The interplay of spin and charge degrees of freedom is believed to underlie various unresolved phenomena in strongly correlated systems. Quantum simulators based on neutral atoms provide an excellent testbed for investigating such phenomena and resolving their microscopic origins. Up to now, the majority of experimental and theoretical studies has focused on systems with fermionic exchange statistics. Here we expand the existing cold atom toolbox through the use of negative temperature states, enabling us to realize an antiferromagnetic, bosonic $t-J$ model in two spatial dimensions, subject to a strong staggered magnetic field in a quantum gas microscope. Through comparison of the spreading dynamics of a single hole in a Néel versus a spin-polarized initial state, we establish the relevance of memory effects resulting from the buildup of strong spin-charge correlations in the dynamics of charge carriers in antiferromagnets. We further numerically predict rich dynamics of pairs of doped holes, which we demonstrate to be bound by a similar memory effect, while their center-of-mass can expand freely. Our work paves the way for the systematic exploration of the effect of antiferromagnetic spin ordering on the properties of individual charge carriers as well as finite doping phases: Our study demonstrates that the staggered field can be used to single out the effect of antiferromagnetism and holds the prospect to prepare low-temperature states in the near future.
The interplay of spin and charge degrees of freedom is believed to underlie various unresolved phenomena in strongly correlated systems. Quantum simulators based on neutral atoms provide an excellent testbed for investigating such phenomena and resolving their microscopic origins. Up to now, the majority of experimental and theoretical studies has focused on systems with fermionic exchange statistics. Here we expand the existing cold atom toolbox through the use of negative temperature states, enabling us to realize an antiferromagnetic, bosonic t−J model in two spatial dimensions, subject to a strong staggered magnetic field in a quantum gas microscope. Through comparison of the spreading dynamics of a single hole in a Néel versus a spin-polarized initial state, we establish the relevance of memory effects resulting from the buildup of strong spin-charge correlations in the dynamics of charge carriers in antiferromagnets. We further numerically predict rich dynamics of pairs of doped holes, which we demonstrate to be bound by a similar memory effect, while their center-of-mass can expand freely. Our work paves the way for the systematic exploration of the effect of antiferromagnetic spin ordering on the properties of individual charge carriers as well as finite doping phases: Our study demonstrates that the staggered field can be used to single out the effect of antiferromagnetism and holds the prospect to prepare low-temperature states in the near future.
Unraveling the microscopic mechanisms governing the physics of doped quantum magnets is key to advancing our understanding of strongly correlated quantum matter. Quantum simulation platforms, e.g., ultracold atoms in optical lattices or tweezer arrays, provide a powerful tool to investigate the interplay between spin and charge motion in microscopic detail. Here, in a twist, we disentangle the role of particle statistics from the physics of strong correlations by exploring the strong coupling limit of doped bosonic quantum magnets, specifically the antiferromagnetic (AFM) bosonic t − J model. Using large-scale density matrix renormalization group calculations, we map out the phase diagram on the two-dimensional square lattice at finite doping. In the low-doping regime, bosonic holes form partially filled stripes, akin to those observed in high- T c cuprates. As doping increases, a transition occurs to a partially polarized ferromagnetic (FM) phase, driven by the motion of mobile bosonic charge carriers forming Nagaoka polarons. At high doping or large t / J , the system evolves into a fully polarized FM. These findings shed light on the role of particle statistics in strongly correlated many-body systems, revealing connections to stripe formation and the physics of kinetic (Nagaoka-type) ferromagnetism. Our results may be realized in state-of-the-art quantum simulation platforms, including bosonic quantum gas microscopes, Rydberg atom tweezer arrays, and ultracold polar molecules, paving the way for future experimental studies of doped bosonic quantum magnets.
Obtaining a microscopic understanding of the dynamics in strongly correlated electronic systems has remained a challenge for many decades. The interplay between the spin and charge degrees of freedom in these materials at different temperatures and dopant concentrations is not well understood and is still an area of intense scientific research. Recently, quantum simulators based on ultracold atoms in optical lattices have emerged as a promising platform to probe strongly correlated fermionic systems. This thesis reports on the work carried out with a quantum gas microscope of ultracold fermionic Li-6, where Fermi-Hubbard systems are prepared and imaged with single site spin and density resolution. The main results of the thesis explore the microscopic dynamics underlying one-dimensional materials, where individual constituents such as the electron with charge e and spin-1/2 are not relevant to the description of the system anymore and are instead replaced by spin and charge excitations that can propagate independent of one another - a phenomenon called spin-charge separation. In our quantum simulator, we use analogous one-dimensional Fermi-Hubbard chains of Li-6, to perform time- and space-resolved microscopy of the spin and charge excitations following a local quench. By extracting their strikingly different velocities and showing an absence of binding between the excitations, we demonstrate spin-charge separation. Our microscopic technique also allows us to quantitatively extract the excess spin carried by the spin excitiation, connecting our results to the phenomenon of fractionalization. In another set of experiments, Fermi-Hubbard chains are probed at equilibrium and incommensurate spin correlations arising in the presence of both density doping and spin polarization are observed. The wavevector of these incommensurate correlations are found to have a linear dependence on doping and polarization. Finally, the effect of the spin-charge interplay is probed in the crossover from one to two dimensions. The spin correlations across dopants are seen to be dramatically different in two dimensions, and the strong antiferromagnetic correlations across dopants present in one dimension disappear. For a single dopant in a fully two dimensional system, the spin-charge interplay manifests as a distorted spin cloud surrounding the dopant, indicating the formation of a magnetic polaron. The experiments reported here demonstrate the power of a quantum simulator; by probing the physics of strongly correlated systems in real space with unprecedented resolution, we can zoom into emergent phenomena, validate theories and access regimes that are not possible in other experimental settings.
