Continuous time crystals (CTCs) are a phase of matter characterized by spontaneous breaking of continuous time-translation symmetry. Recently, CTCs have garnered interest due to breakthroughs in experimental implementation. Here we report the experimental observation of CTCs in noble-gas nuclear spins and uncover previously unexplored dynamical phenomena. We observe that the CTCs manifest as persistent limit cycle oscillations of nuclear spins, with coherence times exceeding hours. Notably, these oscillations are robust against noise perturbations and exhibit random time phases upon repetitive realization, epitomizing continuous time-translation symmetry-breaking intrinsic to CTCs. Additionally, we observe a dynamical phase featuring quasi-periodic oscillations and random time phases, indicating the emergence of the continuous time quasi-crystals proposed by recent theories. By varying the feedback strength and magnetic gradient, we observe complex dynamical phase transitions between time crystal phases and chaotic regimes. This work broadens the catalog of phases of spin gases and unlocks opportunities in precision measurements. The authors report on the observation of continuous time crystals of nuclear spins of 129Xe atoms within a Rb-Xe gaseous mixture in a magnetic feedback scheme. This unveils nontrivial role of magnetic fields and a new continuous time quasi-crystal phase.
Continuous time crystals (CTCs) are a phase of matter characterized by spontaneous breaking of continuous time-translation symmetry. Recently, CTCs have garnered interest due to breakthroughs in experimental implementation. Here we report the experimental observation of CTCs in noble-gas nuclear spins and uncover previously unexplored dynamical phenomena. We observe that the CTCs manifest as persistent limit cycle oscillations of nuclear spins, with coherence times exceeding hours. Notably, these oscillations are robust against noise perturbations and exhibit random time phases upon repetitive realization, epitomizing continuous time-translation symmetry-breaking intrinsic to CTCs. Additionally, we observe a dynamical phase featuring quasi-periodic oscillations and random time phases, indicating the emergence of the continuous time quasi-crystals proposed by recent theories. By varying the feedback strength and magnetic gradient, we observe complex dynamical phase transitions between time crystal phases and chaotic regimes. This work broadens the catalog of phases of spin gases and unlocks opportunities in precision measurements. The authors report on the observation of continuous time crystals of nuclear spins of 129Xe atoms within a Rb-Xe gaseous mixture in a magnetic feedback scheme. This unveils nontrivial role of magnetic fields and a new continuous time quasi-crystal phase.
Spontaneous symmetry breaking plays a pivotal role in physics ranging from the emergence of elementary particles to the phase transitions of matter. The spontaneous breaking of continuous time translation symmetry leads to a novel state of matter named continuous time crystal (CTC). It exhibits periodic oscillation without the need for periodic driving, and the relative phases for repetitively realized oscillations are random. However, the mechanism behind the spontaneous symmetry breaking in CTCs, particularly the random phases, remains elusive. Here we propose and experimentally realize two types of CTCs based on distinct mechanisms: manifold topology and near-chaotic motion. We observe both types of CTCs in thermal atomic ensembles by artificially synthesizing spin-spin nonlinear interactions through a measurement-feedback scheme. Our work provides general recipes for the realization of CTCs, and paves the way for exploring CTCs in various systems.
Time crystals are classified as discrete or continuous depending on whether they spontaneously break discrete or continuous time translation symmetry. Although discrete time crystals have been extensively studied in periodically driven systems, the experimental realization of a continuous time crystal is still pending. We report the observation of a limit cycle phase in a continuously pumped dissipative atom-cavity system that is characterized by emergent oscillations in the intracavity photon number. The phase of the oscillation was found to be random for different realizations, and hence, this dynamical many-body state breaks continuous time translation symmetry spontaneously. Furthermore, the observed limit cycles are robust against temporal perturbations and therefore demonstrate the realization of a continuous time crystal.
