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arXiv:2411.18570 · Journal of Quantitative Spectroscopy and Radiative Transfer

Frequency redistribution and step-size distribution of light scattered by atomic vapor: Applications to Lévy flight random walk

I.C. Nunes, M. Araujo, J. P. Lopez, Thierry Passerat de Silans

Published May 4, 2025• 3 citations
arXivHTMLPDF
DOI
10.1016/j.jqsrt.2025.109481

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We experimentally investigate the transmission of light by dense atomic vapor. The light propagating in dense atomic vapor can be modeled as a Lévy flight random walk. For such system, the step-length distribution can be modeled as P(ℓ)∼ℓ−1−α(ℓ)P(\ell)\sim \ell^{-1-α(\ell)}P(ℓ)∼ℓ−1−α(ℓ), with the Lévy index α(ℓ)α(\ell)α(ℓ) varying smoothly with the step length. Moreover, the walkers alternate between two distinct distributions depending on the occurrence of collisions between atoms in the light scattering. We obtain the Lévy index from transmission measurements for different system sizes and atomic densities. The measured Lévy index is determined by the system size α=α(ℓ=L)α=α(\ell=L)α=α(ℓ=L). Simulations are made for walkers alternating between two Lévy like step-length
The propagation of a photon in an atomic medium can be seen as a L\'evy-flight random walk where the probability distribution P(z)P(z)P(z) for the photon step length zzz scales with ${z}^{\ensuremath{-}(\ensuremath{\alpha}+1)}$, with $0<\ensuremath{\alpha}<2$. In atomic vapors, previous work reported the value of $\ensuremath{\alpha}$ obtained from direct measurement of P(z)P(z)P(z) and also from the dependence of transmission on sample opacity, both for Doppler and Lorentz profiles. In this work, we report the measurement of $\ensuremath{\alpha}$ in a Cs cell from the scaling of transmission with starting point, i.e., the average penetration depth of the photon in the medium before the first scattering event. We show that the parameter $\ensuremath{\alpha}$ depends on the size of the system and on the probability that an atom suffers a collision before spontaneous emission. The measured $\ensuremath{\alpha}$ parameter corresponds to the expectation value for P(z=L)P(z=L)P(z=L), with LLL the size of the system, which is consistent with the so-called single-big-jump principle that states that a single jump rules the transport.
The propagation of light in a resonant atomic vapor can a priori be thought of as a multiple scattering process, in which each scattering event redistributes both the direction and the frequency of the photons. Particularly, the frequency redistribution may result in L\'evy flights of photons, directly affecting the transport properties of light in a resonant atomic vapor and turning this propagation into a superdiffusion process. Here, we report on a Monte Carlo simulation developed to study the evolution of the spectrum of the light in a resonant thermal vapor. We observe the gradual change of the spectrum and its convergence towards a regime of complete frequency redistribution as the number of scattering events increases. We also analyze the probability density function of the step length of photons between emissions and reabsorptions in the vapor, which governs the statistics of the light diffusion. We observe two different regimes in the light transport: superdiffusion when the vapor is excited near the line center and normal diffusion for excitation far from the line center. The regime of complete frequency redistribution is not reached for excitation far from resonance even after many absorption and reemission cycles due to correlations between emitted and absorbed frequencies.