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arXiv:2410.17710

Quantum correlations of the photon fields in a waveguide quantum electrodynamics

Ya. S. Greenberg. O. A. Chuikin, Aleksey G. Moiseev, Alexander A. Shtygashev

Published Oct 23, 2024• 0 citations
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Abstract

We present a time-dependent quantum calculations of the first order and second order photon correlation functions for the scattering of a single-photon pulse on a two-level atom (qubit) embedded in a one-dimensional open waveguide. Within Markov approximation we find the analytic expression for the quantum operator of positive frequency electric field. We restricted Hilbert space of initial states by the states with one and two excitations and show that the photon probability amplitudes are given by the off-diagonal matrix elements of the electric field operator between these states. For two-excitation initial state where the atom is excited and there exists a single photon in a waveguide we calculate the second order correlation function which describes the measurements by two detectors at two different space-time points. The second order correlation function exhibits the interference term showing that the measurements of two detectors are correlated. This interference is similar to that found in the Hanbury Brown and Twiss correlation experiment with two indistinguishable photons.

DOI
10.48550/arxiv.2410.17710

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We present a time-dependent quantum calculations of the first order and second order photon correlation functions for the scattering of a single-photon pulse on a two-level atom (qubit) embedded in a one-dimensional open waveguide. Within Markov approximation we find the analytic expression for the quantum operator of positive frequency electric field. We restricted Hilbert space of initial states by the states with one and two excitations and show that the photon probability amplitudes are given by the off-diagonal matrix elements of the electric field operator between these states. For two-excitation initial state where the atom is excited and there exists a single photon in a waveguide we calculate the second order correlation function which describes the measurements by two detectors at two different space-time points. The second order correlation function exhibits the interference term showing that the measurements of two detectors are correlated. This interference is similar to that found in the Hanbury Brown and Twiss correlation experiment with two indistinguishable photons.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.
For a one-dimensional (1D) waveguide coupled to two or three qubits, we show that the photon-photon correlations have a wide variety of behavior, with structure that depends sensitively on the frequency and on the qubit-qubit separation L. We study the correlations by calculating the second-order correlation function in which the interference among the photons multiply scattered from the qubits causes rich structure. In one case, for example, transmitted and reflected photons are both bunched initially, but then become strongly anti-bunched for a long time interval. We first calculate the correlation function including non-Markovian effects and then show that a much simpler Markovian treatment, which can be solved analytically, is accurate for small qubit separation. As a result, the non-classical properties of microwaves in a 1D waveguide coupled to many superconducting qubits with experimentally accessible separation L could be readily explored with our approach.
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Quantum nonlinearity is an essential ingredient for many quantum technologies, but often the nonlinearity is too weak to be exploited at the few-photon level. However, few photons interacting strongly with single quantum emitters in a waveguide environment can impact a significant nonlinear response, opening up a wide range of photon-photon correlations. Using a waveguide-QED system containing a single atom (treated as a two-level system) chirally coupled to a waveguide, we theoretically investigate two-photon nonlinearities with delay-controlled temporal correlations. We use both matrix product states (MPS) and a frequency-dependent scattering theory approach to analyze the exact population dynamics, as well as the first-order and second-order photon correlation functions in transmission of the system, when pumped by a two-photon Fock-state pulse with a bimodal temporal pulse envelope. The two-photon Fock-state pulses are considered to be either two single photons localized to each peak of the pulse, or both photons delocalized (but correlated) between the two peaks. We consider the regimes of a short, moderate, and (relatively) long distance between the two pulse peaks, comparing the important differences in the temporal correlations with the two types of two-photon pulses. We demonstrate the strikingly different nonlinear features and quantum correlations that occur for uncorrelated and correlated two-photon pairs in experimentally accessible regimes.
We investigate the interaction between a single photon and a chain of NNN equally spaced two-level atoms inside a one-dimensional waveguide. By solving the eigenvectors of the Hamiltonian in the subspace with a single excitation, we address quantum interference effects in two physical processes. First, we analyze the scattering of a single photon when atoms are all initially at their ground states. We discover a set of transmission peaks determined by NNN. These transmission peaks are narrow and sensitive to the relative position between atoms. Second, we examine the spontaneous emission of a photon from an excited atom in the chain in vacuum. The characteristic atomic decay rates are found to be enhanced and reduced by increasing the number of atoms. In particular, the slowest decay rate scales approximately as ${N}^{\ensuremath{-}3}$.