The mechanism underlying charge transport in strongly correlated quantum systems, such as doped antiferromagnetic Mott insulators, remains poorly understood. Here, we study the expansion dynamics of an initially localized hole inside a two-dimensional (2D) Ising antiferromagnet at variable temperature. Using a combination of classical Monte Carlo and truncated-basis methods, we reveal two dynamically distinct regimes: a spin-charge confined region below a critical temperature T∗, characterized by slow spreading, and a spin-charge deconfined region above T∗, characterized by an unbounded diffusive expansion. The deconfinement temperature ${T}^{*}\ensuremath{\approx}0.65{J}_{z}$ we find is around the N\'eel temperature TN=0.567Jz of the Ising background in 2D, but we expect T∗<TN in higher dimensions. In both regimes we find that the mobile hole does not thermalize with the Ising spin background on the considered time scales, indicating weak effective coupling of spin and charge degrees of freedom. Our results can be qualitatively understood by an effective parton model and can be tested experimentally in state-of-the-art quantum gas microscopes.
It is a widely accepted view that the interplay of spin and charge degrees of freedom in doped antiferromagnets (AFMs) gives rise to the rich physics of high-temperature superconductors. Nevertheless, it remains unclear how effective low-energy degrees of freedom and the corresponding field theories emerge from microscopic models, including $t\ensuremath{-}J$ and Hubbard Hamiltonians. A promising view comprises that the charge carriers have a rich internal parton structure on intermediate scales, but the interplay of the emergent partons with collective magnon excitations of the surrounding AFM remains unexplored. Here we study a doped one-dimensional spin chain in a staggered magnetic field and demonstrate that it supports a zoo of various long-lived excitations. These include magnons, mesonic pairs of spinons and chargons along with their rovibrational excitations, and tetra-parton bound states of mesons and magnons. We identify these types of quasiparticles in various spectra using density-matrix renormalization group simulations. Moreover, we introduce a strong-coupling theory describing the polaronic dressing and molecular binding of mesons to collective magnon excitations. The effective theory can be solved by standard tools developed for polaronic problems and can be extended to study similar physics in two-dimensional doped AFMs in the future. Experimentally, the doped spin-chain in a staggered field can be directly realized in quantum gas microscopes.
Exotic phenomena in strongly correlated electron systems emerge from the interplay between spin and motional degrees of freedom. For example, doping an antiferromagnet is expected to give rise to pseudogap states and high-temperature superconductors. Quantum simulation with ultracold fermions in optical lattices offers the potential to answer open questions about the doped Hubbard Hamiltonian, and has recently been advanced by quantum gas microscopy. In order to take advantage of these possibilities, a stable, high-power, 2D square lattice system was developed and coupled with an image plane based spatial light modulator. The ability to finely tune the atomic potential has made it possible to realize an antiferromagnet in a repulsively interacting Fermi gas on a 2D square lattice. At our lowest temperatures of T/t=0.25(2), antiferromagnetic long-range order (LRO) manifests through the divergence of the correlation length that reaches the size of the system, the development of a peak in the spin structure factor and a value of the staggered magnetization approaching the ground state value. Similarly, by carefully shaping the confinement, we have produced ultra-low entropy band insulators, which promise to be a perfect starting point for more advanced cooling schemes. In addition to the production of new states, Fermi gas microscopy is superbly well suited to studies of many-body dynamics. To this end I report on preliminary measurements of the propagation of holes in a Mott insualtor. These results demonstrate that Fermi gas microscopy can address open questions on the low-temperature Hubbard model.
The combination of optical tweezer arrays with strong interactions-via dipole exchange of molecules and Van der Waals interactions of Rydberg atoms-has opened the door for the exploration of a wide variety of quantum spin models. A next significant step will be the combination of such settings with mobile dopants. This will enable one to simulate the physics believed to underlie many strongly correlated quantum materials. Here, we propose an experimental scheme to realize bosonic t-J models via encoding the local Hilbert space in a set of three internal atomic or molecular states. By engineering antiferromagnetic (AFM) couplings between spins, competition between charge motion and magnetic order similar to that in high-T_{c} cuprates can be realized. Since the ground states of the 2D bosonic AFM t-J model we propose to realize have not been studied extensively before, we start by analyzing the case of two dopants-the simplest instance in which their bosonic statistics plays a role-and compare our results to the fermionic case. We perform large-scale density matrix renormalization group calculations on six-legged cylinders, and find a strong tendency for bosonic holes to form stripes. This demonstrates that bosonic, AFM t-J models may contain similar physics as the collective phases in strongly correlated electrons.