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arXiv:2410.19592 · Physical Review Applied

High-impedance resonators for strong coupling to an electron on helium

Gerwin Koolstra, E. O. Glen, N. R. Beysengulov, Heejun Byeon, Kyle E. Castoria, Michael J. Sammon, Brennan Dizdar, C. S. Wang, David Schuster, S. A. Lyon, J. Pollanen, D. G. Rees

Published Feb 3, 2025• 7 citations
arXivHTMLPDF

Abstract

The in-plane motion of an electron on helium can couple to superconducting microwave resonators via electrical dipole coupling, offering a robust and rapid readout scheme. In previous efforts, microwave resonator designs for electrons on helium have lacked the coupling strength to reach the strong coupling regime, where coherent quantum effects outlast both electron and resonator decoherence rates. High-impedance superconducting microwave resonators offer a path to strong coupling, but integrating such resonators with electrons on helium remains an outstanding challenge. Here, we introduce a high-impedance resonator design compatible with strong coupling to electrons on helium. We fabricate and measure titanium nitride resonators with median internal quality factors of $3.9\ifmmode\times\else\texttimes\fi{}{10}^{5}$ and average impedance of 2.5 $\mathrm{k}\mathrm{\ensuremath{\Omega}}$, promising a sevenfold increase in coupling strength compared with standard 50-$\mathrm{\ensuremath{\Omega}}$ resonators. In addition, we develop a simplified resonator model from the capacitance matrix and sheet inductance that accurately predicts the mode frequencies, significantly simplifying the design process of future resonators for investigating quantum effects with electrons on helium.