Nonlinear spin systems exhibit rich and exotic dynamical phenomena, offering promising applications ranging from spin masers and time crystals to precision measurement. Recent theoretical work [T. Wang et al., Commun. Phys. 8, 41 (2025)] predicted intriguing nonlinear dynamical phases arising from inhomogeneous magnetic fields and feedback interactions. However, experimental exploration of these predictions remains lacking. Here, we report the observation of nonlinear spin dynamics in dual-bias magnetic fields with dual-cell alkali-metal atomic gases and present three representative stable dynamical behaviors of limit cycles, quasi-periodic orbits, and chaos. Additionally, we probe the nonlinear phase transitions between these phases by varying the feedback gain and the difference of dual-bias magnetic fields. Furthermore, we demonstrate the robustness of the limit cycle and quasi-periodic orbit against the noise of magnetic fields. Our findings establish a versatile platform for exploring complex spin dynamics and open new avenues for the realization of multimode spin masers, time crystals and quasi-crystals, and high-precision magnetometers.
Time crystals are a nonequilibrium phase of matter that extend fundamental spontaneous symmetry breaking into the temporal dimension, typically requiring external driving for their realization. Here, we explore the nonequilibrium phase diagram of a two-dimensional dissipative Heisenberg spin system without external coherent or incoherent driving. Through numerical analysis of spin dynamics, we identify nonstationary steady states, some of which are limit cycles with persistent periodic oscillations, while others exhibit chaotic, aperiodic behavior. The emergence of limit cycle steady states breaks the continuous time-translation symmetry of this time-independent many-body system, classifying them as continuous time crystals. We further validate these oscillatory behaviors by testing their stability against local perturbations and assess the robustness of the emergent continuous time crystals by introducing isotropic Gaussian white noise. This work provides insights into the intricate interplay between the dissipation and spin interaction, and opens possibilities for realizing dissipation-induced, heating-immune time crystals. Time crystals represent a nonequilibrium phase of matter without an equilibrium counterpart. The authors investigate the nonequilibrium steadystate phase diagram of a two-dimensional dissipative Heisenberg model in the absence of driving, and identify a continuous time crystalline phase exhibiting persistent oscillations in time.
While a generic open quantum system decays to its steady state, continuous time crystals (CTCs) develop spontaneous oscillation and never converge to a stationary state. Just as crystals develop correlations in space, CTCs do so in time. Here, we introduce a continuous quasi time crystals (CQTC). Despite being characterized by the presence of nondecaying oscillations, this phase does not retain its long-range order, making it time analogous to quasicrystal structures. We investigate the emergence of this phase in a minimal model, made of two coupled collective spin subsystems, each developing a CTC phase upon the action of a strong enough drive. The addition of a coupling enables the emergence of different synchronized phases, where both subsystems oscillate at the same frequency. In the transition between different CTC orders, the system develops chaotic dynamics with aperiodic oscillations. These chaotic features differ from those of closed quantum systems, as the dynamics is not characterized by a unitary evolution. We investigate the connection between chaos and this quasicrystalline phase using mean-field techniques, and we confirm these results by including quantum fluctuations at the lowest order.
Nonlinear spin dynamics are essential in exploring nonequilibrium quantum phenomena and have broad applications in precision measurement. Among these systems, the combination of a bias magnetic field and feedback mechanisms can induce self-sustained oscillations at the base Larmor frequency due to nonlinearity. These features have driven the development of single-species and multiple-species spin masers. The latter, with multiple discrete Larmor frequencies, provides significant advantages for precision measurement by mitigating uncertainties in precession frequencies due to long-term drifts in experimental conditions. The self-sustained oscillations of single-species and multiple-species spin masers correspond to limit cycles and quasi-periodic orbits of the stable nonlinear dynamics of the systems, respectively; the correspondence is elucidated in a recent study on a related spin system featuring two discrete intrinsic Larmor frequencies under dual bias magnetic fields [T. Wang et al., Commun. Phys. 8, 41 (2025)]. Here, we extend the study to the case where the intrinsic Larmor frequencies of individual spins of the system, given rise to by an inhomogeneous bias magnetic field, form a continuum. We show that generically the stable dynamics of the system includes limit cycles, quasi-periodic orbits, and chaos. We establish the relation between the synchronization frequency of limit cycles and the field inhomogeneity and derive an equation determining the stability of limit cycles. Furthermore, detailed characteristics of different dynamical phases, especially the robustness of limit cycles and quasi-periodic orbits against experimental fluctuations, are discussed. Our findings not only encompass the case of discrete Larmor frequencies, but also provide crucial insights for precision measurement and the exploration of continuous time crystals and quasi-crystals.