute to the pairing.
We analyze the possibility of odd-frequency pairing near a quantum critical point(QCP) in a metal. We consider a model with dynamical pairing interaction $V({\mathrm{\ensuremath{\Omega}}}_{n})\ensuremath{\sim}1/{|{\mathrm{\ensuremath{\Omega}}}_{n}|}^{\ensuremath{\gamma}}$ (the $\ensuremath{\gamma}$ model). This interaction gives rise to a non-Fermi liquid in the normal state and is attractive for pairing. The two trends compete with each other. We search for odd-frequency solutions for the pairing gap $\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{m})=\ensuremath{-}\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{m})$. We show that for $\ensuremath{\gamma}<1$, odd-frequency superconductivity loses the competition with a non-Fermi liquid and does not develop. We show that the pairing does develop in the extended model in which interaction in the pairing channel is larger than the one in the particle-hole channel. For $\ensuremath{\gamma}>1$, we argue that the original model is at the boundary towards odd-frequency pairing and analyze in detail how superconductivity is triggered by a small external perturbation. In addition, we show that for $\ensuremath{\gamma}>2$, the system gets frozen at the critical point towards pairing in a finite range in the parameter space. This gives rise to highly unconventional phase diagrams with flat regions.
Near a quantum-critical point in a metal strong fermion-fermion interaction mediated by a soft collective boson gives rise to incoherent, non-Fermi liquid behavior. It also often gives rise to superconductivity which masks the non-Fermi liquid behavior. We analyze the interplay between the tendency to pairing and fermionic incoherence for a set of quantum-critical models with effective dynamical interaction between low-energy fermions. We argue that superconducting T_{c} is nonzero even for strong incoherence and/or weak interaction due to the fact that the self-energy from dynamic critical fluctuations vanishes for the two lowest fermionic Matsubara frequencies ω_{m}=±πT. We obtain the analytic formula for T_{c}, which reproduces well earlier numerical results for the electron-phonon model at vanishing Debye frequency.
This paper is a continuation and a partial summary of our analysis of the pairing at a quantum-critical point (QCP) in a metal for a set of quantum-critical systems, whose low-energy physics is described by an effective model with dynamical electron-electron interaction $V({\mathrm{\ensuremath{\Omega}}}_{m})=(\overline{g}/|{\mathrm{\ensuremath{\Omega}}}_{m}{|)}^{\ensuremath{\gamma}}$ (the $\ensuremath{\gamma}$ model). Examples include pairing at the onset of various spin and charge-density-wave and nematic orders and pairing in SYK-type models. In previous papers, we analyzed the physics for $\ensuremath{\gamma}<2$. We have shown that the onset temperature for the pairing Tp{T}_{p}Tp​ is finite, of order g‾\overline{g}g​, yet the gap equation at T=0T=0T=0 has an infinite set of solutions within the same spatial symmetry. As the consequence, the condensation energy Ec{E}_{c}Ec​ has an infinite number of minima. The spectrum of Ec{E}_{c}Ec​ is discrete, but becomes more dense as $\ensuremath{\gamma}$ increases. Here we consider the case $\ensuremath{\gamma}=2$. The $\ensuremath{\gamma}=2$ model attracted special interest in the past as it describes the pairing by an Einstein phonon in the limit when the dressed phonon mass ${\ensuremath{\omega}}_{D}$ vanishes. We show that for $\ensuremath{\gamma}=2$, the spectrum of Ec{E}_{c}Ec​ becomes continuous. We argue that the associated gapless ``longitudinal'' fluctuations destroy superconducting phase coherence at a finite TTT, such that at 0<T<Tp0<T<{T}_{p}0<T<Tp​, the system displays pseudogap behavior of preformed pairs. We show that for each gap function from the continuum spectrum, there is an infinite array of dynamical vortices in the upper half-plane of frequency. For the electron-phonon case, our results show that Tp=0.1827g‾{T}_{p}=0.1827\overline{g}Tp​=0.1827g​, obtained in earlier studies, marks the onset of the pseudogap behavior, while the actual superconducting Tc{T}_{c}Tc​ vanishes at ${\ensuremath{\omega}}_{D}\ensuremath{\rightarrow}0$.