DOI
10.1103/physrevapplied.23.024001

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The in-plane motion of an electron on helium can couple to superconducting microwave resonators via electrical dipole coupling, offering a robust and rapid readout scheme. In previous efforts, microwave resonator designs for electrons on helium have lacked the coupling strength to reach the strong coupling regime, where coherent quantum effects outlast both electron and resonator decoherence rates. High-impedance superconducting microwave resonators offer a path to strong coupling, but integrating such resonators with electrons on helium remains an outstanding challenge. Here, we introduce a high-impedance resonator design compatible with strong coupling to electrons on helium. We fabricate and measure titanium nitride resonators with median internal quality factors of 3.9\ifmmode×\else\texttimes\fi1053.9\ifmmode\times\else\texttimes\fi{}{10}^{5}3.9\ifmmode×\else\texttimes\fi105 and average impedance of 2.5 k\ensuremathΩ\mathrm{k}\mathrm{\ensuremath{\Omega}}k\ensuremathΩ, promising a sevenfold increase in coupling strength compared with standard 50-\ensuremathΩ\mathrm{\ensuremath{\Omega}}\ensuremathΩ resonators. In addition, we develop a simplified resonator model from the capacitance matrix and sheet inductance that accurately predicts the mode frequencies, significantly simplifying the design process of future resonators for investigating quantum effects with electrons on helium.
The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer.Circuit quantum electrodynamics allows strong dipole coupling between electrons and a high-Q superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom.Here, we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator.The high finesse of the resonator allows us to observe large dispersive shifts that are many times the linewidth and make fast and sensitive measurements on the collective vibrational modes of the electron ensemble, as well as the superfluid helium film underneath.Furthermore, a large ensemble coupling is observed in the dispersive regime during experiment, and it shows excellent agreement with our numeric model.The coupling strength of the ensemble to the cavity is found to be ≈1 MHz per electron, indicating the feasibility of achieving single electron strong coupling.
The quest towards precise measurement and control of quantum mechanical systems is behind many if not most of the advances in mesoscopic physics in the recent years. This thesis follows that tradition, and describes the first realization of a hybrid circuit integrating electrons on helium (EonHe) with the circuit quantum electrodynamics (cQED) architecture. In this hybrid architecture, the quantized lateral motion of the electrons strongly couples with the transverse electric field inside a high-Q superconducting resonator, enabling sensitive detection and manipulation of the electron's in-plane motion degree of freedom. Such architecture also provide a plausible road map towards using the spin degrees of freedom of the electrons as a quantum memory. Our hope is to establish a novel model system for quantum control and manipulation, where the uncanny similarity between the electron hamiltonian and the strong coulomb interactions could give rise to unparallelly rich quantum phenomena. In our first experiment towards this goal, we demonstrate strong dispersive coupling between ∼105\sim 10^5∼105 electrons and a superconducting co-planar waveguide resonator. The effort of the second experiment focuses on bringing down this number to just a few electrons in an isolated trap. The CPW resonator was replaced by a quarter-wavelength strip-line resonator with one side terminated by a short (``the tuning fork"). This design changes the microwave mode that is visible to the electron dipole interaction, improves the coupling strength, and opens up the geometry for more sophisticated DC controls isolating an individual electron. The third experiment implements such DC control scheme, and manages to trap just a single electron in a small trap. This small electron trap is defined by multiple DC electrodes near the open-end of the tuning fork. The overall circuit design resembles those seen in the quantum dot community. Much effort was spent on hitting the tight space between the dispersive constraints of the cQED measurement scheme and the increasing complication of the sample. Single or few electron spectra are measured, and we provided an upper estimate on the acoustically broadened electron line-width, together with design changes that reduce the line-width of the electron states.
Electrons on helium form a unique two-dimensional system on the interface of superfluid 4^44He and vacuum. At low temperatures and weak confinement, trapped electrons can arrange into strongly correlated states known as Wigner molecules, which can be used to study electron interactions in the absence of disorder, or as a promising resource for quantum computation. Wigner molecules have orbital frequencies in the microwave regime and can therefore be integrated with circuit quantum electrodynamics, which would allow rapid detection and manipulation of such a molecule's orbital state. In this thesis, we demonstrate deterministic preparation of one to four-electron Wigner molecules in an electron-on-helium quantum dot located at the tip of an on-chip microwave resonator. The Wigner molecule dipole coupling to the resonator allows us to measure spectral features of Wigner molecules in the microwave regime. We find that different-sized Wigner molecules have strikingly different spectra, and each spectrum serves as a fingerprint for the molecule's internal structure and its surroundings. By modeling the electron-cavity system, we extract each molecule's orbital frequency and electron configuration. For a single electron, the orbital frequency crosses the cavity resonance and we measure a large coherent electron-photon coupling rate of g/2π=4.8g/2\pi = 4.8g/2π=4.8 MHz, which exceeds the incoherent cavity decay rate by ten times. These results provide a solid base for the development of an electron-on-helium qubit. Looking forward, our platform allows for new microwave studies of strongly correlated electron states and can be used to couple a single microwave photon to a single electron spin.
The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer.Circuit quantum electrodynamics allows strong dipole coupling between electrons and a high-Q superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom.Here, we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator.The high finesse of the resonator allows us to observe large dispersive shifts that are many times the linewidth and make fast and sensitive measurements on the collective vibrational modes of the electron ensemble, as well as the superfluid helium film underneath.Furthermore, a large ensemble coupling is observed in the dispersive regime during experiment, and it shows excellent agreement with our numeric model.The coupling strength of the ensemble to the cavity is found to be ≈1 MHz per electron, indicating the feasibility of achieving single electron strong coupling.
Superconducting resonators with high-kinetic inductance play a central role in hybrid quantum circuits, enabling strong coupling with quantum systems with small electric dipole moment and improved parametric amplification. However, optimizing these resonators simultaneously for high internal quality factors (QiQ_iQi​) and resilience to strong magnetic fields remains challenging. In this study, we systematically compare superconducting resonators fabricated from niobium nitride (NbN) and granular aluminum (grAl) thin films, each having similar kinetic inductance values (Lk∼100L_k \sim 100Lk​∼100 pH/sq). At zero magnetic field, resonators made from grAl exhibit higher QiQ_iQi​ compared to their NbN counterparts. However, under applied magnetic fields, NbN resonators demonstrate significantly better resilience. Moreover, NbN resonators exhibit an unexpected increase in QiQ_iQi​ at intermediate in-plane magnetic fields (B∥∼1B_{\parallel} \sim 1B∥​∼1 T), which we attribute to an enhanced frequency detuning that reduce coupling to two-level system defects. In contrast, grAl resonators show a distinct critical field above which QiQ_iQi​ rapidly decreases, strongly depending on resonator cross-section respect to the applied field direction. Characterization of the nonlinear properties at zero magnetic field reveals that the self-Kerr coefficient in grAl resonators is more than an order of magnitude higher than in NbN resonators, making grAl particularly attractive for applications requiring pronounced nonlinear interactions. Our findings illustrate a clear trade-off between the two materials: NbN offers superior magnetic-field resilience beneficial for hybrid circuit quantum electrodynamics applications, while grAl is more advantageous in low-field regimes demanding high impedance and strong nonlinearity.
Aluminum-based platforms have allowed to reach major milestones for superconducting quantum circuits. For the next generation of devices, materials that are able to maintain low microwave losses while providing new functionalities, such as large kinetic inductance or compatibility with CMOS platform, are needed. Here, we report on a combined direct current and microwave investigation of titanium nitride films of different thicknesses grown using CMOS compatible methods. For microwave resonators made of 3 nm thick TiN, we measured large kinetic inductance LK ∼240 pH/sq, high mode impedance of ∼4.2 kΩ while maintaining microwave quality factor ∼105 in the single photon limit. We present an in-depth study of the microwave loss mechanisms in these devices that indicates the importance of quasiparticles and provide insight for further improvement.